Journal
SURFACE & COATINGS TECHNOLOGY
Volume 261, Issue -, Pages 364-374Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.surfcoat.2014.10.061
Keywords
Ni-Al-Cr bond coat/substrate; Interdiffusion; Temperature gradient; Phase-field simulation; CALPHAD
Funding
- National Natural Science Foundation of China [51301208, 51474239]
- Hunan Provincial Natural Science Foundation for Youths of China [2015JJ3146]
- National Basic Research Program of China [2011CB610401, 2014CB644002]
- Sino-German Center for Promotion of Science [GZ 755]
- Shenghua Scholar Program of Central South University, Changsha, PR China
- Foundation for the Author of Provincial Excellent Doctoral Dissertation of Hunan
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Two-dimensional (2-D) phase-field simulations were employed in the present work to investigate the effect of temperature gradient on the microstructure evolution in various Ni-Al-Cr bond coat/substrate systems (i.e., beta/gamma + gamma', gamma + beta/gamma + gamma', gamma' + beta/gamma + gamma') with the aid of MICRESS (MICRostructure Evolution Simulation Software). Reliable CALPHAD (CALculation of PHAse Diagram) thermodynamic and atomic mobility databases were coupled via TQ interface. The gamma/gamma' interfacial energy was estimated by using the Kaptay's method. The present phase-field simulations indicate that component Al migrates towards substrate, while component Cr towards bond coat during the interdiffusion process. The temperature gradient promotes diffusion of both Al and Cr, which greatly accelerates the failure of various bond coat/substrate systems caused by the rapid depletion of Al concentration in bond coat. Furthermore, the formation of gamma' polycrystalline structure around bond coat/substrate interface as well as in the substrate is also observed, which may result in the generation of intergranular fracture and crack propagation. (C) 2014 Elsevier B.V. All rights reserved.
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