4.7 Article

A TiO2 Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue

Journal

NANOMATERIALS
Volume 11, Issue 1, Pages -

Publisher

MDPI
DOI: 10.3390/nano11010239

Keywords

cellulose; carbon aerogel; titanium dioxide; photo-catalytic degradation; methylene blue

Funding

  1. National Natural Science Foundation of China [51861165203]
  2. Sichuan Science and Technology Program [2019YJ0125]
  3. State Key Laboratory of Polymer Materials Engineering [sklpme2019-2-19]
  4. Opening Project of Guangxi Key Laboratory of Calcium Carbonate Resources Comprehensive Utilization [HZXYKFKT201902]
  5. Special Foundation for Innovation-Driven Development of Hezhou [Hekechuang PT0710004]

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Carbon aerogels coupled with TiO2 derived from bamboo cellulose fibers exhibit extraordinary performance on the photo-catalytic degradation of methylene blue. The CA/TiO2 hybrid demonstrates superior adsorption capacity and photo-catalytic activity, outperforming many similar materials reported in the literature.
Carbon aerogels (CA) derived from bamboo cellulose fibers were coupled with TiO2 to form CA/TiO2 hybrids, which exhibited extraordinary performance on the photo-catalytic degradation of methylene blue (MB). The structure and morphology of CA/TiO2 were characterized by field emission scanning electron microscopy, Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction, and Raman spectrum. The CA displayed a highly porous and interconnected three-dimensional framework structure, while introducing the catalytic active sites of TiO2 onto the aerogel scaffold could remarkably enhance its photo-catalytic activity. The adsorption and photo-catalytic degradation of MB by the CA/TiO2 hybrid were investigated. The maximum adsorption capacity of CA/TiO2 for MB was 18.5 mg/g, which outperformed many similar materials reported in the literature. In addition, compared with other photo-catalysts, the present CA/TiO2 demonstrated superior photo-catalytic performance. Almost 85% of MB in 50 mL solution with a MB concentration of 10 mg/L could be effectively degraded by 15 mg CA/TiO2 in 300 min.

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