标题
New Approaches to the Synthesis of Metal Carbenes
作者
关键词
-
出版物
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 55, Issue 32, Pages 9134-9166
出版商
Wiley
发表日期
2016-06-16
DOI
10.1002/anie.201508119
参考文献
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- Gold(I) Carbenes by Retro-Buchner Reaction: Generation and Fate
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- 1,6-Carbene Transfer: Gold-Catalyzed Oxidative Diyne Cyclizations
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- Palladium-Catalyzed Oxidative Cross-Coupling of N-Tosylhydrazones with Indoles: Synthesis of N-Vinylindoles
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- Copper-Catalyzed C–O Bond Formation: An Efficient One-Pot Highly Regioselective Synthesis of Furans from (2-Furyl)Carbene Complexes
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- Direct Spectroscopic Characterization of a Transitory Dirhodium Donor-Acceptor Carbene Complex
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- Direct Evidence of a Dinuclear Copper Intermediate in Cu(I)-Catalyzed Azide-Alkyne Cycloadditions
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- General approach to benzo[b]thiophenes, benzo[b]furans, and dibenzofurans via gold-catalyzed cyclization of 1-heteroarylalka-2,3-dienyl acetates
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- Synthesis and esterification reactions of aryl diazomethanes derived from hydrazone oxidations catalyzed by TEMPO
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- Transition-Metal-Free Synthesis of Pinacol Alkylboronates from Tosylhydrazones
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- Gold-Catalyzed One-Step Construction of 2,3-Dihydro-1H-Pyrrolizines with an Electron-Withdrawing group in the 5-position: A Formal Synthesis of 7-Methoxymitosene
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- Highly Efficient Stereoselective Catalytic C(sp3)H Insertions with Donor Rhodium Carbenoids Generated from Cyclopropenes
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- A Facile Parallel Synthesis of Trifluoroethyl-Substituted Alkynes
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- A Chiral Cagelike Copper(I) Catalyst for the Highly Enantioselective Synthesis of 1,1-Cyclopropane Diesters
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- Sulfonyl-1,2,3-Triazoles: Convenient Synthones for Heterocyclic Compounds
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- Gold-Catalyzed Synthesis of Furans and Furanones from Sulfur Ylides
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- Olefination of Carbonyl Compounds through Reductive Coupling of Alkenylboronic Acids and Tosylhydrazones
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- Gold-Catalyzed Carbene Transfer to Alkynes: Access to 2,4-Disubstituted Furans
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- Rapid Access to Chroman-3-ones through Gold-Catalyzed Oxidation of Propargyl Aryl Ethers
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- Gold-Catalyzed Oxidative Cyclizations ofcis-3-En-1-ynes To Form Cyclopentenone Derivatives
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- Catalytic Generation of Zinc Carbenes from Alkynes: Zinc-Catalyzed Cyclopropanation and SiH Bond Insertion Reactions
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- Gold for the Generation and Control of Fluxional Barbaralyl Cations
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- Recent developments in copper-catalyzed reactions of diazo compounds
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- New highly soluble dimedone-derived iodonium ylides: preparation, X-ray structure, and reaction with carbodiimide leading to oxazole derivatives
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- Ring expansion of alkynyl cyclopropanes to highly substituted cyclobutenes via a N-sulfonyl-1,2,3-triazole intermediate
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- Enantioselective, transition metal catalyzed cycloisomerizations
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- Rhodium-catalyzed acyloxy migration of propargylic esters in cycloadditions, inspiration from the recent “gold rush”
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- Gold(I)-Catalysed Cycloisomerisation of 1,6-Cyclopropene-enes
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- Rh-Catalyzed [5+1] and [4+1] Cycloaddition Reactions of 1,4-Enyne Esters with CO: A Shortcut to Functionalized Resorcinols and Cyclopentenones
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- CRTH2 Antagonist MK-7246: A Synthetic Evolution from Discovery through Development
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- Arylation of Rhodium(II) Azavinyl Carbenes with Boronic Acids
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- Gold(I)-Catalyzed Asymmetric Cyclopropenation of Internal Alkynes
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- Rhodium(II)-Catalyzed Asymmetric Sulfur(VI) Reduction of Diazo Sulfonylamidines
