Article
Biotechnology & Applied Microbiology
Meng Wang, Qida Hu, Junmin Huang, Xinyu Zhao, Shiyi Shao, Fu Zhang, Zhuo Yao, Yuan Ping, Tingbo Liang
Summary: The dual-targeting nanomedicine, PG@KMCM, was developed to target tumor-associated macrophages and reprogram the tumor microenvironment, enhancing the therapeutic potential against pancreatic cancer. Combination with PD-L1 immune checkpoint inhibitor further improved the anti-tumoral effect by reprograming the immune-suppressive tumor microenvironment.
JOURNAL OF NANOBIOTECHNOLOGY
(2022)
Article
Materials Science, Multidisciplinary
Jianhua Liu, Zhongmin Li, Duoyi Zhao, Xiangru Feng, Chunxi Wang, Di Li, Jianxun Ding
Summary: Nanomedicine-based chemotherapeutic formulations can induce immunogenic cell death, which enhances the effectiveness of combination chemoimmunotherapy. The combination of these formulations with immunoactivating agents is a promising strategy for clinical cancer treatment.
MATERIALS & DESIGN
(2021)
Article
Engineering, Biomedical
Qian Wang, Weiji Qin, Lei Qiao, Min Gao, Man Zhou, Huiru Zhang, Qiuting Sun, Wanqing Yao, Tianhao Yang, Xiaohe Ren, Gengyun Sun, Xiaoyan He
Summary: A photo-activated ROS amplifying system is developed to induce antitumor immune response and improve the efficacy of immunotherapy in cancer treatment.
ADVANCED HEALTHCARE MATERIALS
(2023)
Review
Chemistry, Physical
Guojun Huang, Lanlan Liu, Hong Pan, Lintao Cai
Summary: This review summarizes the recent advances in using biomimetic active materials to guide immunogenic cell death (ICD) for cancer immunotherapy. It introduces two main strategies, including naive organism-derived nanoagents and engineered bioactive platforms. The challenges and future developments of using biomimetic active materials guided ICD in cancer immunotherapy applications are also discussed.
Article
Chemistry, Multidisciplinary
Fan Zhang, Fangman Chen, Chao Yang, Lei Wang, Hanze Hu, Xuezhao Li, Xiao Zheng, Zheng Wang, Zhimin Chang, Tianyu Li, Li Li, Mingfeng Ge, Jinzhi Du, Wen Sun, Wen-Fei Dong, Dan Shao
Summary: The potential ICD nanoamplifier containing diselenide-bridged mesoporous organosilica nanoparticles (MONs) and chemotherapeutic ruthenium compound (KP1339) showed controlled drug release profiles and evoked robust antitumor immunological responses by amplifying ICD of KP1339.
Article
Pharmacology & Pharmacy
Xiaoxian Huang, Lingfei Han, Ruyi Wang, Wanfang Zhu, Ning Zhang, Wei Qu, Wenyuan Liu, Fulei Liu, Feng Feng, Jingwei Xue
Summary: A dual-responsive prodrug micelle is designed to co-deliver a TGF-beta receptor inhibitor and a chemotherapy drug to remodel the tumor microenvironment and trigger immunogenic cell death, thereby inducing an antitumor immune response.
Article
Chemistry, Multidisciplinary
Yuan Ding, Zhongquan Sun, Yong Gao, Sitong Zhang, Caixia Yang, Zhefeng Qian, Lulu Jin, Jiaojiao Zhang, Cheng Zeng, Zhengwei Mao, Weilin Wang
Summary: Clinical trials have shown that combining IDO blockade with immunogenic chemotherapy has great potential in cancer therapy. A hybrid nanomedicine was designed to co-deliver an IDO inhibitor and a chemotherapeutic prodrug, effectively activating chemo-immunotherapy and overcoming the immunosuppressive tumor microenvironment, leading to tumor growth suppression.
ADVANCED MATERIALS
(2021)
Article
Multidisciplinary Sciences
Xiangru Feng, Weiguo Xu, Jianhua Liu, Di Li, Gao Li, Jianxun Ding, Xuesi Chen
Summary: Conventional chemotherapeutics induce immunogenic cell death in tumor cells, but are limited by the presence of immunosuppressive lymphocytes in the tumor microenvironment. Combining low-dose DOX with 1MT to overcome immune suppression, delivered via a reduction-responsive polypeptide nanogel, effectively suppressed tumor growth and enhanced CD8(+) T cell frequency. The chemoimmunotherapy strategy shows great potential in clinical cancer therapy.
