Article
Engineering, Environmental
Jiang Wu, Handan Lei, Jianjun Li, Zhanzhan Zhang, Guangyu Zhu, Guang Yang, Zhongkai Wang, Zan Hua
Summary: Sustainable functional materials derived from natural biomass have attracted significant attention, with renewable plant oil-based polymers showing excellent performance as pressure sensitive adhesives. Supramolecular interactions using complementary nucleobases contribute to the high performance of biomass-based polymeric materials.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Materials Science, Paper & Wood
Yuanyuan Zhang, Jianfeng Xi, Liucheng Meng, Yanling Lou, Shan Jiang, Huining Xiao, Weibing Wu
Summary: A green paper-based material with underwater superoleophobicity, high wet strength, and high flux was developed for efficient oil-water emulsion separation. Various steps were adopted to control pore size, enhance wet strength, and improve superoleophobicity. The material exhibited high separation efficiency, low-cost, environmentally-friendly, and recyclability, making it suitable for oily wastewater treatment.
Article
Chemistry, Physical
Jiaqi Chao, Jiekai Feng, Faze Chen, Bo Wang, Yanling Tian, Dawei Zhang
Summary: This article reports a method for fabricating superamphiphobic surfaces with tunable oil adhesion, achieved by adjusting parameters during the processing to control the adhesion of oil droplets on the surface. This work provides a simple approach to fabricate superamphiphobic surfaces and control oil adhesion in the atmosphere.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2021)
Article
Chemistry, Physical
Hui-Min Zeng, Bo-Xing Jin, Wei-Hong Wu, Chao Wang, Zhan-Guo Jiang, Zhigang Jin, Cai-Hong Zhan
Summary: The controllable construction of pure inorganic polyoxometalate (POM) zite materials with well-defined secondary building units (SBUs) is challenging. In this work, three distinct POM porous framework compounds 1-3 based on specific SBUs and transition-metal Ag linkers were self-assembled, providing valuable experience for synthetic chemists to obtain more interesting materials. Compound 1-3 exhibit cell type-specific, dose-dependent, and pH-sensitive anticancer behavior, making them promising anticancer agents for lung cancer therapy.
CHEMISTRY OF MATERIALS
(2022)
Article
Engineering, Mechanical
Lu Tie, Weimin Liu
Summary: Superwetting properties with multiple superlyphobic states have unique advantages in specific interfacial applications. However, there is currently a lack of systematic research on fine controlling superwetting surfaces. Controllable fabrication of superoleophobic surfaces from superhydrophilicity to superhydrophobicity in oil is still a challenge due to the harsh conditions involved.
TRIBOLOGY INTERNATIONAL
(2023)
Article
Engineering, Environmental
Xiaojuan Ming, Weibing Zhong, Yiming Ke, Jing Lu, Kangyu Jia, Xincheng Ding, Haiqing Jiang, Mufang Li, Dong Wang
Summary: This study successfully overcame the challenge of monitoring electrocardiograms in underwater environments by fabricating conductive gels with high adhesion strengths. These gels exhibited strong adhesion on various substrates and intrinsic conductivity, enabling them to collect continuous and reliable electrocardiogram signals. They have significant potential for applications in health monitoring and robotic arms.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Polymer Science
Xuehui Gong, Peipei Yang, Kristen Rohm, Yi Zhong, Boran Zhao, Ica Manas-Zloczower, Harihara Baskaran, Donald L. Feke
Summary: The technique of fabricating hollow fibers with porous walls using high internal phase emulsions (HIPEs) as templates offers an environmentally friendly alternative to conventional methods. This method allows for control over the hollow structures of polyHIPE fibers, producing porous fibers with a hollow core and potential applications in drug release studies and size-selective loading and separation of materials.
