Article
Materials Science, Multidisciplinary
Dan Tu, Wenyao Yang, Yi Li, Yujiu Zhou, Liuwei Shi, Jianhua Xu, Yajie Yang
Summary: The research successfully synthesized MXene/BCN composite materials and applied them to flexible microsupercapacitors, showing high areal capacitance and remarkable mechanical flexibility.
JOURNAL OF MATERIALS CHEMISTRY C
(2021)
Article
Chemistry, Physical
Shuqi Hu, Yuying Liu, Shuangbao Wang, Xinyi Zhang, Pei Kang Shen
Summary: The study demonstrates that ultrathin Co(OH)(2) nanoparticles can be converted into Co3O4-Pt core-shell nanoparticles with high Pt utilization through thermal annealing and controlled replacement reaction on 3D graphene. This nanostructure shows optimized mass activity and specific activity, significantly outperforming traditional Pt/C catalysts.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2021)
Article
Chemistry, Analytical
Hongyin Pan, Chen Yang, Wei Zheng, Xianghong Liu, Yong Wan, Jun Zhang
Summary: A gas sensor based on porous Co3O4 thin films decorated by dual Pt/Rh catalysts is demonstrated for efficient NO2 detection in humid environment. The sensor exhibits high response and moisture resistance due to the three-dimensional ordered microstructure of the Co3O4 thin films and the loading of Pt/Rh catalysts by atom layer deposition (ALD). With optimized ALD Pt and Rh thickness, the sensor shows fast response/recovery speed, a low detection limit and the capability to operate under high humidity.
SENSORS AND ACTUATORS B-CHEMICAL
(2023)
Article
Chemistry, Multidisciplinary
Yongjiu Lei, Wenli Zhao, Yunpei Zhu, Ulrich Buttner, Xiaochen Dong, Husam N. Alshareef
Summary: This study demonstrates the construction of a hybrid microsupercapacitor using suitable materials and microfabrication methods, resulting in high areal energy density and excellent electrochemical performance.
Article
Engineering, Environmental
Yiyang Ma, Hongjie Wang, Xiaofan Lv, Dongbin Xiong, Haijiao Xie, Zhenghua Zhang
Summary: This study synthesized three-dimensional ordered mesoporous Co3O4 (3D OM-Co3O4) to enhance the activation ability of PMS and achieve rapid removal of RAN. 3D OM-Co3O4 can activate PMS through non-radical and radical pathways simultaneously, and it has good catalytic stability.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Analytical
James S. Ng, Michinao Hashimoto
Summary: This paper introduces a method of utilizing FDM printing to fabricate paper-based analytical devices with three-dimensional features, using two types of thermoplastics to overcome limitations related to organic solvents in traditional PADs. The study validated the capability and potential applications of 3D-PADs in holding increased amounts of liquid samples and demonstrated colorimetric assays for organic solvent-based reactions.
Article
Chemistry, Physical
Lang He, Wenyuan Zhang, Sheng Liu, Yan Zhao
Summary: Three-dimensional palm frondlike S-scheme heterojunction based Co3O4@NiO/graphitic carbon composites were fabricated as photocatalysts for CO2 reduction reactions. The optimal Co@Ni/GC-700 catalyst exhibited excellent performance and stability with maximum yields of 9.79 µmol g-1h-1 for CH4 and 4.89 µmol g-1h-1 for CO under visible light irradiation. The superior photocatalytic CO2RR activity of the Co@Ni/GC catalysts can be attributed to the direct S-scheme heterojunction induced by the interfacial electric field (EF) and the improved CO2 adsorption capacity.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
Review
Optics
V. Harinarayana, Y. C. Shin
Summary: With the introduction of femtosecond lasers in the early 1990s, ultrafast laser processing has become crucial for micro/nano machining, with Two-photon lithography (TPL) being a unique technique that has revolutionized laser material processing. This paper provides an overview of TPL, including its working principle, experimental setup, and materials, as well as techniques to improve resolution and pave the way for industrialization. The paper also thoroughly reviews TPL for microfabrication, with an emphasis on metamaterials.