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- Tempering the Reactivities of Postulated α-Oxo Gold Carbenes Using Bidentate Ligands: Implication of Tricoordinated Gold Intermediates and the Development of an Expedient Bimolecular Assembly of 2,4-Disubstituted Oxazoles
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- Synthesis of Enaminones by Rhodium-Catalyzed Denitrogenative Rearrangement of 1-(N-Sulfonyl-1,2,3-triazol-4-yl)alkanols
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- Rhodium-Catalyzed Intra- and Intermolecular [5 + 2] Cycloaddition of 3-Acyloxy-1,4-enyne and Alkyne with Concomitant 1,2-Acyloxy Migration
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- One-Point Binding Ligands for Asymmetric Gold Catalysis: Phosphoramidites with a TADDOL-Related but Acyclic Backbone
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- C(sp)–C(sp3) Bond Formation through Cu-Catalyzed Cross-Coupling of N-Tosylhydrazones and Trialkylsilylethynes
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- A novel copper-catalyzed reductive coupling of N-tosylhydrazones with H-phosphorus oxides
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- An efficient Au-catalyzed synthesis of isomukonidine, clausine L, mukonidine, glycosinine, mukonal, and clausine V from propadienyl methyl ether
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- Carbazoles via AuCl3-Catalyzed Cyclization of 1-(Indol-2-yl)-3-alkyn-1-ols
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- Iron-Catalyzed Cyclopropanation with Glycine Ethyl Ester Hydrochloride in Water
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- Regiodivergent Synthesis of Functionalized Indene Derivatives via Pt-Catalyzed Rautenstrauch Reaction of Propargyl Carbonates
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- Atom-Economical Synthesis of Functionalized Cycloalkanes via Catalytic Redox Cycloisomerization of Propargyl Alcohols
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- Olefin Cyclopropanation Catalyzed by Iridium(III) Porphyrin Complexes
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- Iron-Catalyzed Cyclopropanation in 6 M KOH with in Situ Generation of Diazomethane
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- Rh(II)-catalyzed [2,3]-sigmatropic rearrangement of sulfur ylides derived from N-tosylhydrazones and sulfides
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- Catalytic enantioselective carbon-carbon bond formation using cycloisomerization reactions
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- Intermolecular and Selective Synthesis of 2,4,5-Trisubstituted Oxazoles by a Gold-Catalyzed Formal [3+2] Cycloaddition
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- Interception of a Rautenstrauch Intermediate by Alkynes for [5+2] Cycloaddition: Rhodium-Catalyzed Cycloisomerization of 3-Acyloxy-4-ene-1,9-diynes to Bicyclo[5.3.0]decatrienes
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- Rhodium-Catalyzed Cycloisomerization Involving Cyclopropenes: Efficient Stereoselective Synthesis of Medium-Sized Heterocyclic Scaffolds
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- Palladium-Catalyzed Oxidative Cross-Coupling of N-Tosylhydrazones or Diazoesters with Terminal Alkynes: A Route to Conjugated Enynes
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- Isolation of Azomethine Ylides and Their Complexes: Iridium(III)-Mediated Cyclization of Nitrone Substrates Containing Alkynes
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- A Flexible and Stereoselective Synthesis of Azetidin-3-ones through Gold-Catalyzed Intermolecular Oxidation of Alkynes
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- Gold-Catalyzed Oxidative Cyclization of 1,5-Enynes Using External Oxidants
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- Transition-Metal-Catalyzed Denitrogenative Transannulation: Converting Triazoles into Other Heterocyclic Systems
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- Gold α-Oxo Carbenoids in Catalysis: Catalytic Oxygen-Atom Transfer to Alkynes
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- Tosylhydrazones: New Uses for Classic Reagents in Palladium-Catalyzed Cross-Coupling and Metal-Free Reactions
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- When cyclopropenes meet gold catalysts
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- A gold(i)-catalyzed intramolecular oxidation–cyclopropanation sequence of 1,6-enynes: a convenient access to [n.1.0]bicycloalkanes
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- Recent developments of cyclopropene chemistry
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- Guiding principles for site selective and stereoselective intermolecular C–H functionalization by donor/acceptor rhodium carbenes
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- N-Tosylhydrazones: versatile reagents for metal-catalyzed and metal-free cross-coupling reactions
