Journal
RSC ADVANCES
Volume 3, Issue 40, Pages 18661-18670Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ra42076k
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Funding
- National Ministry of Science and Technology Innovation Fund for High-tech Small and Medium Enterprise Technology [09C26215112399]
- National Ministry of Human Resources and Social Security Start-up Support Projects for Students Returned to Business, Office of Human Resources and Social Security [143]
- Fundamental Research Funds for the Central Universities [XDJK2013C120]
- Xihua University Key Projects [Z1223321]
- Sichuan Province Applied Basic Research Projects [2013JY0090]
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A series of novel types of chiral salen Mn(III) anchored onto ZnPS-PVPA containing 1,2,3-triazole were synthesized by means of click chemistry. These supported catalysts were highly active and enantioselective (conversion up to 99%; ee up to 99%) in the asymmetric epoxidation of unfunctionalized olefins and were selective for the oxidants. Moreover, these heterogeneous catalysts could still show good catalytic ability after recycling nine times. Furthermore, the catalyst could also maintain its superior catalytic properties in large-scale reactions, which demonstrate their potential for application in industry.
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