Article
Pharmacology & Pharmacy
Xinlong Zang, Jingyi Zhou, Xiaoxu Zhang, Dawei Chen, Yantao Han, Xuehong Chen
Summary: CaZOL@BMNPs is a dual-targeting drug delivery system that reduced angiogenesis, reprogrammed the immunosuppressive tumor microenvironment, and inhibited the progression of NSCLC with negligible systemic toxicity.
INTERNATIONAL JOURNAL OF PHARMACEUTICS
(2021)
Article
Chemistry, Multidisciplinary
Hsuan-Yu Mu, Yen-Nhi Ngoc Ta, Max Jing Rui Tham, Fu-Fei Hsu, Yu-Chieh Lin, Hsi-Chien Huang, Yun-Chieh Sung, Chih- Huang, Ching-Ling Wu, Chao-Hung Chang, Sheng Yang, Tsung-Ying Lee, Dehui Wan, Jane Wang, Dan G. Duda, Yves Boucher, Jen-Huang Huang, Wee Han Ang, Yunching Chen
Summary: A new chemoimmunotherapy nanogel (IL2-Pt@Nanogel) capable of delivering IL-2 and Pt-NHC has been developed. This nanogel reduces the immunosuppressive phenotype of tumor-associated macrophages and regulatory T cell infiltration, and can change the tumor microenvironment to an immunostimulatory state. Combining this nanogel with the angiotensin II receptor blocker losartan can further reduce desmoplasia and enhance the anti-tumor efficacy in models of primary and metastatic PDAC and HCC with liver fibrosis. This study presents a promising IL-2-based chemoimmunotherapy strategy for the treatment of solid tumors.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Engineering, Biomedical
Mingqi Chen, Yucui Shen, Yinying Pu, Bangguo Zhou, Jinhong Bing, Min Ge, Yaxuan Zhu, Shuang Gao, Wencheng Wu, Min Zhou, Jianlin Shi
Summary: This study reports a novel biomimetic ferroptosis inducer capable of regulating the immunosuppressive tumor microenvironment for enhanced cancer ferroptosis immunotherapy. The inducer triggers both cancer cell and TAMs ferroptosis, activating the anticancer immune response and favoring the normalization of the tumor microenvironment.
Article
Nanoscience & Nanotechnology
Mingxia Jiang, Wenqiang Chen, Wenjing Yu, Zhiwei Xu, Xinyue Liu, Qingmiao Jia, Xiuwen Guan, Weifen Zhang
Summary: The sequentially pH-responsive DOX delivery nanosystem designed for simultaneous chemotherapy and tumor immunogenic cell death holds great potential for cancer chemoimmunotherapy, by utilizing immune checkpoint blockade to enhance antitumor activity.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Kaipei Luo, Lu Yang, Chunmei Yan, Yuxin Zhao, Qiuxia Li, Xing Liu, Long Xie, Qiang Sun, Xiaofang Li
Summary: This study develops a dual-modified liposome loaded with paclitaxel and cryptotanshinone for triple-negative breast cancer chemoimmunotherapy, which enhances cellular uptake and induces immunogenic cell death while inhibiting STAT3 activation.
Article
Engineering, Biomedical
Qilin Li, Jia Liu, Huiling Fan, Lin Shi, Yan Deng, Lei Zhao, Mengxi Xiang, Yunruo Xu, Xulin Jiang, Guobin Wang, Lin Wang, Zheng Wang
Summary: This study introduces a nano system that co-delivers immunogenic chemodrugs and IDO inhibitors to cancer cells, effectively reducing immunosuppression and promoting antitumor immune responses. The system shows promising results in preclinical cancer models, indicating its strong translational potential for clinical applications.
Article
Pharmacology & Pharmacy
Zheng Zeng, Yu Liu, Qinglian Wen, Yixian Li, Jing Yu, Qiang Xu, Wenwu Wan, Yu He, Chen Ma, Yan Huang, Helin Yang, Ou Jiang, Fuyu Li
Summary: The study aimed to develop a novel therapy targeting M2 macrophages, using MIC-NPs to inhibit M2 cell growth effectively and have a positive impact on anti-tumor immune responses.
