Article
Chemistry, Physical
Chen Li, Tianyi Sun, Dashuai Zhang, Xiaopeng Zhang, Yuehua Qian, Yan Zhang, Xiaoxue Lin, Jinrui Liu, Linhua Zhu, Xianghui Wang, Zaifeng Shi, Qiang Lin
Summary: The ternary Ag/La-TiO2-x heterojunctions were successfully prepared for photocatalytic degradation of tetracycline under visible light irradiation. The as-prepared composites showed excellent visible-light photocatalytic activity due to higher photoinduced charge separation efficiency. The mechanism of photocatalytic degradation of tetracycline by Ag/La-TiO2-x composites was discussed, highlighting the significant potential applications in energy conversion and environmental remediation.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Environmental Sciences
Mengxue Li, Mengmeng Chen, Stephanie Ling Jie Lee, Sijie Lin
Summary: A nanocomposite consisting of CoFe-layered double hydroxides grown on graphitic carbon nitride nanosheets (CoFe-LDH/g-C3N4) has been successfully synthesized and exhibits significant photocatalytic activity for the degradation of tetracycline. The enhanced performance is attributed to the intimate interfacial contact, enlarged surface area, broadened absorbance range, and improved electron transfer. This study demonstrates the feasibility and potential application of the nanocomposite for the removal of tetracycline from contaminated water.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2023)
Article
Chemistry, Multidisciplinary
Mitra Malekkiani, Fatemeh Ravari, Abbas Heshmati Jannat Magham, Mehdi Dadmehr, Heiko Groiss, Hasan Ali Hosseini, Reza Sharif
Summary: The synthesis of core-shell heterostructures composed of titanium oxide and cerium oxide deposited on reduced graphene oxide was described. These heterostructures showed superior photocatalytic performance for the degradation of organic pollutants, attributed to effective electron-hole separation and charge recombination suppression. Biological assay demonstrated low cytotoxicity against breast cancer cells.
Article
Materials Science, Ceramics
Minggao Song, Mingchun Li, Yintong Guo, Xiyao Huang, Sijin Wang, Long Ren, Laishi Li, Yusheng Wu
Summary: A series of assembled porous TiO2/g-C3N4 (TC) powders were synthesized by controlling the molar ratio of urea to tetrabutyl titanate (TBOT) in a hydrothermal process, resulting in hierarchical nanosheets with uniform mesopores and interconnected macropores. The material showed outstanding photocatalytic behavior towards Rhodamine B and tetracycline hydrochloride degradation, with degradation efficiencies remaining above 90% even after five consecutive cycles.
CERAMICS INTERNATIONAL
(2021)
Article
Materials Science, Multidisciplinary
Lu Yang, Yong Liu, Pengfei Tan, Ying Lu, Qingguo Ding, Jun Pan
Summary: An innovative g-C3N4-TiO2@CsPbBr3 composite catalyst was prepared and demonstrated to have enhanced photocatalytic performance for tetracycline hydrochloride degradation. The catalyst exhibited increased light-harvesting capability and more efficient charge carrier separation, leading to a degradation rate of 75.6% in 120 min, which was 2.30 and 2.03 times higher than TiO2@CPB and pure g-C3N4, respectively. The study also identified O-2(-) as the dominant active specie in the photocatalytic degradation process and proposed a possible photocatalytic mechanism.
DIAMOND AND RELATED MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Reda M. Mohamed, Adel A. Ismail, Mohammad W. Kadi, Ajayb S. Alresheedi, Ibraheem A. Mkhalid
Summary: This study demonstrates the enhanced photocatalytic performance of PtO-ZnO nanocomposites for tetracycline degradation. The optimized 0.6% PtO-ZnO catalyst showed exceptional degradation efficiency, outperforming pristine ZnO and commercial P-25. The PtO-ZnO nanocomposites exhibited high stability and recyclability, making them promising for wastewater treatment applications.
