Article
Public, Environmental & Occupational Health
Siqin Chen, Xingyue Yin, Yuefeng He, Qinghua He, Xiaomei Li, Maosheng Yan, Suli Huang, Jiachun Lu, Binyao Yang
Summary: This study suggests that co-exposure to PAHs and smoking, along with XPC gene polymorphisms, can increase individual susceptibility to DNA damage. More specifically, base modifications in the KRAS and BRAF exons were positively associated with levels of 1-hydroxypyrene (1-OH-Pyr). Additionally, the effects were more pronounced in individuals carrying specific XPC genotypes. These findings highlight the importance of considering genetic factors in understanding individual responses to environmental exposure.
FRONTIERS IN PUBLIC HEALTH
(2022)
Article
Chemistry, Analytical
Jeerakit Thangphatthanarungruang, Chuleekorn Chotsuwan, Weena Siangproh
Summary: 1-Hydroxypyrene (1-OHP), as a metabolite of polycyclic aromatic hydrocarbons (PAHs), is commonly used to assess human exposure to PAHs. A new electrochemical device based on poly(L-glutamic acid)-modified a screen-printed graphene electrode (poly(L-GA)/SPGE) for 1-OHP detection was created. The developed sensor showed a linear detection range of 1-1000 nM with detection and quantification limits of 0.95 and 3.16 nM, respectively. This sensor was successfully applied to determine 1-OHP in human urine samples, providing a valuable tool for early detection of illness risk related to PAHs in the human body.
Article
Multidisciplinary Sciences
Yusuke Nakakuki, Takashi Hirose, Hikaru Sotome, Min Gao, Daiki Shimizu, Ruiji Li, Jun-Ya Hasegawa, Hiroshi Miyasaka, Kenji Matsuda
Summary: Helically twisted conductive nanocarbon materials are suitable for optoelectronic and electromagnetic molecular devices on the nanometer scale, showing a large effective conjugation length and ultrafast decay dynamics. The extended π-helicenes achieved a large effective conjugation length through helical fusion, leading to an absorption edge in the near-infrared region.
NATURE COMMUNICATIONS
(2022)
Article
Chemistry, Multidisciplinary
Xiushang Xu, Amy L. Vonder Haar, Rengo Yoshioka, Qizheng Zhang, Serhii Vasylevskyi, Andrew J. Musser, Akimitsu Narita
Summary: A benzo[rst]pentaphene derivative, BPP-MeOPA, was synthesized and characterized by NMR and single-crystal X-ray analysis. Investigation of its photophysical properties, including transient absorption spectroscopy, revealed improved absorption and emission features from an S-1 state with excitonic and charge-transfer character by introducing MeOPA groups.
CHEMICAL COMMUNICATIONS
(2023)
Review
Environmental Sciences
Meng Qiao, Weixiao Qi, Huijuan Liu, Jiuhui Qu
Summary: Oxygenated polycyclic aromatic hydrocarbons (OPAHs) have higher concentrations and toxicity in water environments, posing significant ecological risks to surface water ecosystems.
ENVIRONMENT INTERNATIONAL
(2022)
Article
Chemistry, Organic
Yushi Ohno, Shogo Ando, Daisuke Furusho, Ryoyu Hifumi, Yuuya Nagata, Ikuyoshi Tomita, Shinsuke Inagi
Summary: Here, a facile and selective synthesis of cationic azatriphenylene derivatives was achieved through electrochemical intramolecular cyclization, where the key step involves atom-economical C-H pyridination without a transition-metal catalyst or an oxidant. This proposed strategy provides a practical approach for introducing cationic nitrogen (N (+)) into pi-electron systems, thus expanding the molecular design of N (+)-doped polycyclic aromatic hydrocarbons.
Article
Chemistry, Inorganic & Nuclear
Huimin Zhong, Cong Jiang, Jiahui Zou, Guancheng Zhu, Yanyan Huang
Summary: In this study, CeO2-based porous carbonaceous frameworks (CeO2 PCFs) were used as antioxidant nanozymes to scavenge reactive oxygen species and absorb benzo[a]pyrene. CeO2 PCFs exhibited excellent superoxide dismutase-like and catalase-like activity, effectively eliminating superoxide radical, hydroxyl radical, and hydrogen peroxide. The 2,2'-azino-bis(3-ethylbenzthiazoline-6-sulfonic acid) free radical scavenging assay confirmed the free radical scavenging ability of CeO2 PCFs. Furthermore, CeO2 PCFs with large surface area and porous structure efficiently adsorbed benzo[a]pyrene. The designed CeO2 PCFs can serve as new antioxidant nanozymes for scavenging reactive oxygen species and adsorbing polycyclic aromatic hydrocarbons (PAHs).