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- General Au-Catalyzed Benzannulation Towards Naturally Occurring Carbazole Alkaloids from Methoxypropadiene
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- Enantioselective IrI-Catalyzed Carbocyclization of 1,6-Enynes by the Chiral Counterion Strategy
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- Gold-Catalyzed Synthesis of 3-Pyrrolidinones and Nitrones from N-Sulfonyl Hydroxylamines via Oxygen-Transfer Redox and 1,3-Sulfonyl Migration
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- Concise Synthesis of the Antidepressive Drug Candidate GSK1360707 by a Highly Enantioselective Gold-Catalyzed Enyne Cycloisomerization Reaction
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- Palladium-Catalyzed Amidation of N-Tosylhydrazones with Isocyanides
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- Auxiliary-Controlled Asymmetric [3+2]-Dipolar Cycloaddition of Azomethine Ylides Generated from Au-Catalyzed Intramolecular Redox Reaction of Nitronyl Alkynes
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- Synthesis of Sulfones by Iron-Catalyzed Decomposition of Sulfonylhydrazones
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- Gold(I)-Catalyzed Reactions of Propargyl Esters with Vinyl Derivatives
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- Recent Developments in Pd-Catalyzed Reactions of Diazo Compounds
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- Pd-Catalyzed Carbonylation of Diazo Compounds at Atmospheric Pressure: A Catalytic Approach to Ketenes
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- Catalytic Asymmetric C–H Insertions of Rhodium(II) Azavinyl Carbenes
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- Synthesis of α-Amino Ketones from Terminal Alkynes via Rhodium-Catalyzed Denitrogenative Hydration of N-Sulfonyl-1,2,3-triazoles
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- Propargyl Alcohols as β-Oxocarbenoid Precursors for the Ruthenium-Catalyzed Cyclopropanation of Unactivated Olefins by Redox Isomerization
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- An Efficient [2 + 2 + 1] Synthesis of 2,5-Disubstituted Oxazoles via Gold-Catalyzed Intermolecular Alkyne Oxidation
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- Triazole Bridges as Versatile Linkers in Electron Donor–Acceptor Conjugates
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- Gold-Catalyzed 1,2-Difunctionalizations of Aminoalkynes Using Only N- and O-Containing Oxidants
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- Copper-Catalyzed Direct Benzylation or Allylation of 1,3-Azoles withN-Tosylhydrazones
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- Cyclopropanation with Gold(I) Carbenes by Retro-Buchner Reaction from Cycloheptatrienes
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- Copper-catalyzed reductive coupling of tosylhydrazones with amines: A convenient route to α-branched amines
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- Efficient synthesis of carbazoles via PtCl2-catalyzed RT cyclization of 1-(indol-2-yl)-2,3-allenols: scope and mechanism
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- Rh-Catalyzed Transannulation ofN-Tosyl-1,2,3-Triazoles with Terminal Alkynes
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- Synthesis and Reactivity of Sulfamoyl Azides and 1-Sulfamoyl-1,2,3-triazoles
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- Iron-Catalyzed Preparation of Trifluoromethyl Substituted Vinyl- and Alkynylcyclopropanes
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- Chiral Diene-Phosphine Tridentate Ligands for Rhodium-Catalyzed Asymmetric Cycloisomerization of 1,6-Enynes
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- Gold-Catalyzed Nitrene Transfer to Activated Alkynes: Formation of α,β-Unsaturated Amidines
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- Reactivity ofN-(1,2,4-Triazolyl)-Substituted 1,2,3-Triazoles
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- A Concise Synthesis of a β-Lactamase Inhibitor
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- Stereoselective One-Pot Synthesis of 1-Aminoindanes and 5,6-Fused Azacycles Using a Gold-Catalyzed Redox-Pinacol-Mannich-Michael Cascade
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- Enantioselective Cobalt-Catalyzed Preparation of Trifluoromethyl-Substituted Cyclopropanes
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- Rhodium-Catalyzed Cyclopropenation of Alkynes: Synthesis of Trifluoromethyl-Substituted Cyclopropenes
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- Enantioselective Gold Catalysis: Opportunities Provided by Monodentate Phosphoramidite Ligands with an Acyclic TADDOL Backbone
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- Chiral Tetrafluorobenzobarrelene Ligands for the Rhodium-Catalyzed Asymmetric Cycloisomerization of Oxygen- and Nitrogen-Bridged 1,6-Enynes