OPTICS AND LASER TECHNOLOGY
(2021)
Article
Biochemistry & Molecular Biology
Yingxian Lu, Yigong Shi
Summary: This study proposes a micro-fabricated low-frequency EM stimulation lab-on-chip for observing cell lines using a microscope. The research examines the effects of EM signals on biological structures and finds that a 10 kHz EM signal significantly affects cell growth.
BIOELECTROCHEMISTRY
(2023)
Article
Chemistry, Analytical
Kangning Wang, Limin He, Andreas Manz, Wenming Wu
Summary: Traditional methods for manufacturing microfluidic chips face challenges in producing complex topologies and three-dimensional microchannels, relying on expensive equipment and complex processes. The proposed low-cost approach of sewing chip pipes to substrates with an embroidery machine offers a more efficient alternative, eliminating the need for specialized equipment and skills.
ANALYTICAL CHEMISTRY
(2021)
Article
Engineering, Environmental
Sonia Zoltowska, Juan F. Minambres, Adam Piasecki, Florian Mertens, Teofil Jesionowski
Summary: This study utilized spongin-based scaffolds of commercial sponge origin for the preparation of novel catalysts through simple functionalization with cobalt, showing good activity and reusability in oxidation-reduction reactions. The materials prepared demonstrated a fibrous structure with open porous canals, allowing for good accessibility of substrates to the catalyst surfaces. The adaptability of spongin-based scaffolds in preparing biocarbons with high potential for various catalytic applications was proven.
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
(2021)
Article
Chemistry, Inorganic & Nuclear
Huazhong Liu, Mahmoud Motlak, Zhi Feng, Afsaneh Kaffash
Summary: In this study, a novel electrochemical sensor based on a hierarchical Co3O4/carbon composite was developed for determination of morphine (MOR). The sensor showed high electrochemical catalytic activity and excellent response for MOR detection. It also demonstrated good selectivity, stability, and reproducibility, making it a suitable platform for MOR detection in body fluids. The simplicity, low cost, and short analysis time of this approach suggest its potential application in clinical and forensic testing for MOR.
INORGANIC CHEMISTRY COMMUNICATIONS
(2023)
Article
Nanoscience & Nanotechnology
Yuki Maegawa, Yosuke Nakata, Atsushi Sanada
Summary: In this article, all-dielectric carpet cloaks composed of jungle gym shaped dielectric unit cells are proposed. A design strategy for three-dimensional anisotropy control based on transformation optics is presented. The carpet cloaks are 3D printable and operate with polarization independent incident waves in arbitrary incident angles.
Article
Chemistry, Physical
Dan Tang, Yanfang Ma, Yang Liu, Keke Wang, Zeng Liu, Wenzhang Li, Jie Li
Summary: Co3O4 as a potential catalyst for OER, synthesized as a nanowire network on nickel foam, was transformed through a lithium-ion rocking chair mechanism to improve OER performance.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Materials Science, Multidisciplinary
Nan Bu, Jun Xiang, Sroeurb Loy, Wen-Duo Yang, Yi-Fei Di, Rong-Da Zhao, Fu-Fa Wu, Dong-Mei Ma, Mei-Ting Li, Jia Li
Summary: The Co3O4@NiMoO4 composite electrode material with Co3O4 nanowire as the precursor has been prepared successfully by hydrothermal method and thermal annealing treatment. The material exhibits outstanding electrochemical performance and cycling stability, making it a promising electrode material in high-performance supercapacitor applications.
MATERIALS CHEMISTRY AND PHYSICS
(2022)
Article
Materials Science, Multidisciplinary
Xinghang Chen, Ming Li, Qi Li, Yuzhu Chen, Buke Wu, Meng Lin, Qinyou An, Liqiang Mai
Summary: This study applied a simple and effective approach of controlled-current zinc pre-deposition at copper mesh, resulting in a highly reversible and dendrite-free zinc anode for high-performance zinc ion batteries. The pre-deposited zinc layer with (002) crystal plane orientation and compactly aligned platelet morphology exhibited significantly enhanced cycling stability compared to zinc foil. Moreover, a significant improvement in capacity-retention was also achieved in a Zn||MnO2 full battery.