INORGANIC CHEMISTRY
(2023)
Article
Environmental Sciences
Siqin Chen, Yuefeng He, Maosheng Yan, Yun Zhou, Qinghua He, Jingwen Tan, Binyao Yang
Summary: The study revealed a linear dose-effect association between exon damage of EGFR and PAH exposure, with differences in genetic contributions to exon damage. The presence of FEN1rs rs174538 showed modifying effects on the associations of urinary 1-OH-pyr with EGFR-19 and EGFR-21, indicating potential at-risk subpopulations susceptible to adverse health effects induced by PAH exposure.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2021)
Article
Chemistry, Multidisciplinary
Hong Cui, Shuaishuai Cui, Qiuju Tian, Siyuan Zhang, Mingxiu Wang, Ping Zhang, Yunfeng Liu, Jialing Zhang, Xiangjun Li
Summary: The nanocomposite of PAMAM/Cr-MOF/GO showed enhanced electrocatalytic effect on the electrochemical reduction of 1-OHPyr. The synergistic effect from the high porosity of Cr-MOF and high conductivity of ERGO, along with further electron transport action of the nanocomposite, contributed to this enhancement. The constructed electrochemical sensor exhibited good linear relationship in detecting 1-OHPyr, with a low detection limit, suggesting potential wide applications in electrochemical sensing platforms.
Article
Chemistry, Physical
Thomas Liu, Baptiste Carles, Christine Elias, Claire Tonnele, Daniel Medina-Lopez, Akimitsu Narita, Yannick Chassagneux, Christophe Voisin, David Beljonne, Stephane Campidelli, Loic Rondin, Jean-Sebastien Lauret
Summary: In this study, we conducted single-molecule spectroscopy at cryogenic temperatures to investigate the optical properties of graphene quantum dots (GQDs). We found that temperature has an effect on the spectral characteristics of GQDs, and we used density functional theory calculations to explain these observations. Additionally, we discovered that the vibrational features can serve as a unique fingerprint for identifying GQDs.
JOURNAL OF CHEMICAL PHYSICS
(2022)
Article
Thermodynamics
Chia Chun Lee, Manh-Vu Tran, Boon Thong Tan, Gianfranco Scribano, Cheng Tung Chong, Jong Boon Ooi
Summary: The study found that the addition of ethanol can increase the concentration of aromatic substances in methane diffusion flames, with the chemical effect being the main factor, followed by the dilution effect and the thermal effect. The increase in pressure accelerates the production of aromatics, as the narrowing of the flames improves air entrainment and significantly speeds up overall reactivity.
Article
Environmental Sciences
Hao Zhang, Xuan Zhang, Yan Wang, Pengchu Bai, Lulu Zhang, Lijiang Chen, Chong Han, Wangjin Yang, Qimin Wang, Yunping Cai, Seiya Nagao, Ning Tang
Summary: Shenyang, the provincial capital of Liaoning province in China, is heavily polluted due to its high population and heavy machinery manufacturing. This study analyzed the concentrations of nine polycyclic aromatic hydrocarbons (PAHs) and 1-nitropyrene (1NP) in aerosol samples collected in Shenyang from 2014 to 2020. The results showed a decrease in the annual mean concentration of PAHs and 1-NP during this period, attributed to the transition from coal to electric and natural gas heating, upgrades in heating stoves and improved vehicle and fuel standards. Notably, the proportion of 4-ring PAHs increased in summer but decreased in winter from 2014 to 2020. Possible reasons for this difference were identified, such as the use of higher cetane rating fuel in summer and the use of air pollution control devices in winter. Despite the decrease in health risks, the concentrations of PAHs and 1-NP in Shenyang during the winter of 2020 still exceeded national standards, indicating the need for additional environmental regulations to further improve air quality in the city.
ATMOSPHERIC POLLUTION RESEARCH
(2023)
Review
Environmental Sciences
Jamie M. Dearnley, Charles Killeen, Rebecca L. Davis, Vince P. Palace, Gregg T. Tomy
Summary: This article reviews the metabolism and toxicity of polycyclic aromatic compounds (PACs) in fish and presents various methods for analyzing metabolite-containing bile. Recent environmental monitoring studies demonstrate the utility of this technique in assessing oil spill pollution, establishing baseline exposure, and evaluating pollution in urban waterways.
CRITICAL REVIEWS IN ENVIRONMENTAL SCIENCE AND TECHNOLOGY
(2022)
Article
Chemistry, Multidisciplinary
Matthias Schnitzlein, Chongwei Zhu, Kazutaka Shoyama, Frank Wuerthner
Summary: In this study, negatively curved pi-extended pleiadienes were synthesized using palladium-catalyzed reaction. The crystal structure and theoretical calculations revealed the unique properties of these compounds. Additionally, a naphthalene-fused pleiadiene was formed through a chemical reaction, resulting in a new aromatic compound with distinct properties.
