Recent Advances in Organocatalytic Methods for Asymmetric CC Bond Formation
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Title
Recent Advances in Organocatalytic Methods for Asymmetric CC Bond Formation
Authors
Keywords
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Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 19, Issue 43, Pages 14346-14396
Publisher
Wiley
Online
2013-10-08
DOI
10.1002/chem.201301996
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- Novel pyrrolidine-thiohydantoins/thioxotetrahydropyrimidinones as highly effective catalysts for the asymmetric Michael addition
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- Asymmetric Aza-Mannich Addition: Synthesis of Modified Chiral 2-(Ethylthio)-thiazolone Derivatives with Anticancer Potency
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- Switching Regioselectivity in Crossed Acyloin Condensations between Aromatic Aldehydes and Acetaldehyde by AlteringN-Heterocyclic Carbene Catalysts
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- Enantioselective Direct Vinylogous Michael Addition of Functionalized Furanones to Nitroalkenes Catalyzed by an Axially Chiral Guanidine Base
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- Organocatalytic Sequential Michael Reactions: Stereoselective Synthesis of Multifunctionalized Tetrahydroindan Derivatives
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- Organocatalyzed Regio- and Enantioselective Allylic Trifluoromethylation of Morita–Baylis–Hillman Adducts Using Ruppert–Prakash Reagent
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- Development of a Formal Catalytic Asymmetric [4 + 2] Addition of Ethyl-2,3-butadienoate with Acyclic Enones
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- Highly Enantioselective Intermolecular Stetter Reactions of β-Aryl Acceptors: α-Ketoester Moiety as Handle for Activation and Synthetic Manipulations
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- Highly Enantioselective and Regioselective Substitution of Morita–Baylis–Hillman Carbonates with Nitroalkanes
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- Organocatalytic Asymmetric Aldol Reaction of Hydroxyacetone with β,γ-Unsaturated α-Keto Esters: Facile Access to Chiral Tertiary Alcohols
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- Organocatalytic Approach to Polysubstituted Piperidines and Tetrahydropyrans
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- Organocatalysis in Water at Room Temperature with In-Flask Catalyst Recycling
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- Tertiary Amine-Catalyzed Chemoselective and Asymmetric [3 + 2] Annulation of Morita–Baylis–Hillman Carbonates of Isatins with Propargyl Sulfones
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- Enantioselective Diels–Alder Reactions of Enals and Alkylidene Diketones Catalyzed by N-Heterocyclic Carbenes
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- Highly Regio- and Diastereoselective Construction of Spirocyclopenteneoxindoles through Phosphine-Catalyzed [3 + 2] Annulation of Morita–Baylis–Hillman Carbonates with Isatylidene Malononitriles
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- Highly Efficient Organocatalytic Kinetic Resolution of Activated Nitroallylic Acetates with Aldehydes via Conjugate Addition−Elimination
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- Formal Diels–Alder Reactions of Chalcones and Formylcyclopropanes Catalyzed by Chiral N-Heterocyclic Carbenes
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- N-(Heteroarenesulfonyl)prolinamides-Catalyzed Aldol Reaction between Acetone and Aryl Trihalomethyl Ketones
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- Organocatalytic Tail-to-Tail Dimerization of Olefin: Umpolung of Methyl Methacrylate Mediated by N-Heterocyclic Carbene
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- Highly Enantioselective Direct Vinylogous Michael Addition of γ-Butenolide to Enals
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- Organocatalytic Michael and Friedel–Crafts reactions in enantioselective synthesis of biologically active compounds
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- 1,6-Conjugated Addition of Nitromethane to (E)-2-Styrylchromones: A New Synthesis of Novel 2-Substituted 4-Arylpyrrole Derivatives
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- A sustainable procedure for highly enantioselective organocatalyzed Diels–Alder cycloadditions in homogeneous ionic liquid/water phase
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- Organocatalytic Michael Addition of Aldehydes to Protected 2-Amino-1-Nitroethenes: The Practical Syntheses of Oseltamivir (Tamiflu) and Substituted 3-Aminopyrrolidines
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- Recent Contributions from the Baylis−Hillman Reaction to Organic Chemistry
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- High-Yielding Synthesis of the Anti-Influenza Neuraminidase Inhibitor (−)-Oseltamivir by Two “One-Pot” Sequences
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- Organocatalytic Direct Vinylogous Michael Addition of α,β-Unsaturated γ-Butyrolactam to α,β-Unsaturated Aldehydes and an Illustration to Scaffold Diversity Synthesis
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- Asymmetric Conjugate Addition of Oxindoles to 2-Chloroacrylonitrile: A Highly Effective Organocatalytic Strategy for Simultaneous Construction of 1,3-Nonadjacent Stereocenters Leading to Chiral Pyrroloindolines
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- Enantioselective Organocatalytic Addition of Oxazolones to 1,1-Bis(phenylsulfonyl)ethylene: A Convenient Asymmetric Synthesis of Quaternary α-Amino Acids
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- Chiral Ionic Liquids Bearing O-Silylated α,α-Diphenyl (S)- or (R)-Prolinol Units: Recoverable Organocatalysts for Asymmetric Michael Addition of Nitroalkanes to α,β-Enals
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- Asymmetric 1,3-Dipolar Cycloaddition Reactions of Azomethine Imines with Acrolein Catalyzed by L-Proline and Its Derivatives