Article
Materials Science, Multidisciplinary
Qianru Zhao, Shuangyang Chen, Binghua Ren, Sinan Liu, Yongchao Zhang, Xi Luo, Wei Feng, Yan Sun
Summary: Rutile TiO2 microspheres and WO3 nanosheets were synthesized via hydrothermal treatment, and a WO3/TiO2 heterojunction was prepared with different mass ratios using physical mixing. Photocatalytic performance was evaluated using the degradation of Rhodamine B dye under simulated sunlight. The WO3/TiO2 with a mass ratio of 1:5 showed the highest photocatalytic efficiency of 91.5% within 60 minutes. Holes (h(+)) and superoxide radical (center dot O-2(-)) were found to play key roles in the degradation process. The unique type-II WO3/TiO2 heterojunction extended the light absorption range and improved photocatalytic activity.
Article
Environmental Sciences
Almudena Aguinaco, Beatriz Amaya, Milagrosa Ramirez-del-Solar
Summary: Fe3+-TiO2 thin films were successfully prepared using a sandwich approach, and their structural, morphological, optical, and photocatalytic properties were studied. The incorporation of Fe3+ altered the material properties to enhance photocatalytic activity.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2022)
Article
Chemistry, Physical
Chu Wang, Yuanxu Liu, Yangyang Li, Xiao Sun, Leiming Xu, Weixin Huang
Summary: Developing facile photocatalysts with high activity and stability is a promising strategy for tetracycline degradation. The well-designed photocatalysts prepared via facile Ar atmosphere calcination with H-titanate nanotubes as precursors showed excellent visible light behavior by utilizing suitable oxygen vacancies (Ti3+ sites) as charge carrier traps. The efficient photocatalytic efficiency for TC degradation demonstrated significant activity of both h(+) and center dot O-2(-) under visible light irradiation.
JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY
(2023)
Article
Materials Science, Ceramics
Tingting Xiong, Yin Ye, Bin Luo, Liping Shen, Dongmei Wang, Meikun Fan, Zhengjun Gong
Summary: The 3D TA-TiO2-GA with network architectures and in situ growth of TiO2 NPs showed excellent photocatalytic performance and reusability in degrading organic contaminants. Mechanistic studies revealed the important roles of adsorption and photocatalysis, with superoxide radical anions and hydroxyl radicals as major reactive oxidative species. This study provides a novel alternative for solar light-driven environmental applications.
CERAMICS INTERNATIONAL
(2021)
Article
Environmental Sciences
Yuyang Li, Jian Sun, Yihua Chen, Hang Ma, Jiaxin Zhu, Zhiqiang Chen, Liao Meng, Tongzhou Liu
Summary: A simple technique for fabricating TiO2 thin film photocatalyst was developed in this work. The fabricated photocatalyst featured a homogeneous nanowire layer grown in situ on the Ti plate. The photocatalytic activity of the fabricated TiO2 thin film photocatalyst showed efficient degradation of RhB and CBZ under UVC irradiation, and the degradation kinetics were affected by the pH and the presence of Cl-, SO42-, or NO3-.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2023)
Article
Materials Science, Multidisciplinary
Yong Huang, Xiaofang Zhang, Fuzhong Zheng, Shiying Zou, Mingliang Li, Pan Huang, Ying Zeng
Summary: Well-dispersed beta-Bi2O3/Bi2O2CO3 hollow microspheres were synthesized by controlling the roasting conditions, which showed reliable photocatalytic activity and recycle stability for tetracycline degradation.
MATERIALS TODAY COMMUNICATIONS
(2022)
Article
Nanoscience & Nanotechnology
Yarabahally R. Girish, Udayabhanu, Gubran Alnaggar, Abdo Hezam, Mysore B. Nayan, Ganganagappa Nagaraju, Kullaiah Byrappa
Summary: TiO2 was successfully coupled with g-C3N4 to create an advanced heterojunction photocatalyst. The prepared nanocomposite showed significantly enhanced photocatalytic efficiency in hydrogen production and dye degradation. The interfacial contact between TiO2 and g-C3N4 effectively reduced electron hole recombination, resulting in improved photocatalytic activity.
JOURNAL OF SCIENCE-ADVANCED MATERIALS AND DEVICES
(2022)
Article
Chemistry, Physical
Jishu Rawal, Urooj Kamran, Mira Park, Bishweshwar Pant, Soo-Jin Park
Summary: Nitrogen and sulfur co-doped graphene quantum dots (GQDs) were synthesized using different 1-D carbon nanomaterials as precursors, showing superior photocatalytic performance when heterojunctioned with TiO2 and exhibiting efficient degradation of organic dyes.
