Journal
CHEMSUSCHEM
Volume 4, Issue 2, Pages 173-179Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201000385
Keywords
catalysis; oxidations; photochemistry; photosynthesis; water splitting
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The state-of-the-art of research on artificial photosynthesis is briefly reviewed. Insights into how Nature takes electrons from water, the photon-flux density of sunlight, the time scale for the arrival of the next photon (electron-hole) at the oxygen-evolving complex, how Nature solves the photon-flux-density problem, and how we can get through the bottleneck of water oxidation are discussed. An alternate route for a two-electron process induced by one-photon excitation is postulated for getting through the bottleneck of water oxidation.
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