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- A General Approach for Preparation of Polymer-Supported Chiral Organocatalysts via Acrylic Copolymerization
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- Organocatalytic Enantioselective Synthesis of Both Diastereomers of α-Hydroxyphosphinates
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- Water-Compatible Iminium Activation: Highly Enantioselective Organocatalytic Michael Addition of Malonates to α,β-Unsaturated Enones
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- Highly Stereoselective and Scalableanti-Aldol Reactions UsingN-(p-Dodecylphenylsulfonyl)-2-pyrrolidinecarboxamide: Scope and Origins of Stereoselectivities
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- Chiral Amine Thiourea-Promoted Enantioselective Michael Addition Reactions of 3-Substituted Benzofuran-2(3H)-ones to Maleimides
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- Asymmetric Synthesis of Telcagepant, a CGRP Receptor Antagonist for the Treatment of Migraine
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- Highly Chemoselective Direct Crossed Aliphatic−Aromatic Acyloin Condensations with Triazolium-Derived Carbene Catalysts
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- Enantioselective Organocatalytic Biginelli Reaction: Dependence of the Catalyst on Sterics, Hydrogen Bonding, and Reinforced Chirality
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- Asymmetric Cyclopropanation of β,γ-Unsaturated α-Ketoesters with Stabilized Sulfur Ylides Catalyzed byC2-Symmetric Ureas
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- Enantioselective Organo-SOMO Cascade Cycloadditions: A Rapid Approach to Molecular Complexity from Simple Aldehydes and Olefins
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- Chiral Bisguanidine-Catalyzed Inverse-Electron-Demand Hetero-Diels−Alder Reaction of Chalcones with Azlactones
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- An Organocatalytic Asymmetric Nazarov Cyclization
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- Enantioselective Thiourea-Catalyzed Cationic Polycyclizations
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- Enantioselective Polyene Cyclization via Organo-SOMO Catalysis
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- Acyl Phosphonates: Good Hydrogen Bond Acceptors and Ester/Amide Equivalents in Asymmetric Organocatalysis
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- N-Heterocyclic Carbene-Catalyzed Cascade Reaction Involving the Hydroacylation of Unactivated Alkynes
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- An Enantioselective Claisen Rearrangement Catalyzed by N-Heterocyclic Carbenes
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- Main-Chain Ionic Chiral Polymers: Synthesis of Optically Active Quaternary Ammonium Sulfonate Polymers and Their Application in Asymmetric Catalysis
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- N-silyl oxyketene imines are underused yet highly versatile reagents for catalytic asymmetric synthesis
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- Organocatalytic cascade reactions as a new tool in total synthesis
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- Organocatalytic kinetic resolution via intramolecular aldol reactions: Enantioselective synthesis of both enantiomers of chiral cyclohexenones
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- Organocatalytic asymmetric intramolecular [3+2] cycloaddition: A straightforward approach to access multiply substituted hexahydrochromeno[4,3-b]pyrrolidine derivatives in high optical purity
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- A New Powerful Strategy for the Organocatalytic Asymmetric Construction of a Quaternary Carbon Stereogenic Center
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- Enantioselective Total Synthesis of (+)-Conicol via Cascade Three-Component Organocatalysis
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- Friedel−Crafts Acylation of Pyrroles and Indoles using 1,5-Diazabicyclo[4.3.0]non-5-ene (DBN) as a Nucleophilic Catalyst
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- Direct Asymmetric Aldol Reaction with Recyclable Fluorous Organocatalyst
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- Primary Amine/(+)-CSA Salt-Promoted Organocatalytic Conjugate Addition of Nitro Esters to Enones
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- Enantio- and Diastereoselective Synthesis of Piperidines by Coupling of Four Components in a “One-Pot” Sequence Involving Diphenylprolinol Silyl Ether Mediated Michael Reaction
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- Crystal structures of proline-derived enamines
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- Direct asymmetric vinylogous Michael addition of cyclic enones to nitroalkenes via dienamine catalysis
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- Asymmetric Cooperative Catalysis of Strong Bronsted Acid-Promoted Reactions Using Chiral Ureas
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- The enantioselective intramolecular Morita–Baylis–Hillman reaction catalyzed by amino acid-derived phosphinothiourea
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- The NHCs-mediated cross-coupling of aromatic aldehydes with benzyl halides: synthesis of α-aryl ketones
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- Synthesis and use of a stable aminal derived from TsDPEN in asymmetric organocatalysis
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- Organocatalytic approach to 3,5,6-trisubstituted and 4,6-disubstituted tetrahydropyran-2-ones
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- Novel polymer-supported organocatalyst via ion exchange reaction: facile immobilization of chiral imidazolidin-4-one and its application to Diels–Alder reaction