JOURNAL OF APPLIED POLYMER SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Jialing Li, Yunfei Zhang, Qiao Zhang, Changyong Cai, Fenfang Li, Shengyi Dong
Summary: In this study, polymeric supramolecular structures were fabricated using thioctic acid (TA) and phytic acid (PA). The resulting poly(TA-PA) materials exhibited rapid and strong adhesion on various surfaces, and displayed good stability and adhesion in the presence of water, making them suitable for underwater surface coatings and adhesion.
ADVANCED MATERIALS INTERFACES
(2023)
Article
Chemistry, Multidisciplinary
Quirin Prasser, Daniel Steinbach, Daniel Kodura, Vincent Schildknecht, Katja Koenig, Christian Weber, Erica Brendler, Carla Vogt, Urs Peuker, Christopher Barner-Kowollik, Florian Mertens, Felix H. Schacher, Anja S. Goldmann, Felix A. Plamper
Summary: The research introduced an electrochemical approach using polymers to control the interfacial tension between water and n-decane, and demonstrated micellar formation in the aqueous phase by varying the ratio of complexants through electrochemical control.
Article
Engineering, Chemical
Yanping Duan, Guangli Dong, Ruijie Wu, Xia Zhao, Mingwei Li, Fengfeng Zhang, Zhimin Song, Hong Hao
Summary: A new coating with superhydrophilicity and underwater superoleophobicity was synthesized for oil/water separation in subaqueous environments. The coating demonstrated high oil/water separation efficiency, stability, and weather resistance even after multiple cycles.
POLYMER ENGINEERING AND SCIENCE
(2022)
Review
Chemistry, Multidisciplinary
Nikunjkumar R. Visaveliya, Johann Michael Koehler
Summary: Hierarchical assembly architectures of functional polymer particles are promising due to their physicochemical and surface properties, and various assembly structures can be constructed by adjusting the surface, cross-linked network, and interfacial agents of polymer nanoparticles for controlled interfacial interactions. Microfluidic-mediated platform is used to synthesize polymer nanoparticles with different structural and interfacial properties, followed by assembly under batch or flow conditions.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Physical
Yining Wu, Lisha Tang, Mengjiao Cao, Li Li, Kai Liu, Demin Kong, Qingshan Zhao, Xu Jin, He Liu, Caili Dai
Summary: In this study, amino-modified carbon dots (am-CDs) were synthesized and used as a nanofluid for enhanced oil recovery. The am-CDs showed remarkable oil recovery efficiency, outperforming traditional methods. This study provides a new strategy for developing efficient carbon dots-based nanofluids for enhanced oil recovery.
Article
Polymer Science
Lidan Lan, Yun Huang, Zoufei Du, Yi Dan, Long Jiang
Summary: A beta-ketoenamine-linked porous organic polymer, TFP-TAPT, was fabricated via Schiff-base reaction and demonstrated efficient adsorption-desorption of gaseous toluene under humid conditions. The TFP-TAPT showed visible light-induced toluene adsorption, which can be easily desorbed by turning off the visible light due to its unique photoisomerization property. The work provides a simple, energy-saving, and environmentally friendly strategy for toluene adsorption-desorption and presents an ideal sorbent with both high adsorption capacity and convenient desorption capacity.
Article
Nanoscience & Nanotechnology
Yongsen Zhou, Chao Zhang, Shouwei Gao, Wanbo Li, Ji-jung Kai, Zuankai Wang
Summary: A chemically functionalized PSA (f-PSA) with enhanced and phototunable underwater adhesion has been developed by incorporating an underwater adhesion enhancer (mussel-inspired catechol) and a photo-responsive functionality (anthracene) into a standard acrylic PSA matrix. This synergistic coupling secures sufficient interfacial molecular interactions and leads to enhanced underwater adhesion, while the efficient dimerization of anthracene via light-triggered cycloaddition facilitates the viscoelastic property of f-PSA, rendering it phototunable. The f-PSA is envisioned to open up more opportunities for applications such as underwater manipulation, transfer printing, and medical adhesives.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Engineering, Chemical
Zhecun Wang, Jianlin Yang, Xiadong Dai, Jing Guo, Shenghai Li, Tauqir A. Sherazi, Suobo Zhang
Summary: The development of a novel integrated Janus porous membrane enables self-propelled energy free directional water transport in oil systems, holding significant implications for areas such as liquid separation.
