4.4 Article

Energy transfer in plasmonic systems

Journal

JOURNAL OF OPTICS
Volume 16, Issue 11, Pages -

Publisher

IOP PUBLISHING LTD
DOI: 10.1088/2040-8978/16/11/114015

Keywords

energy transfer; plasmons; fluorescence

Categories

Funding

  1. NSF Grant [DMR-1206975]
  2. Division Of Human Resource Development
  3. Direct For Education and Human Resources [0833178] Funding Source: National Science Foundation
  4. Division Of Materials Research
  5. Direct For Mathematical & Physical Scien [1206975] Funding Source: National Science Foundation

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We present our results on energy transfer between donor and acceptor molecules or quantum dots near a plasmonic nanoparticle. In such systems, the Forster resonance energy transfer is strongly modified due to plasmon-mediated coupling between donors and acceptors. The transfer efficiency is determined by a competition between transfer, radiation and dissipation that depends sensitively on system parameters. When donor and accepror spectral bands overlap with dipole surface plasmon resonance, the dominant transfer mechanism is through plasmon-enhanced radiative coupling. When transfer takes place from an ensemble of donors to an acceptor, a cooperative amplification of energy transfer takes place in a wide range of system parameters.

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