4.8 Article

Modulation of Binary Neuroplasticity in a Heterojunction-Based Ambipolar Transistor

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 12, Issue 13, Pages 15370-15379

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.0c00635

Keywords

ambipolar transistor; heterojunction; charge-trapping; synaptic plasticity; image recognition

Funding

  1. National Natural Science Foundation of China [61974093]
  2. Guangdong Province Special Support Plan for High-Level Talents [2017TQ04X082]
  3. Guangdong Provincial Department of Science and Technology [2018B030306028]
  4. Science and Technology Innovation Commission of Shenzhen [JCYJ20180507182042530, JCYJ20180507182000722]
  5. Natural Science Foundation of SZU

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To keep pace with the upcoming big-data era, the development of a device-level neuromorphic system with highly efficient computing paradigms is underway with numerous attempts. Synaptic transistors based on an all-solution processing method have received growing interest as building blocks for neuromorphic computing based on spikes. Here, we propose and experimentally demonstrated the dual operation mode in poly{2,2-(2,5-bis(2-octyldodecyI)-3,6-dioxo-2,3,5,6-tetrahydropyrrolo [3,4-c] pyrrole - 1,4-diyl) dithieno [3,2- b] thiophene-S,Sdiyl-alt-thiophen-2,5-diyl} (PDPPBTT)/ZnO junction-based synaptic transistor from ambipolar charge-trapping mechanism to analog the spiking interfere with synaptic plasticity. The heterojunction formed by PDPPBTT and ZnO layers serves as the basis for hole-enhancement and electron-enhancement modes of the synaptic transistor. Distinctive synaptic responses of paired-pulse facilitation (PPF) and paired-pulse depression (PPD) were configured to achieve the training/recognition function for digit image patterns at the device-to-system level. The experimental results indicate the potential application of the ambipolar transistor in future neuromorphic intelligent systems.

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