Article
Chemistry, Multidisciplinary
He Wang, Yi-sha Du, Wen-shuo Xu, Chang-jian Li, Hong Sun, Kang-rui Hu, Yuan-zhuo Hu, Teng-jie Yu, Hui-min Guo, Lin Xie, Guang-ji Wang, Yan Liang
Summary: The study demonstrates that exogenous GSH exerts a therapeutic effect on ischemic stroke by increasing intrastriatal DA levels in rats. The accumulated DA enhances the exposure of GSH and its related substances, thereby promoting the therapeutic effect of GSH.
ACTA PHARMACOLOGICA SINICA
(2022)
Article
Chemistry, Multidisciplinary
Bin Wang, Zongyu Cai, Siliang Chen, Ya Chen, Shixuan Jiao, Qiang Ren, Xuekun Wang, Xinqian Geng, Zheng Li, Guangji Wang
Summary: This study successfully developed a partial agonist of the free fatty acid receptor 1 (FFA1) with reduced lipophilicity, which showed good activity in lowering blood glucose.
Article
Oncology
Mengjie Yu, Wei Wen, Xin Yi, Wei Zhu, Jiye Aa, Guangji Wang
Summary: This study found impaired oxidative stress function in ESCC patients and identified risk metabolites associated with the development of ESCC. The levels of alpha-tocopherol and cysteine decreased progressively, while the levels of aminomalonic acid increased progressively. A high level of aminomalonic acid was a risk factor for the development of ESD to ESCC and for lymphatic metastasis in ESCC patients. A low level of alpha-tocopherol was an independent risk factor for ESCC. The panel constructed by glycolic acid, oxalic acid, glyceric acid, malate, and alpha-tocopherol performed well in distinguishing ESD/ESCC from healthy controls.
FRONTIERS IN ONCOLOGY
(2022)
Article
Engineering, Biomedical
Suleixin Yang, Peng Hua, Chengwei He, Hua Yu, Dan Shao, Zhi Shi, Meiwan Chen, Ka Hong Wong
Summary: In this study, a ferroptosis/apoptosis combinational therapy was achieved by depleting GSH and downregulating GPX4 to disrupt redox homeostasis and amplify ferroptosis-related oxidation effect. ROS-responsive serum-resistant nanoparticles were used to co-deliver shGPX4 and shMTHFD2 plasmids, leading to efficient transfection, lysosomal escape, and induction of ferroptosis and apoptosis in tumor cells.
ACTA BIOMATERIALIA
(2022)
Article
Immunology
Youying Zhang, Qilin Fan, Yuanlong Hou, Xuanshuang Zhang, Zhe Yin, Xiaoying Cai, Wei Wei, Jiaying Wang, Dandan He, Guangji Wang, Yonggui Yuan, Haiping Hao, Xiao Zheng
Summary: Disturbances in gut microbiome, particularly Bacteroides species, are implicated in major depressive disorder (MDD) susceptibility. This study demonstrates the differential impacts of Bacteroides fragilis, Bacteroides uniformis, Bacteroides caccae, and Bacteroides ovatus on depressive behavior and neurogenesis. The effects are partially mediated by alterations in tryptophan pathway metabolites and neurotransmitters along the gut-brain axis. Moreover, the intensified depletion of cerebral serotonin is associated with increased susceptibility to depression.
BRAIN BEHAVIOR AND IMMUNITY
(2022)
Article
Chemistry, Multidisciplinary
Ya-Wen Xu, Bi-Xin Xu, Jiankun Wang, Hao-Wen Jin, Si-Tao Xu, Guangji Wang, Le Zhen
Summary: The newly emerging persulfide prodrugs provide more options for studying persulfide, a molecule with potential biological functions and disease intervention. By designing prodrugs with a 2-oxo-2-phenylacetamide trigger, persulfide can be released through 1,6-N, S-relay. These prodrugs have been shown to degrade and form persulfide in a peroxynitrite-responsive manner. Additionally, the prodrugs exhibit potent peroxynitrite scavenging activity and therapeutic potential in cellular models. Evaluation of their in vitro metabolic properties is also favorable.
CHEMISTRY-A EUROPEAN JOURNAL
(2022)
Article
Biochemical Research Methods
Zixin Jiao, Zhenyao Lu, Ying Peng, Chen Xu, Yunge Lou, Guangji Wang, Jiye Aa, Yue Zhang
Summary: The study developed a simple, fast, and reliable method for simultaneous detection of 14 methionine-related metabolites. This method can help understand the mechanisms involved in methylation and redox homeostasis in cellular metabolomic studies.