ENERGY & ENVIRONMENTAL MATERIALS
(2023)
Article
Materials Science, Multidisciplinary
Wenzhong Huang, Shanlin Liu, Ruohan Yu, Liang Zhou, Zhenhui Liu, Liqiang Mai
Summary: This study proposes an ordered mesoporous N-doped carbon with lithiophilic single atoms to induce uniform nucleation and deposition of Li metal, addressing the challenges of lithium dendrites and huge volume change. The ordered mesoporous structure and lithiophilic single-atom sites enable regulated local current density and rapid mass transfer, resulting in uniform Li deposition with inhibition of dendrites and buffered volume expansion. The fabricated anode exhibits a high CE of 99.8% for 200 cycles and a stable voltage hysteresis of 14 mV at 5 mA cm(-2) for over 1330 hours in the symmetric cell. The full cell coupled with commercial LiFePO4 shows a high reversible capacity of 108 mAh g(-1) and average Coulombic efficiency of 99.8% from the 5th to 350th cycles at 1 C. The ordered mesoporous carbon host with lithiophilic single-atom sites provides new inspirations for the rational design of high-performance Li metal anodes.
ENERGY & ENVIRONMENTAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Ruohan Yu, Yexin Pan, Yihang Liu, Liang Zhou, Dongyuan Zhao, Jinsong Wu, Liqiang Mai
Summary: A sub 10 nm scale interfused TiO2/SiOx hybrid with a bicontinuous structure was constructed through the oxidation of MAX Ti3SiC2 ceramic. This hybrid material exhibited a mutual stabilizing effect during lithiation, resulting in a high and stable specific capacity with low volume expansion. The concept of mutual-stabilizing effect can be applied to the design of LIB anode materials with high capacity and longevity.
Article
Chemistry, Multidisciplinary
Yu Liu, Yongkang An, Lu Wu, Jianguo Sun, Fangyu Xiong, Han Tang, Shulin Chen, Yue Guo, Lei Zhang, Qinyou An, Liqiang Mai
Summary: In this study, glycine is used as an additive to modulate the solvation shell structure and enhance the interfacial stability of aqueous Zn ion batteries. The results show that the cycle life of the symmetrical cells reaches over 3200 h in glycine-containing electrolytes, and the Zn//NVO full cell exhibits exceptional cycling stability for 3000 cycles at 5 A g-1. Therefore, the proposed strategy for interfacial chemistry modulation, represented by glycine, has considerable potential in promoting the commercialization progress of aqueous batteries.
Article
Chemistry, Multidisciplinary
Nannan Zhang, Lulu Du, Jianyong Zhang, Hantao Xu, Xuan Zhou, Liqiang Mai, Lin Xu
Summary: A flexible tent-like interface constructed by self-assembly of graphene oxide on zinc nanosheets is proposed to achieve stable lithium metal anode. This interface immobilizes the graphene oxide layer and enables homogeneous lithium deposition within nanocavities. The confinement of Li plating/stripping inside the nanocavities effectively reduces electrolyte-Li reaction and eliminates continuous consumption of Li metal, leading to excellent cycling performance and high-capacity retention.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Review
Chemistry, Multidisciplinary
Peng Hu, Ping Hu, Tuan Duc Vu, Ming Li, Shancheng Wang, Yujie Ke, Xianting Zeng, Liqiang Mai, Yi Long
Summary: Vanadium oxides with multioxidation states and various crystalline structures have unique electrical, optical, optoelectronic and magnetic properties, which can be utilized for various applications. In the past 30 years, significant efforts have been made to study the fundamental science and explore the potential of vanadium oxide materials in fields such as ion batteries, water splitting, smart windows, supercapacitors, and sensors. This review focuses on the synthesis methods and applications of thermodynamically stable and metastable vanadium oxides, providing a comprehensive overview to accelerate their development in related applications.
