Journal
JOURNAL OF MATERIALS CHEMISTRY C
Volume 4, Issue 33, Pages 7783-7789Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6tc02750d
Keywords
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Funding
- Major State Basic Research Development Program of China [2013CB922101, 2011CB808704]
- National Natural Science Foundation of China [21371090]
- Natural Science Foundation of Jiangsu Province [BK20130054]
- China-South Africa joint research program [CS08-L07, UID: 95421]
- NRF of South Africa CUSR grant [UID: 93627]
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The synthesis and characterization of a subphthalocyanine-bisazobenzene-subphthalocyanine triad are reported. Evidence for E,E <-> E,Z isomerization of the linking bisazobenzene moiety is observed in the optical and NMR spectra when the subphthalocyanine rings are used as light-harvesting units. Electronic coupling and communication between the two para-azo units decrease the photoisomerization efficiency. An obvious decrease in fluorescence intensity is observed on moving from E -> Z with a recovery in intensity observed on moving back from Z -> E that can be attributed to a change in the rate of non-radiative decay.
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