Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 1, Issue 8, Pages 1336-1339Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cy00253h
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Funding
- EPSRC
- Washington and Lee University
- R.E. Lee Research Fellowship
- Swedish Reseach Council
- Associated Colleges of the South Andrew W. Mellon Faculty
- EPSRC [EP/G036314/1, EP/F030576/1, EP/G063591/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/G036314/1, EP/G063591/1, EP/F030576/1] Funding Source: researchfish
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Methods to produce a range of new phosphine-diamine ligands from phosphino-aldehydes have been developed and a hypothesis that larger P-substituents would increase the enantioselectivity towards the (S) isomer in Ru-catalysed ketone hydrogenation of acetophenone has been examined; the successful validation of this hypothesis is further evidence that the mechanism of these catalysts involves a secondary amine assisted reduction.
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