Article
Chemistry, Physical
Wei Yang, Lin Xu, Wen Luo, Ming Li, Ping Hu, Yuhang Dai, Fazhi Ye, Chunhua Han, Minxuan Zhou, Rong Tu, Ji Shi, Liqiang Mai
Summary: In this study, a facile manufacturing process is used to fabricate Zn-MnO2 microbatteries with a 3D macroporous microelectrode, which exhibit easy integration, mass customization, and superior electrochemical performance. The microbatteries achieve ultrahigh capacity and outstanding areal energy density due to the high electron/ion transport path and high mass-loading of the PEDOT-MnO2 film. Additionally, a 3D macroporous PEDOT-MnO2 hybrid film is achieved, which improves the cycling performance without reducing areal capacity or hindering ion diffusion. Therefore, the PEDOT-MnO2//Zn microbatteries hold great potential as a next-generation component for self-powered microelectronic devices.
ADVANCED ENERGY MATERIALS
(2023)
Article
Chemistry, Physical
Ruhan He, Yutao Wang, Chengyi Zhang, Zhenhui Liu, Pan He, Xufeng Hong, Ruohan Yu, Yan Zhao, Jingsong Wu, Liang Zhou, Liqiang Mai
Summary: An ultrathin layer of stable and electroactive yolk-shell SiOx/C@C is constructed on Cu foil with designed differences in lithiophilicity, demonstrating effective Li dendrite suppression and high specific capacity. The Cu-based Li-SiOx/C@C anode exhibits good cyclability in symmetric cells under strict conditions. When paired with a LiFePO4 cathode, the full cell shows a high capacity retention of 91.3% over 350 cycles, highlighting its practical application value in future lithium metal batteries.
ADVANCED ENERGY MATERIALS
(2023)
Article
Chemistry, Physical
Hantao Xu, Jianyong Zhang, Hong Zhang, Juncai Long, Lin Xu, Liqiang Mai
Summary: By rational topological design, a topological polymer-reinforced interphase layer is in situ constructed using a synthesized solid polymer electrolyte, which addresses the incompatible interphases resulting from the contradiction between impedance and mechanical strength. The constructed topological solid electrolyte interphase (SEI) layer harmonizes mechanochemical stability and fast diffusion dynamics of Li+, ensuring the integrity and stability of the SEI layer. Additionally, the formation of the topological interphase layer enables highly stable and reversible Li nucleation/stripping behaviors exceeding 3000 h and superior cycling performance of practical LiFePO4/Li metal battery beyond 500 cycles.
ADVANCED ENERGY MATERIALS
(2023)
Article
Chemistry, Physical
Jiahui Deng, Xuri Zuo, Hong Zhang, Fan Fei, Xuan Zhou, Liqiang Mai, Lin Xu
Summary: In this work, an ultrathin solid-state electrolyte (SSE) named LA-SSE was developed by combining a lipoic acid-assisted semi-interpenetrating polymer network and an ultrathin porous membrane. LA-SSE, with a thickness of only 10 μm, showed excellent mechanical properties to suppress lithium dendrite growth and favorable interfacial compatibility between the lithium anode and electrolyte. By using LA-SSE as the electrolyte, long-term cycling of over 3000 hours was achieved in a Li parallel to LA-SSE parallel to Li symmetric cell, and a LiFePO4 parallel to LA-SSE parallel to Li full battery exhibited stable operation over 200 cycles with a capacity retention of 84% at room temperature. This study provides a promising strategy for designing ultrathin SSEs with satisfactory mechanical properties, excellent interfacial compatibility, and safety for lithium-ion batteries.