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- The highly enantioselective 1,3-dipolar cycloaddition of alkyl glyoxylate-derived nitrones to E-crotonaldehyde catalyzed by hybrid diamines
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- Nucleophilic acylation of α-haloketones with aldehydes: an umpolung strategy for the synthesis of 1,3-diketones
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- Performance of C1-symmetric chiral ammonium betaines as catalysts for the enantioselective Mannich-type reaction of α-nitrocarboxylates
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- Enantioselective intramolecular Morita–Baylis–Hillman reaction using chiral bifunctional phosphinothiourea as an organocatalyst
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- One-step, efficient synthesis of combined threonine–surfactant organocatalysts for the highly enantioselective direct aldol reactions of cyclic ketones with aromatic aldehydes in the presence of water
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- Thiazolidine-based organocatalysts for a highly enantioselective direct aldol reaction
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- Stereoselective synthesis of functionalised cyclopropanes from nitroalkenes via an organocatalysed Michael-initiated ring-closure approach
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- Studies on the asymmetric, phosphine-promoted [3+2] annulations of allenic esters with 2-aryl-1,1-dicyanoalkenes
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- Organocatalyst-mediated enantioselective intramolecular Michael addition of aldehydes to vinyl sulfones
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- Highly enantio-, regio- and diastereo-selective one-pot [2 + 3]-cycloaddition reaction via isomerization of 3-butynoates to allenoates,
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- Ionic liquid mediated recyclable sulphonimide based organocatalysis for aldol reaction
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- Enantiodivergent Organocascade Reactions
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- Polarity-Directed One-Pot Asymmetric Cascade Reactions Mediated by Two Catalysts in an Aqueous Buffer
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- Anodic Oxidation and Organocatalysis: Direct Regio- and Stereoselective Access to meta-Substituted Anilines by α-Arylation of Aldehydes
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- Gold and Organocatalysis Combined
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- Flexible synthesis, structural determination, and synthetic application of a new C1-symmetric chiral ammonium betaine
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- Catalytic asymmetric direct Mannich reaction: a powerful tool for the synthesis of α,β-diamino acids
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- Enantioselective Synthesis of α-Fluorinated β-Amino Acid Derivatives by an Asymmetric Mannich Reaction and Selective Deacylation/Decarboxylation Reactions
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- Expanding the Scope of Enantioselective FerroPHANE-Promoted [3+2] Annulations with α,β-Unsaturated Ketones
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- Organocatalytic Domino Reactions
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- 2-Pyrrolidinecarboxylic Acid Ionic Liquid as a Highly Efficient Organocatalyst for the Asymmetric One-Pot Mannich Reaction
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- Synthesis of Chiral 3-Substituted Phthalides by a Sequential Organocatalytic Enantioselective Aldol-Lactonization Reaction. Three-Step Synthesis of (S)-(−)-3-Butylphthalide
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- Enantioselective Brønsted Acid-CatalyzedN-Acyliminium Cyclization Cascades
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- Diarylprolinol Silyl Ether Salts as New, Efficient, Water-Soluble, and Recyclable Organocatalysts for the Asymmetric Michael Addition on Water
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- Enamine Catalysis with Low Catalyst Loadings - High Efficiency via Kinetic Studies
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- Enantioselective construction of lactone[2,3-b]piperidine skeletons via organocatalytic tandem reactions
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- Asymmetric Michael addition reaction of 3-substituted-N-Boc oxindoles to activated terminal alkenes catalyzed by a bifunctional tertiary-amine thiourea catalyst
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- Enamine-Iminium Ion Nazarov Cyclization of α-Ketoenones
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- Microwave-Assisted Organocatalytic Quadruple Domino Reactions of Acetaldehyde and Nitroalkenes
- (2009) Dieter Enders et al. SYNTHESIS-STUTTGART
- Chiral phosphinothiourea-catalyzed asymmetric Morita–Baylis–Hillman reactions of acrylates with aromatic aldehydes
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- A new (S)-prolinamide modified by an ionic liquid moiety—a high performance recoverable catalyst for asymmetric aldol reactions in aqueous media
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- One-pot highly enantioselective catalytic Mannich-type reactions between aldehydes and stable α-amido sulfones: asymmetric synthesis of β-amino aldehydes and β-amino acids
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- Organocatalytic Reactions with Acetaldehyde
- (2008) Benito Alcaide et al. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
- Asymmetric Alkaloid Synthesis: A One-Pot Organocatalytic Reaction to Quinolizidine Derivatives
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- Chiral Tetraaminophosphonium Carboxylate-Catalyzed Direct Mannich-Type Reaction
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- A novel (S)-proline-modified task-specific chiral ionic liquid—an amphiphilic recoverable catalyst for direct asymmetric aldol reactions in water
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- Organocatalysed asymmetric Mannich reactions
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