4.6 Article

A self-driven, polarized-liquid-based ultraviolet photodetector

Journal

CELL REPORTS PHYSICAL SCIENCE
Volume 3, Issue 12, Pages -

Publisher

CELL PRESS
DOI: 10.1016/j.xcrp.2022.101192

Keywords

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Funding

  1. National Natural Science Foundation of China [51202216, 51551203, 61774135]
  2. Outstanding Youth Fund of Zhejiang Natural Science Foundation of China [LR21F040001]
  3. Special Foundation of Young Professor of Zhejiang University [2013QNA5007]
  4. China Postdoctoral Science Foundation [2021M692767]

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In this study, a novel photodetector using polarized liquid to trigger current is demonstrated, which achieves repeatably photoelectric performance without requiring complex growth technologies. Under specific illumination conditions, the photodetector exhibits high responsivity and specific detectivity, which may have significant implications for self-powered photodetectors.
Traditionally, photodetectors are based on solid materials composed of P-N junctions, which require delicate growth technol-ogies. In this article, we demonstrate the feasibility of a polarized -liquid-triggered photodetector where the liquid is sandwiched between P-and N-type semiconductors. Under multiple cycles of optical switching, a transient photopolarized current, a steady-state photopolarized current, and a depolarized current are repeatably observed in a semiconductor/polar liquid/semiconductor structure. The responsivity and specific detectivity of the transient photopo-larized current in N-GaN/W/P-GaN reaches 104.2 mA/W and 4.4 3 10(12) Jones at 365 nm, 52.8 mA/W, and 1.9 3 10(12) Jones at 254 nm illumination under zero bias voltage. We anticipate that our research may be useful for integrating self-powered photodetectors with freely selectable wavelength bands.

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