Journal
FOOD CHEMISTRY
Volume 349, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.foodchem.2021.129202
Keywords
Nonenzymatic electrochemical sensor; Glucose; Conductive metal organic frameworks; Human serum; Beverage
Funding
- Talented Program [A279021724]
- Fundamental Research Funds for Northwest A F University [Z111021601]
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A novel electrochemical enzyme-free glucose sensor was developed by growing Ni/Co bimetal MOF on carbon cloth via a facile hydrothermal method, showing excellent activity and sensitivity for monitoring glucose in biological and food samples.
In this work, we propose a electrochemical enzyme-free glucose sensor by direct growth of conductive Ni/Co bimetal MOF on carbon cloth [Ni/Co(HHTP)MOF/CC] via a facile hydrothermal method. Due to excellent conductivity between Ni/Co(HHTP)MOF and CC, synergic catalytic effect of Ni and Co elements, the Ni/Co (HHTP)MOF/CC not only provides larger surface area and more effective active sites, but also boosts the charge transports and electro-catalytic performance. Under optimized conditions, the Ni/Co(HHTP)MOF/CC shows excellent activity with a linear range of 0.3 mu M-2.312 mM, a low detection limit of 100 nM (S/N = 3), a fast response time of 2 s and a high sensitivity of 3250 mu A mM(-1) cm(-2). Furthermore, the Ni/Co(HHTP)MOF/CC was successfully applied for the detection of glucose in real serum and beverages with competitive performances. This facile and cost-effective method provides a novel strategy for monitoring of glucose in biological and food samples.
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