ACS APPLIED ENERGY MATERIALS
(2023)
Article
Nanoscience & Nanotechnology
Fan Fei, Hong Zhang, Jiahui Deng, Hantao Xu, Jun Xie, Hemdan S. H. Mohamed, Ahmed Eissa Abdelmaoula, Liqiang Mai, Lin Xu
Summary: A confinement strategy based on hydrogen bonding was proposed to achieve low-energy-barrier lithium ion transport in composite solid-state electrolytes for all-solid-state lithium metal batteries. The use of ultrafine boehmite nanowires in a polymer matrix resulted in the formation of template channels for continuous transport of dissociated lithium ions. The electrolytes exhibited high ionic conductivity, low energy barrier, and excellent specific capacity retention after cycling.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Chemistry, Multidisciplinary
Yu Cheng, Xiaowei Liu, Yaqing Guo, Guangyao Dong, Xinkuan Hu, Hong Zhang, Xidan Xiao, Qin Liu, Lin Xu, Liqiang Mai
Summary: This study proposes a new strategy to enhance Li+ transport by eliminating Li+ non-conductive areas and optimizing Li+ pathways through the construction of fully active Li+ conductive networks. The 3D networks formed by the monodispersed cluster chains provide homogeneous, large-scale, continuous Li+ fast transport channels, resulting in high ionic conductivity and Li+ transference number. In addition, the assembled LiFePO4/Li cell exhibits excellent cycling stability.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Wen Luo, Xin Yan, Xuelei Pan, Jinying Jiao, Liqiang Mai
Summary: This article introduces a unique on-chip micro/nano device that combines nanofabrication and low-dimensional electrochemical materials, achieving functions such as material structure analysis, field-effect regulation, in-situ monitoring, and simulation modeling. It discusses the key mechanisms that influence electrochemical response and emphasizes the advantages and challenges of the on-chip micro/nano device.
Article
Chemistry, Physical
Wencong Feng, Chuanqi Pan, Hong Wang, Biluan Zhang, Wen Luo, Chunli Shen, Junjun Wang, Chaojie Cheng, Xianmin Xv, Ruohan Yu, Yanbing Guo, Liqiang Mai
Summary: In this study, an approach for designing anode materials based on two-dimensional ion transport channels is proposed, which achieves self-regulating ion channels through self-reversible conversion. The results show that the material based on graphdiyne exhibits a large diffusion coefficient and high reversible capacity, demonstrating excellent durability.
ENERGY STORAGE MATERIALS
(2023)
Article
Chemistry, Physical
Wei Chen, Jiahao Wu, Kai Fu, Zhaohui Deng, Xingbao Chen, Hongwei Cai, Xinfei Wu, Boyu Xing, Wen Luo, Liqiang Mai
Summary: Researchers have designed and constructed a solvation structure of propylene carbonate (PC)-trifluoromethanesulfonate (Otf)-H2O to overcome the challenges in aqueous Zn battery. The addition of PC inhibits phase transition, broadens electrochemical stability window, and inhibits dendrite growth. The MnHCF/Zn hybrid co-solvent battery exhibits high cycling performance and a capacity retention of 65.6% after 1000 cycles.
Article
Chemistry, Multidisciplinary
Laetitia Bardet, Herve Roussel, Stefano Saroglia, Masoud Akbari, David Munoz-Rojas, Carmen Jimenez, Aurore Denneulin, Daniel Bellet
Summary: The thermal instability of silver nanowires leads to increased electrical resistance in AgNW networks. Understanding the relationship between structural and electrical properties of AgNW networks is crucial for their integration as transparent electrodes in flexible optoelectronics. In situ X-ray diffraction measurements were used to study the crystallographic evolution of Ag-specific Bragg peaks during thermal ramping, revealing differences in thermal and structural transitions between bare and SnO2-coated AgNW networks.
Article
Chemistry, Multidisciplinary
Nathalia Cancino-Fuentes, Arnau Manasanch, Joana Covelo, Alex Suarez-Perez, Enrique Fernandez, Stratis Matsoukis, Christoph Guger, Xavi Illa, Anton Guimera-Brunet, Maria V. Sanchez-Vives
Summary: This study provides a comprehensive characterization of graphene-based solution-gated field-effect transistors (gSGFETs) for brain recordings, highlighting their potential clinical applications.