CHEMISTRY-A EUROPEAN JOURNAL
(2022)
Article
Engineering, Environmental
Jiaxing Lu, Jian Zhang, Huijun Xie, Yuming Jing, Mingde Ji, Zhen Hu
Summary: In this study, a novel wastewater treatment process combining sequencing batch reactor, constructed wetland and microalgal membrane photobioreactor (BCM process) was proposed. The process achieved satisfactory removal of polycyclic aromatic hydrocarbons (PAHs) and their substituted derivatives (SPAHs), and significantly reduced bacterial toxicity and genotoxicity. Microalgae played an important role in ensuring water security.
Article
Environmental Sciences
Yu-Sheng Shen, Shih-Chun Candice Lung, Shenghui Cui
Summary: This study examines the mediating effects of urban form on suicide mortality and identifies crucial factors such as urban development intensity, land mix, and urban sprawl. It also highlights the importance of air pollution and high temperature in relation to suicide rates. The findings emphasize the role of urban policy and planning in suicide prevention and building healthy cities.
ENVIRONMENTAL POLLUTION
(2022)
Article
Environmental Sciences
Shih-Chun Candice Lung, To Thi Hien, Maria Obiminda L. Cambaliza, Ohnmar May Tin Hlaing, Nguyen Thi Kim Oanh, Mohd Talib Latif, Puji Lestari, Abdus Salam, Shih-Yu Lee, Wen-Cheng Vincent Wang, Ming-Chien Mark Tsou, Tran Cong-Thanh, Melliza Templonuevo Cruz, Kraichat Tantrakarnapa, Murnira Othman, Shatabdi Roy, Tran Ngoc Dang, Dwi Agustian
Summary: The low-cost and easy-to-use PM2.5 sensors provide an opportunity for breakthroughs in PM2.5 research in resource-limited countries in Southeast Asia. This review evaluates the available literature and identifies research priorities for low-cost sensor deployment in PM2.5 environmental and health research in the region. The research priorities focus on filling gaps in PM2.5 research, including source evaluation, hot spot investigation, exposure assessment, and health impacts evaluation.
INTERNATIONAL JOURNAL OF ENVIRONMENTAL RESEARCH AND PUBLIC HEALTH
(2022)
Article
Environmental Sciences
Ming-Lun Zou, Chuen-Bin Jiang, Yi-Hua Chen, Chih-Da Wu, Shih-Chun Candice Lung, Ling-Chu Chien, Kraiwuth Kallawicha, Yu-Chun Lo, Hsing Jasmine Chao
Summary: This study investigated the effects of air pollution, land use types, and parental mental health on respiratory symptoms in children aged <2 years in the Greater Taipei area. The results showed that postnatal exposure to PM2.5 and O-3 was positively associated with respiratory symptoms in children. Traffic-related land use types, sports facilities, and commercial land had adverse effects, while the presence of schools in the neighborhood was beneficial. Parental mental health was also associated with children's respiratory symptoms.
ENVIRONMENTAL RESEARCH
(2022)
Article
Multidisciplinary Sciences
Murnira Othman, Mohd Talib Latif, Haris Hafizal Abd Hamid, Royston Uning, Thipsukon Khumsaeng, Worradorn Phairuang, Zawawi Daud, Juferi Idris, Nurzawani Md Sofwan, Shih-Chun Candice Lung
Summary: This study investigates the characteristics of particulate matter (PM) in Southeast Asia, particularly in Malaysia and Thailand, using spatial-temporal data. The results indicate that these regions are significantly affected by biomass burning activity during the dry seasons and the Southwest monsoon.
SCIENTIFIC REPORTS
(2022)
Article
Geosciences, Multidisciplinary
Wan-Yu Shih, Shih-Chun Candice Lung, Shu-Chuan Hu
Summary: Extreme high temperature poses significant threats to public health. Subjective heat-health symptoms are more direct motivations for heat adaptive behaviours. Age, gender, and health condition are related to the frequency of feeling moody and ill, as well as the use of umbrellas and hats. Biophysical acclimatisation and adaptation of behaviours were found among people frequently working outdoors.
INTERNATIONAL JOURNAL OF DISASTER RISK REDUCTION
(2022)
Review
Allergy
Marine Savoure, Jean Bousquet, Jouni J. K. Jaakkola, Maritta S. Jaakkola, Benedicte Jacquemin, Rachel Nadif
Summary: This review summarizes the literature on the prevalence of rhinitis in the general adult population. It found a great heterogeneity in the definitions of rhinitis. Most studies focused on allergic rhinitis, with limited epidemiological data on nonallergic rhinitis. Rhinitis prevalence varied geographically and seemed to increase over time.