JOURNAL OF MEMBRANE SCIENCE
(2021)
Article
Environmental Sciences
Yitong Zhou, Junxue Wu, Bin Wang, Lei Duan, Yizhe Zhang, Wenxing Zhao, Fang Wang, Qian Sui, Zhongying Chen, Dongjiong Xu, Qingxue Li, Gang Yu
ENVIRONMENTAL POLLUTION
(2020)
Article
Environmental Sciences
Yunzhu Huang, Qian Sui, Shuguang Lyu, Jiaqi Wang, Shaoxin Huang, Wentao Zhao, Bin Wang, Dongjiong Xu, Ming Kong, Yimin Zhang, Gang Yu
ENVIRONMENTAL POLLUTION
(2020)
Article
Engineering, Environmental
Han Qu, Holly Barrett, Bin Wang, Jiajun Han, Fang Wang, Wenwen Gong, Junxue Wu, Wei Wang, Gang Yu
Summary: The study revealed that the co-occurrence of ibuprofen and triclocarban residues in sediment have synergistic adverse effects on the environment and pose a synergistic threat to human health.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Environmental Sciences
Wenxing Zhao, Gang Yu, Lee Blaney, Bin Wang
Summary: This study established a facile approach for calculating emission factors of nine priority PPCPs in raw wastewater and wastewater effluent, estimating the mass of these pollutants discharged in the Yangtze River valley. The total mass of the nine PPCPs emitted into the watershed in 2018 was estimated under low, medium and high emission scenarios, providing a viable alternative to traditional estimation strategies in developing countries.
SCIENCE OF THE TOTAL ENVIRONMENT
(2021)
Article
Environmental Sciences
Lei Duan, Yizhe Zhang, Bin Wang, Yitong Zhou, Fang Wang, Qian Sui, Dongjiong Xu, Gang Yu
Summary: Pharmaceutically active compounds (PhACs) have been found in most megacities in China but rarely in small and medium-sized cities. This study investigated the occurrence and distribution of PhACs in a typical small and medium-sized city in China, revealing lower levels in surface water compared to larger cities. Agricultural sources were identified as a concern, with indicators showing more untreated wastewater input in certain areas.
SCIENCE OF THE TOTAL ENVIRONMENT
(2021)
Article
Engineering, Environmental
Wenkai An, Lei Duan, Yizhe Zhang, Bin Wang, Cristina Su Liu, Fang Wang, Qian Sui, Dongjiong Xu, Gang Yu
Summary: PFASs have been continuously monitored in the northwest of Tai Lake Basin for two years. The study investigated their occurrence, spatial distribution, seasonal variations, and sources. The results suggest that local industrial restructuring has contributed to the improvement of PFASs concentrations in the area.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Engineering, Environmental
Yinqiao Zhang, Juhong Zhan, Bin Wang, Jun Huang, Shubo Deng, Gang Yu, Sridhar Komarneni, Yujue Wang
Summary: This research evaluated the combination of UV irradiation and electrochemical processes for micropollutant abatement in water treatment, finding that the divided E-UV/Cl-2/H2O2 process was more effective and energy-efficient for removing micropollutants. The study highlights the potential synergistic effects of combining UV and electrochemical methods in different configurations for decentralized water treatment.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Environmental Sciences
Mohammadtaghi Vakili, Ruobing Qin, Giovanni Cagnetta, Jun Huang, Bin Wang, Gang Yu
Summary: Mechanochemical destruction of organic pollutants using high energy milling with inorganic reagents is a promising non-thermal technology for detoxifying hazardous waste. A fractal model was validated as a flexible tool to interpolate pollutant mechanochemical destruction data and estimate the contributions of the inorganic reagent and the pollutant to the overall reaction rate. The kinetic constants associated with mechanical activation of the co-milling reagent and pollutant destruction reaction were found to be dependent on the specific compound, allowing for prediction of pollutant degradation rates for various mixtures.
