Journal
LANGMUIR
Volume 30, Issue 12, Pages 3502-3506Publisher
AMER CHEMICAL SOC
DOI: 10.1021/la500873y
Keywords
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Funding
- National Key Project on Basic Research [2011CB808700, 2011CB932304]
- National Natural Science Foundation of China [21121063, 21073204, 21373236, 21127901]
- Beijing Municipal Education Commission [20118000101]
- Chinese Academy of Sciences
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Hybrid bilayers consisting of 8-hydroxypyrene-1,3,6-trisulfonic acid trisodium salt (HPTS) and meso-tetra(4-pyridyl)porphine (TPyP) have been successfully constructed on Au(111) and investigated by electrochemical scanning tunneling microscopy (ECSTM). Under the guidance of the electrostatic interaction between negatively charged sulfonate groups and positively charged pyridyl groups, the underlying HPTS arrays act as templates for the deposition of cationic TPyPs, forming two types of TPyP/HPTS complex bilayers. The present work provides a feasible way to fabricate hybrid multilayers on the electrode surface via electrostatic interaction, which has great significance for the design of molecular nano devices.
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