Article
Chemistry, Multidisciplinary
Sikandar Aftab, Hailiang Liu, Dhanasekaran Vikraman, Sajjad Hussain, Jungwon Kang, Abdullah A. Al-Kahtani
Summary: This study examines the effects of hybrid nanoparticles made of NiO@rGO and NiO@CNT on the active layers of polymer solar cells and X-ray photodetectors. The findings show that these hybrid nanoparticles can enhance the charge carrier capacities and exciton dissociation properties of the active layers. Among the tested configurations, the NiO@CNT device demonstrates superior performance in converting sunlight into electricity, and achieves the best sensitivity for X-ray detection.
Article
Chemistry, Multidisciplinary
Hyo Jung Shin, Seung Gyu Choi, Fengrui Qu, Min-Hee Yi, Choong-Hyun Lee, Sang Ryong Kim, Hyeong-Geug Kim, Jaewon Beom, Yoonyoung Yi, Do Kyung Kim, Eun-Hye Joe, Hee-Jung Song, Yonghyun Kim, Dong Woon Kim
Summary: This study investigates the role of SOX9 in reactive astrocytes following ischemic brain damage using a PLGA nanoparticle plasmid delivery system. The results demonstrate that PLGA nanoparticles can reduce ischemia-induced neurological deficits and infarct volume, providing a potential opportunity for stroke treatment.
Article
Chemistry, Multidisciplinary
Anurag Chaudhury, Koushik Debnath, Nikhil R. Jana, Jaydeep K. Basu
Summary: The study investigates the interaction between nanoparticles and cell membranes, and identifies key parameters, including charge, crowding, and membrane fluidity, that determine the adsorbed concentration and unbinding transition of nanoparticles.
Article
Chemistry, Multidisciplinary
Sina Sadeghi, Fazel Bateni, Taekhoon Kim, Dae Yong Son, Jeffrey A. Bennett, Negin Orouji, Venkat S. Punati, Christine Stark, Teagan D. Cerra, Rami Awad, Fernando Delgado-Licona, Jinge Xu, Nikolai Mukhin, Hannah Dickerson, Kristofer G. Reyes, Milad Abolhasani
Summary: In this study, an autonomous approach for the development of lead-free metal halide perovskite nanocrystals is presented, which integrates a modular microfluidic platform with machine learning-assisted synthesis modeling. This approach enables rapid and optimized synthesis of copper-based lead-free nanocrystals.
Article
Chemistry, Multidisciplinary
Zahir Abbas, Nissar Hussain, Surender Kumar, Shaikh M. Mobin
Summary: The rational construction of free-standing and flexible electrodes for electrochemical energy storage devices is an emerging research focus. In this study, a redox-active metal-organic framework (MOF) was prepared on carbon nanofibers using an in situ approach, resulting in a flexible electrode with high redox-active behavior and unique properties such as high flexibility and lightweight. The prepared electrode showed excellent cyclic retention and rate capability in supercapacitor applications. Additionally, it could be used as a freestanding electrode in flexible devices at different bending angles.
Article
Chemistry, Multidisciplinary
Lishan Zhang, Xiaoting Zhang, Hui Ran, Ze Chen, Yicheng Ye, Jiamiao Jiang, Ziwei Hu, Miral Azechi, Fei Peng, Hao Tian, Zhili Xu, Yingfeng Tu
Summary: Photodynamic therapy (PDT) is a promising local treatment modality in cancer therapy, but its therapeutic efficacy is restricted by ineffective delivery of photosensitizers and tumor hypoxia. In this study, a phototactic Chlorella-based near-infrared (NIR) driven green affording-oxygen microrobot system was developed for enhanced PDT. The system exhibited desirable phototaxis and continuous oxygen generation, leading to the inhibition of tumor growth in mice. This study demonstrates the potential of using a light-driven green affording-oxygen microrobot to enhance photodynamic therapy.