Article
Engineering, Environmental
Lingwei Gao, Yang Guo, Jun Huang, Bin Wang, Shubo Deng, Gang Yu, Yujue Wang
Summary: A probe-based kinetic model was developed to simulate micropollutant abatement during water treatment by a cobalt-mediated peroxymonosulfate process. The model can be used to predict the abatement efficiencies of various micropollutants by measuring the concentrations of sulfate and hydroxyl radicals.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Environmental Sciences
Junxue Wu, Bin Wang, Han Qu, Fang Wang, Lei Duan, Gang Yu
Summary: Acid-washed zero-valent aluminum was found to enhance the degradation efficiency of phenacetin in the persulfate treatment. The degradation of phenacetin mainly involved the break of C-N and C-O bonds and further oxidation.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2023)
Article
Engineering, Environmental
Han Qu, Hongting Diao, Jiajun Han, Bin Wang, Gang Yu
Summary: The production of plastic has significantly increased over the past decades, leading to the emergence of microplastics and nanoplastics, which pose potential risks to the environment and human health. Recent evidence suggests an increasing trend in microplastic concentration, with laboratory studies showing exposure levels much higher than those found in the environment. Microplastics have also been detected in feces, indicating possible excretion from animals and humans. Current studies have uncertainties, emphasizing the need for policies to reduce microplastic emissions and overcome technical obstacles in detection.
FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING
(2023)
Article
Chemistry, Physical
Qinglun You, Chunsheng Zhang, Min Cao, Bin Wang, Jun Huang, Yujue Wang, Shubo Deng, Gang Yu
Summary: In this study, a modified g-C3N4 (SCBCN0.4) was successfully synthesized using a triple strategy of defect controlling, element doping, and crystallinity improving. The research revealed that SCBCN0.4 has optimized microstructure and electronic structure, improved light-harvesting capability, and enhanced carrier separation efficiency. SCBCN0.4 demonstrated excellent performance in pollutant degradation and in-situ H2O2 generation, and showed detoxification, reusability, and stability.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Article
Engineering, Environmental
Chunzhao Chen, Gang Yu, Bin Wang, Fei Li, Huijuan Liu, Wen Zhang
Summary: This study explores the degradation behavior of disposable face masks in simulated seawater through accelerated aging experiments. The release rates of microplastics (MPs) and dissolved organic carbon (DOC) from the masks are influenced by temperature and time. The time-temperature superposition principle is used to estimate the degradation time and predict the release of MPs and DOC into the ocean in the future.
JOURNAL OF HAZARDOUS MATERIALS
(2023)
Article
Environmental Sciences
Chunzhao Chen, Chenxi Sun, Bin Wang, Zhiguo Zhang, Gang Yu
Summary: This study investigated the adsorption behavior of triclosan on differently sized and functionalized polystyrene nanoparticles (PSNPs) and evaluated the effects of environmental factors. The results showed that the physicochemical properties of PSNPs, such as particle size and surface functional groups, are important factors influencing their adsorption capacity.
SCIENCE OF THE TOTAL ENVIRONMENT
(2024)
Article
Green & Sustainable Science & Technology
Jian Chen, Bin Wang, Jun Huang, Shubo Deng, Yujue Wang, Lee Blaney, Georgina L. Brennan, Giovanni Cagnetta, Qimeng Jia, Gang Yu
Summary: In this study, a new framework is proposed to address the mixture regulation of emerging contaminants of concern (CECs). The framework includes experimental data, a machine learning model, and field site validation to reveal the relationship between CEC number and ecological risk. The study also introduces a new redundancy mechanism to clarify interactions among CECs.