JOURNAL OF CHROMATOGRAPHY B-ANALYTICAL TECHNOLOGIES IN THE BIOMEDICAL AND LIFE SCIENCES
(2022)
Article
Oncology
Luyao Ao, Shencun Fang, Kexin Zhang, Yang Gao, Jiawen Cui, Wenjing Jia, Yunlong Shan, Jingwei Zhang, Guangji Wang, Jiali Liu, Fang Zhou
Summary: Combined therapy of pemetrexed and aumolertinib shows synergistic effects in a sequence- and EGFR mutant-dependent manner, with aumolertinib following pemetrexed demonstrating the strongest anti-tumor growth and anti-metastasis abilities. Clinical retrospective study confirms the superiority of this combination therapy over aumolertinib monotherapy in terms of tumor response.
JOURNAL OF EXPERIMENTAL & CLINICAL CANCER RESEARCH
(2022)
Article
Chemistry, Medicinal
Yun Wang, Yuanyuan Xu, Xiaowei Xu, Hong Wang, Dong Wang, Wenchao Yan, Jiaying Zhu, Haiping Hao, Guangji Wang, Lijuan Cao, Jun Zhang
Summary: This study confirmed the beneficial effects of Ginkgo biloba leave extract (GbE) in alleviating hypercholesterolemia, inflammation, and atherosclerosis. GbE treatment reshaped the intestinal microbiota, downregulated proinflammatory cytokines, and enhanced the expression of tight junction proteins. It also reversed the dysfunction of microbial metabolic phenotypes and reduced atherosclerotic plaque areas. These findings provide important insights into the pharmacological mechanism underlying the antiatherogenic efficacy of GbE.
PHYTOTHERAPY RESEARCH
(2022)
Article
Pharmacology & Pharmacy
Hong-can Ren, Jian-guo Sun, A. Ji-ye, Sheng-hua Gu, Jian Shi, Feng Shao, Hua Ai, Jing-wei Zhang, Ying Peng, Bei Yan, Qing Huang, Lin-sheng Liu, Yang Sai, Guang-ji Wang, Cheng-guang Yang
Summary: This study aimed to investigate the pharmacokinetics of the deglycosylation metabolite PPD following Rh2 administration and develop a mechanism-based pharmacokinetic model. Results showed that a certain percentage of Rh2 was transformed into PPD and entered systemic circulation, highlighting the importance of studying deglycosylation kinetics for future pharmacokinetic studies of similar drugs.
FRONTIERS IN PHARMACOLOGY
(2022)
Article
Pharmacology & Pharmacy
Yunlong Shan, Qi Ni, Qixiang Zhang, Mengying Zhang, Bin Wei, Lingge Cheng, Chongjin Zhong, Xinyu Wang, Qingqing Wang, Jiali Liu, Jingwei Zhang, Jingjing Wu, Guangji Wang, Fang Zhou
Summary: This study reveals a potential strategy to improve immunotherapy by targeting the abnormal metabolism of tumor endothelial cells (TECs). Osimertinib inhibits the activity of glyceraldehyde-3-phosphate dehydrogenase (GAPDH) in TECs, leading to reduced secretion of immune inhibitory factors and increased infiltration of immune effector cells in the tumor microenvironment.
ACTA PHARMACEUTICA SINICA B
(2022)
Article
Chemistry, Multidisciplinary
Jing Wu, Yun-ge Lou, Xu-le Yang, Rui Wang, Ran Zhang, Ji-ye Aa, Guang-ji Wang, Yuan Xie
Summary: This study found that ER stress plays a crucial role in the inhibition of P450s activity in NAFLD, and silybin regulates P450s activity by attenuating ER stress. Silybin can restore the activity of P450s in liver microsomes and may have potential benefits for the treatment of NAFLD.
ACTA PHARMACOLOGICA SINICA
(2023)
Article
Biochemical Research Methods
Ning Wan, Nian Wang, Siqin Yu, Hanqing Zhang, Shuo Tang, Dexiang Wang, Wenjie Lu, Huanhuan Li, Daniel G. Delafield, Ying Kong, Xinmiao Wang, Chang Shao, Langlang Lv, Guangji Wang, Renxiang Tan, Nanxi Wang, Haiping Hao, Hui Ye
Summary: This article reports the use of cyclic immonium ion as a diagnostic fragment ion for lysine lactylation. The study shows that lactylation is not only limited to histones but also occurs on nonhistone proteins. Through the use of affinity-enriched lactylproteome analysis and informatic assessment, the authors confidently identified new lactylation sites beyond histones. The study also demonstrated the functional importance of lactylation, specifically in glycolysis.