Article
Engineering, Chemical
Guoli Xu, Meiling Du, Tao Li, Yueping Guan, Chen Guo
Summary: In this study, a novel Fe3O4/BiVO4/CdS (FBC) heterojunction photocatalyst was fabricated to enhance the absorption of visible light and facilitate charge separation and transfer, resulting in high activity and recyclability. The important parameters affecting photocatalytic activity were investigated to simulate pollutant degradation in real aqueous systems. Additionally, a Z-scheme transfer pathway was proposed to improve photocatalytic performance based on radical trapping experiments, electron spin resonance measurement, and optical and photoelectrochemical analysis.
SEPARATION AND PURIFICATION TECHNOLOGY
(2021)
Article
Materials Science, Multidisciplinary
Jinjuan Xue, Xinyao Li, Shuaishuai Ma, Peng Xu, Mingxin Wang, Zhaolian Ye
JOURNAL OF MATERIALS SCIENCE
(2019)
Article
Environmental Sciences
Yuqing Zong, Shuaishuai Ma, Jinjuan Xue, Jiandong Gu, Mingxin Wang
Summary: The NiAlFe LDH/PDA/PVDF membrane with superior wettability and hierarchical rough structure effectively separates oil-in-water emulsions and serves as a photocatalysis paper for antibiotic residue treatment with excellent photocatalytic activity and stability.
SCIENCE OF THE TOTAL ENVIRONMENT
(2021)
Article
Chemistry, Multidisciplinary
Shuaishuai Ma, Jiandong Gu, Yuqing Zong, Jinjuan Xue, Zhaolian Ye
Article
Chemistry, Multidisciplinary
Jiandong Gu, Hailang Jia, Shuaishuai Ma, Zhaolian Ye, Junli Pan, Ruoyu Dong, Yuqing Zong, Jinjuan Xue
Article
Chemistry, Multidisciplinary
Yuqing Zong, Shuaishuai Ma, Jiamin Gao, Minjing Xu, Jinjuan Xue, Mingxin Wang
Summary: This study successfully demonstrated the adsorption removal of antibiotics tetracycline and ciprofloxacin from water using porphyrinic zirconium metal-organic framework material PCN-224, with the 300 nm PCN-224 showing the best adsorption properties. The adsorption process follows the pseudo-second-order kinetic model and Langmuir isotherm model, and is exothermic in nature.
Article
Environmental Sciences
Jiamin Gao, Shuaishuai Ma, Minjing Xu, Meng Yuan, Jin Li, Jinjuan Xue, Mingxin Wang
Summary: The NiFe2O4/TA/PVDF composite membrane, with its superamphilicity and underwater superoleophobicity, shows great potential in the treatment of multicomponent wastewaters. It can efficiently degrade organic dyes and separate emulsified oils with high efficiency and flux. Additionally, it exhibits satisfactory processing efficiency, anti-fouling property, and reusability in dealing with mixed organic pollutants, making it a promising candidate for oil/water separation and organic wastewater treatment.
Article
Chemistry, Physical
Jiaqian Zhang, Jinjuan Xue, Zhenbo Wu, Mingxin Wang, Yiting Lv, Zhaoxia Chen, Shuaishuai Ma
Summary: In this study, a multifunctional membrane (TCPP/UiO@SSM) was fabricated for gravity-driven oil-water/seawater mixtures separation and visible-light-driven bacterial inactivation. The membrane demonstrated high permeation flux and separation efficiency, thanks to its rough hierarchical structure and super-wettability. It effectively dealt with viscous oil fouling and demonstrated superior oil-water separation and photocatalytic sterilization performances compared to UiO@SSM. The doping of photosensitive TCPP in UiO-66-NH2 improved hydrophilicity and enhanced photocatalytic activity. This work provides a new platform for water disinfection and treatment of oily wastewater.
APPLIED SURFACE SCIENCE
(2023)
Article
Biochemistry & Molecular Biology
Chengjuan Huang, Shuaishuai Ma, Yuqing Zong, Jiandong Gu, Jinjuan Xue, Mingxin Wang
PHOTOCHEMICAL & PHOTOBIOLOGICAL SCIENCES
(2020)