CLINICAL AND TRANSLATIONAL ALLERGY
(2022)
Article
Environmental Sciences
Henna Hyrkas-Palmu, Maritta S. Jaakkola, Elina M. S. Makikyro, Jouni J. K. Jaakkola
Summary: The subtype and control of asthma are related to cold weather-related respiratory symptoms, with more severe and poorly controlled asthma patients being more likely to experience these symptoms compared to those with mild and well-controlled asthma.
INTERNATIONAL JOURNAL OF ENVIRONMENTAL RESEARCH AND PUBLIC HEALTH
(2022)
Article
Environmental Sciences
Shih-Yu Lee, Shih-Chun Candice Lung, Ping-Gin Chiu, Wen-Cheng Wang, I-Chun Tsai, Thung-Hong Lin
Summary: Increasing surface air temperature due to global warming leads to heat stress, which has potential impacts on human health. This study found a general increase in heat stress over the past decade, with tropical regions experiencing the highest warming. On the urban scale, heat stress may have led to a reduction in labor hours by up to 20% in some Asian cities. The exposure to heat stress is a collective challenge with environmental, economic, and social implications.
INTERNATIONAL JOURNAL OF ENVIRONMENTAL RESEARCH AND PUBLIC HEALTH
(2022)
Article
Psychiatry
Aji Kusumaning Asri, Hui-Ju Tsai, Wen-Chi Pan, Yue Leon Guo, Chia-Pin Yu, Chi-Shin Wu, Huey-Jen Su, Shih-Chun Candice Lung, Chih-Da Wu, John D. Spengler
Summary: This study aimed to investigate the association between greenness and the burden of depressive disorders globally. The findings showed a significant negative association between greenness and the health burden of depressive disorders. The beneficial effects of greenness were observed across various socio-demographic levels.
FRONTIERS IN PSYCHIATRY
(2022)
Letter
Allergy
Laurent Orsi, Marine Savoure, Jean Bousquet, Benedicte Jacquemin, Valerie Siroux, Maritta S. Jaakkola, Jouni J. K. Jaakkola, Benedicte Leynaert, Rachel Nadif
Article
Environmental Sciences
Maritta S. Jaakkola, Henna Hyrkas-Palmu, Jouni J. K. Jaakkola
Summary: This study assessed the relationship between indoor dampness and mold exposure and the level of asthma control among adults. The results showed that exposure to indoor dampness was associated with reduced asthma control, especially among men. However, indoor visible mold and mold odor were not significantly related to asthma control.
INTERNATIONAL JOURNAL OF ENVIRONMENTAL RESEARCH AND PUBLIC HEALTH
(2022)
Letter
Allergy
Ines Paciencia, Aino K. Rantala, Harri Antikainen, Timo T. Hugg, Maritta S. Jaakkola, Jouni J. K. Jaakkola
Article
Public, Environmental & Occupational Health
Abate Bekele Belachew, Aino K. Rantala, Maritta S. Jaakkola, Timo T. Hugg, Jouni J. K. Jaakkola
Summary: Using data from a population-based prospective study, we found that individuals with asthma are more susceptible to respiratory tract infections (RTIs). This susceptibility is evident from childhood to young adulthood, with increased risks of both upper and lower RTIs. Women with asthma are at a particularly high risk.
AMERICAN JOURNAL OF EPIDEMIOLOGY
(2023)
Article
Public, Environmental & Occupational Health
Abate Bekele Belachew, Aino K. Rantala, Maritta S. Jaakkola, Timo T. Hugg, Reija Ruuhela, Jaakko Kukkonen, Jouni J. K. Jaakkola
Summary: This study found that a decrease in average winter temperature is associated with an increased risk of developing new asthma. A cold winter with below normal temperatures increases the risk of new asthma by 41% in the following year.
OCCUPATIONAL AND ENVIRONMENTAL MEDICINE
(2023)
Article
Food Science & Technology
Kuang-Mao Chiang, Lili Xiu, Chiung-Yu Peng, Shih-Chun Candice Lung, Yu-Cheng Chen, Wen-Harn Pan
Summary: This study comprehensively examined the emissions from deep-frying foods using different oils and explored the relationships between emitted substances, oil quality parameters, and fatty acid profiles. The results showed that palm oil emitted the highest concentration of total particle matters, soybean oil emitted the highest level of gaseous aldehydes, and olive oil seemed to be superior to soybean and palm oils regarding toxic emissions during deep-frying.
NPJ SCIENCE OF FOOD
(2022)