Article
Chemistry, Analytical
Zhenyao Lu, Sijia Li, Nan Aa, Yuanmao Zhang, Ran Zhang, Chen Xu, Shize Zhang, Xiangqing Kong, Guangji Wang, Jiye Aa, Yue Zhang
Summary: In this study, a simple method was developed to simultaneously determine the levels of 20 metabolites related to purine and pyrimidine metabolism. The method was evaluated and found to be accurate, sensitive, and reliable. It was successfully applied to study mice with chronic social defeat stress-induced depression, revealing perturbations in purine metabolism and demonstrating the potential of this method in exploring metabolism-related mechanisms of relevant diseases.
JOURNAL OF PHARMACEUTICAL AND BIOMEDICAL ANALYSIS
(2022)
Article
Plant Sciences
Kangrui Hu, Changjian Li, Tengjie Yu, Huimin Guo, Hong Sun, Shuying Mao, Zhihao Zhou, Wei Jin, Keanqi Liu, Lin Xie, Guangji Wang, Yan Liang
Summary: This study developed a reliable and efficient strategy to investigate the metabolism of active components of traditional Chinese medicine in target organs. The results revealed that NG-R1 was mainly converted to Rg1 in the intestinal flora, while it existed mainly in prototype form in the liver and brain.
Article
Engineering, Environmental
Xinping Zhang, Yuxin Guo, Xiaoyang Liu, Shun-Yu Wu, Ya-Xuan Zhu, Shao-Zhe Wang, Qiu-Yi Duan, Ke-Fei Xu, Zi-Heng Li, Xiao-Yu Zhu, Guang-Yu Pan, Fu-Gen Wu
Summary: This study develops a nanotrigger HCFT for simultaneous photodynamic therapy and light-triggered ferroptosis therapy. The nanotrigger can relieve tumor hypoxia, induce enhanced photodynamic reaction, and facilitate the continuation of Fenton reaction, ultimately leading to lethal ferroptosis in tumor cells.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Olumide Bolarinwa Ayodele, Toyin Daniel Shittu, Olayinka S. Togunwa, Dan Yu, Zhen-Yu Tian
Summary: This study focused on the semihydrogenation of acetylene in an ethylene-rich stream using two alloyed Pt catalysts PtCu and PtCo. The PtCu catalyst showed higher activity and ethylene yield compared to PtCo due to its higher unoccupied Pt d-orbital density. This indicates that alloying Pt with Cu is more promising for industrial relevant SHA catalyst.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Guowei Chen, Wen-Cheng Chen, Yaozu Su, Ruicheng Wang, Jia-Ming Jin, Hui Liang, Bingxue Tan, Dehua Hu, Shaomin Ji, Hao-Li Zhang, Yanping Huo, Yuguang Ma
Summary: This study proposes an intramolecular dual-locking design for organic luminescent materials, achieving high luminescence efficiency and performance for deep-blue organic light-emitting diodes. The material also exhibits unique mechanochromic luminescence behavior and strong fatigue resistance.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Joren van Stee, Gregory Hermans, Jinu Joseph John, Koen Binnemans, Tom Van Gerven
Summary: This work presents a continuous solvent extraction method for the separation of cobalt and nickel in a millifluidic system using Cyphos IL 101 (C101) as the extractant. The optimal conditions for extraction performance and solvent properties were determined by investigating the effects of channel length, flow rate, and temperature. The performance of a developed manifold structure was compared to a single-channel system, and excellent separation results were achieved. The continuous separation process using the manifold structure resulted in high purity cobalt and nickel products.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Yan Xu, Jingai Jiang, Xinyi Lv, Hui Li, Dongliang Yang, Wenjun Wang, Yanling Hu, Longcai Liu, Xiaochen Dong, Yu Cai
Summary: A programmed gas release nanoparticle was developed to address the challenges in treating diabetic infected wounds. It effectively removes drug-resistant pathogens and remodels the wound microenvironment using NO and H2S. The nanoparticle can eliminate bacteria and promote wound healing through antibacterial and anti-inflammatory effects.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Tong Xia, Zhilin Xi, Lianquan Suo, Chen Wang
Summary: This study investigated a highly efficient coal dust suppressant with low initial viscosity and high adhesion-solidification properties. The results demonstrated that the dust suppressant formed a network of multiple hydrogen bonding cross-linking and achieved effective adhesion and solidification of coal dust through various chemical reactions.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Jinzhi Cai, Zhenshan Li
Summary: A density functional theory-based rate equation was developed to predict the gas-solid reaction kinetics of CaO carbonation with CO2 in calcium looping. The negative activation energy of CaO carbonation close to equilibrium was accurately predicted through experimental validation.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Jianxiong Chen, Fuhao Ren, Ningning Yin, Jie Mao
