4.8 Review

Recent Advances in Blue Perovskite Quantum Dots for Light-Emitting Diodes

Journal

SMALL
Volume 18, Issue 1, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/smll.202103527

Keywords

blue emission; light-emitting diodes; metal halide perovskite; quantum dots

Funding

  1. National Natural Science Foundation of China [NSFC] [62074044, 61675049]
  2. Zhongshan-Fudan Joint Innovation Center and Jihua Laboratory Projects of Guangdong Province [X190111UZ190]
  3. Natural Science Foundation of China [61935017, 62004231]
  4. Science and Technology Development Fund, Macao SAR [FDCT-0044/2020/A1, FDCT-091/2017/A2, FDCT-014/2017/AMJ]
  5. UM's research fund [MYRG2018-00148-IAPME]
  6. Natural Science Foundation of Guangdong Province, China [2019A1515012186]
  7. Guangdong-Hong Kong-Macao Joint Laboratory of Optoelectronic and Magnetic Functional Materials [2019B121205002]

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This review highlights recent advances in blue perovskite quantum dots (PQDs), including mixed-halide, quantum-confined all-bromide, metal-doped, and lead-free PQDs, and their applications in PeLEDs. While several excellent PeLEDs based on these PQDs have been demonstrated, there are still many issues to be addressed.
Metal halide perovskite nanostructures have sparked intense research interest due to their excellent optical properties. In recent years, although the green and red perovskite light-emitting diodes (PeLEDs) have achieved a significant breakthrough with the external quantum efficiency exceeding 20%, the blue PeLEDs still suffer from inferior performance. Previous reviews about blue PeLEDs focus more on 2D/quasi-2D or 3D perovskite materials. To develop more stable and efficient blue PeLEDs, a systematic review of blue perovskite quantum dots (PQDs) is urgently demanded to clarify how PQDs evolve. In this review, the recent advances in blue PQDs involving mixed-halide, quantum-confined all-bromide, metal-doped and lead-free PQDs as well as their applications in PeLEDs are highlighted. Although several excellent PeLEDs based on these PQDs have been demonstrated, there are still many problems to be solved. A deep insight into the advantages and disadvantages of these four types of blue-emitting PQDs is provided. Then, their respective potential and issues for blue PeLEDs have been discussed. Finally, the challenges and outlook for efficient and stable blue PeLEDs based on PQDs are addressed.

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