4.8 Article

Strong and Tunable Spin-Orbit Coupling in a Two-Dimensional Hole Gas in Ionic-Liquid Gated Diamond Devices

Journal

NANO LETTERS
Volume 16, Issue 6, Pages 3768-3773

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.6b01155

Keywords

diamond; surface conductivity; 2DHG; spin-orbit splitting; weak antilocalization

Funding

  1. Australian Research Council [DP150101673, DE140100775]
  2. Australian Research Council [DE140100775] Funding Source: Australian Research Council

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Hydrogen-terminated diamond possesses due to transfer doping a quasi-two-dimensional (2D) hole accumulation layer at the surface with a strong, Rashba-type spin orbit coupling that arises from the highly asymmetric confinement potential. By modulating the hole concentration and thus the potential using an electrostatic gate with an ionic-liquid dielectric architecture the spin orbit splitting can be tuned from 4.6-24.5 meV with a concurrent spin relaxation length of 33-16 nm and hole sheet densities of up to 7.23 X 10(13) cm(-2). This demonstrates a spin orbit interaction of unprecedented strength and tunability for a 2D hole system at the surface of a wide band gap semiconductor. With a spin relaxation length that is experimentally accessible using existing nanofabrication techniques, this result suggests that hydrogen-terminated diamond has great potential for the study and application of spin transport phenomena.

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