Summary: This study presents an economically efficient and easily implementable surface modification approach to enhance the high-temperature electrical insulation and energy storage performance of polymer dielectrics. The self-assembly of high-insulation-performance boron nitride nanosheets (BNNS) on the film surface through electrostatic interactions effectively impedes charge injection from electrodes while promoting charge dissipation and heat transfer.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Zijian Li, Zhaohui Yang, Shao Wang, Hongxia Luo, Zhimin Xue, Zhenghui Liu, Tiancheng Mu
Summary: This study reports a strategy for upgrading polyester plastics into value-added chemicals using electrocatalytic methods. By inducing the targeted transfer of *OH species, polyethylene terephthalate was successfully upgraded into potassium diformate with high purity. This work not only develops an excellent electrocatalyst, but also provides guidance for the design of medium entropy metal oxides.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Navneet Singh Shekhawat, Surendra Kumar Patra, Ashok Kumar Patra, Bamaprasad Bag
Summary: This study primarily focuses on developing a sulphur dyeing process at room temperature using bacterial Lysate, which is environmentally friendly, energy and cost effective, and sustainable. The process shows promising improvements in dye uptake and fastness properties.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Dengjia Shen, Hongyang Ma, Madani Khan, Benjamin S. Hsiao
Summary: This study developed cationic PVC nanofibrous membranes with high filtration and adsorption capability for the removal of bacteria and hexavalent chromium ions from wastewater. The membranes demonstrated remarkable performance in terms of filtration efficiency and maximum adsorption capacity. Additionally, modified nanofibrous membranes were produced using recycled materials and showed excellent retention rates in dynamic adsorption processes.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Xiaoyan Wang, Zhikun Wang, Ben Jia, Chunling Li, Shuangqing Sun, Songqing Hu
Summary: Inspired by photosystem II, self-supported Fe-doped NiCoP nanowire arrays modified with carboxylate were constructed to boost industrial-level overall water splitting by employing the concerted proton-coupled electron transfer mechanism. The introduction of Fe and carboxyl ligand led to improved catalytic activity for HER and OER, and NCFCP@NF exhibited long-term durability for overall water splitting.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Pengyao Yu, Ge Yang, Yongming Chai, Lubomira Tosheva, Chunzheng Wang, Heqing Jiang, Chenguang Liu, Hailing Guo
Summary: Thin LTA zeolite membranes were prepared through secondary growth of nano LTA seeds in a highly reactive gel, resulting in membranes with superior permeability and selectivity in gas separation applications.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Baiqin Zhou, Huiping Li, Ziyu Wang, Hui Huang, Yujun Wang, Ruichun Yang, Ranran Huo, Xiaoyan Xu, Ting Zhou, Xiaochen Dong
Summary: The use of machine learning to predict the performance of specific adsorbents in phosphate adsorption shows great promise in saving time and revealing underlying mechanisms. However, the small size of the dataset and insufficient detailed information limits the model training process and the accuracy of results. To address this, the study employs a fuzzing strategy that replaces detailed numeric information with descriptive text messages on the physiochemical properties of adsorbents. This strategy allows the recovery of discarded samples with limited information, leading to accurate prediction of adsorption amount, capacity, and kinetics. The study also finds that phosphate uptake by adsorbents is generally through physisorption, with some involvement of chemisorption. The framework established in this study provides a practical approach for quickly predicting phosphate adsorption performance in urgent scenarios, using easily accessible information.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Paula Alejandra Lamprea Pineda, Joren Bruneel, Kristof Demeestere, Lisa Deraedt, Tex Goetschalckx, Herman Van Langenhove, Christophe Walgraeve
Summary: This study evaluates the use of four esterified fatty acids and three vegetable oils as absorption liquids for hydrophobic VOCs. The experimental results show that isopropyl myristate is the most efficient liquid for absorbing the target VOCs.
CHEMICAL ENGINEERING JOURNAL
(2024)