Journal
CHEMSUSCHEM
Volume 12, Issue 7, Pages 1310-1315Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201900043
Keywords
chemoenzymatic cascades; choline oxidase; limonene; lipase; natural deep eutectic solvents
Funding
- National Key R&D Program of China [2018YFC0311104]
- National Outstanding Youth Science Foundation of China [31725022]
- International Collaboration Base for Molecular Enzymology and Enzyme Engineering [2017A050503001]
- State Key Laboratory of Pulp and Paper Engineering [2017-04-SKLPPE]
- 111 Project [B17018]
- European Research Commission (ERC) [648026]
- European Union [H2020-BBI-PPP-2015-2-1-720297]
- Netherlands Organisation for Scientific Research (VICI grant) [724.014.003]
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The use of natural deep eutectic solvents (NADES) as multifunctional solvents for limonene bioprocessing was reported. NADES were used for the extraction of limonene from orange peel wastes, as solvent for the chemoenzymatic epoxidation of limonene, and as sacrificial electron donor for the insitu generation of H2O2 to promote the epoxidation reaction. The proof-of-concept for this multifunctional use was provided, and the scope and current limitations of the concept were outlined.
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