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- Straightforward Synthesis of Ethers: Metal-Free Reductive Coupling of Tosylhydrazones with Alcohols or Phenols
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- Gold-Catalyzed Cyclopenta- and Cycloheptannulation Cascades: A Stereocontrolled Approach to the Scaffold of Frondosins A and B
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- Coupling of N-Tosylhydrazones with Terminal Alkynes Catalyzed by Copper(I): Synthesis of Trisubstituted Allenes
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- Gold-Catalyzed Oxidative Ring Expansions and Ring Cleavages of Alkynylcyclopropanes by Intermolecular Reactions Oxidized by Diphenylsulfoxide
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- Synthesis of functionalized resorcinols by rhodium-catalyzed [5+1] cycloaddition reaction of 3-acyloxy-1,4-enynes with CO
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- Pd-catalyzed oxidative cross-coupling of N-tosylhydrazones with arylboronic acids
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- Gold(i)-catalysed synthesis of conjugated trienes
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- Copper-catalyzed azide–alkyne cycloaddition (CuAAC) and beyond: new reactivity of copper(i) acetylides
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- Synthesis of 2-acylfurans from 3-(1-alkynyl)-2-alken-1-ones via the oxidation of gold–carbene intermediates by H2O2
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- Synthesis of 2-Azabicyclo[4.1.0]heptanes through Stereoselective Cyclopropanation Reactions
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- An Efficient Synthesis of Polysubstituted Naphthalene Derivatives by Gold-Catalyzed Cyclization of 1-Arylalka-2,3-dienyl Acetates
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- On the Mechanism of Ylide-Mediated Cyclopropanations: Evidence for a Proton-Transfer Step and Its Effect on Stereoselectivity
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- Synthesis and Reactivity of Rhodium(II)N-Triflyl Azavinyl Carbenes
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- Cationic Rhodium(I) Complex-Catalyzed [3 + 2] and [2 + 1] Cycloadditions of Propargyl Esters with Electron-Deficient Alkynes and Alkenes
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- Pt-Catalyzed Tandem 1,2-Acyloxy Migration/Intramolecular [3 + 2] Cycloaddition of Enynyl Esters
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- Computation-Guided Development of Au-Catalyzed Cycloisomerizations Proceeding via 1,2-Si or 1,2-H Migrations: Regiodivergent Synthesis of Silylfurans
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- Alkynes as Equivalents of α-Diazo Ketones in Generating α-Oxo Metal Carbenes: A Gold-Catalyzed Expedient Synthesis of Dihydrofuran-3-ones
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- Pd-Catalyzed Three-Component Coupling ofN-Tosylhydrazone, Terminal Alkyne, and Aryl Halide
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- Gold(I)-Catalyzed Intermolecular [2+2] Cycloaddition of Alkynes with Alkenes
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- Gold-Catalyzed Highly Regioselective Oxidation of C−C Triple Bonds without Acid Additives: Propargyl Moieties as Masked α,β-Unsaturated Carbonyls
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- Gold-Catalyzed One-Step Practical Synthesis of Oxetan-3-ones from Readily Available Propargylic Alcohols
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- Gold-Catalyzed Annulation/Fragmentation: Formation of Free Gold Carbenes by Retro-Cyclopropanation
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- Platinum(II)-Catalyzed Generation and [3+2] Cycloaddition Reaction of α,β-Unsaturated Carbene Complex Intermediates for the Preparation of Polycyclic Compounds
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- Gold(i)-catalysed alcohol additions to cyclopropenes
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- Regioselective syntheses of fully-substituted 1,2,3-triazoles: the CuAAC/C–H bond functionalization nexus
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- Copper-Catalyzed Nitrogen Loss of Sulfonylhydrazones: A Reductive Strategy for the Synthesis of Sulfones from Carbonyl Compounds
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- Synthesis of 3-Oxa- and 3-Azabicyclo[4.1.0]heptanes by Gold-Catalyzed Cycloisomerization of Cyclopropenes
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- Experimental and Theoretical Investigation into the Gold-Catalyzed Reactivity of Cyclopropenylmethyl Acetates
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- Rhodium(I)-catalyzed [3+2+2]-cyclization of alkenyl Fischer carbene complexes with methyl buta-2,3-dienoate
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- Metal-free intramolecular cyclopropanation of alkenes through iodonium ylide methodology
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- Gold-catalyzed intermolecular [4C+3C] cycloaddition reactions
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