Article
Chemistry, Multidisciplinary
Yujin Li, Jing Xu, Xinqi Luo, Futing Wang, Zhong Dong, Ke-Jing Huang, Chengjie Hu, Mengyi Hou, Ren Cai
Summary: In this study, hollow heterostructured materials were constructed using an innovative template-engaged method as cathodes for zinc-ion batteries. The materials exhibited fast Zn2+ transport channels, improved electrical conductivity, and controlled volume expansion during cycling. The designed structure allowed for an admirable reversible capacity and high coulombic efficiency.
Article
Chemistry, Multidisciplinary
Paritosh Mahato, Shashi Shekhar, Rahul Yadav, Saptarshi Mukherjee
Summary: This study comprehensively elucidates the role of the core and electrostatic surface of metal nanoclusters in catalytic reduction reactions. The electrostatic surface dramatically modulates the reactivity of metal nanoclusters.
Article
Chemistry, Multidisciplinary
Pei Liu, Mengdi Liang, Zhengwei Liu, Haiyu Long, Han Cheng, Jiahe Su, Zhongbiao Tan, Xuewen He, Min Sun, Xiangqian Li, Shuai He
Summary: This study demonstrates a simple and environmentally-friendly method for the synthesis of zinc oxide nanozymes (ZnO NZs) using wasted hop extract (WHE). The WHE-ZnO NZs exhibit exceptional peroxidase-like activity and serve as effective catalysts for the oxidation of 3,3,5,5-tetramethylbenzidine (TMB) in the presence of hydrogen peroxide (H2O2). In addition, a straightforward colorimetric technique for detecting both H2O2 and glucose was developed using the WHE-ZnO NZs as peroxidase-like catalysts.
Article
Chemistry, Multidisciplinary
Hyunkyu Oh, Young Jun Lee, Eun Ji Kim, Jinseok Park, Hee-Eun Kim, Hyunsoo Lee, Hyunjoo Lee, Bumjoon J. Kim
Summary: Mesoporous carbon particles have unique structural properties that make them suitable as support materials for catalytic applications. This study investigates the impact of channel nanostructures on the catalytic activity of porous carbon particles (PCPs) by fabricating PCPs with controlled channel exposure on the carbon surface. The results show that PCPs with highly open channel nanostructures exhibit significantly higher catalytic activity compared to those with closed channel nanostructures.
Article
Chemistry, Multidisciplinary
Yunjie Lu, Zhaohui Li, Zewei Li, Shihao Zhou, Ning Zhang, Jianming Zhang, Lu Zong
Summary: A tough, long-lasting adhesive and highly conductive nanocomposite hydrogel (PACPH) was fabricated via the synergy of interfacial entanglement and adhesion group densification. PACPH possesses excellent mechanical properties, interfacial adhesion strength, and conductivity, making it a promising material for long-term monitoring of human activities and electrocardiogram signals.
Article
Chemistry, Multidisciplinary
Zichao Wei, Audrey Vandergriff, Chung-Hao Liu, Maham Liaqat, Mu-Ping Nieh, Yu Lei, Jie He
Summary: We have developed a simple method to prepare polymer-grafted plasmonic metal nanoparticles with pH-responsive surface-enhanced Raman scattering. By using pH-responsive polymers as ligands, the aggregation of nanoparticles can be controlled, leading to enhanced SERS. The pH-responsive polymer-grafted nanoparticles show high reproducibility and sensitivity in solution, providing a novel approach for SERS without the need for sample pre-concentration.
Article
Chemistry, Multidisciplinary
Melis Ozge Alas Colak, Ahmet Gungor, Merve Buldu Akturk, Emre Erdem, Rukan Genc
Summary: This research investigates the effect of functionalizing carbon dots with hydroxyl polymers on their performance as electrode materials in a supercapacitor. The results show that the functionalized carbon dots exhibit excellent electrochemical performance and improved stability.