Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 129, Issue 12, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.2978381
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Funding
- Nanyang Technological University URC [RG 47/07]
- DSO National Laboratories
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We present the theory and the selection procedure of phase-cycling schemes for phase coherent multidimension optical spectroscopy. We apply our selection procedure to determine the phase-cycling schemes with the least number of steps needed to measure the two-dimensional spectra of various time resolved four wave mixing optical processes. The phase-cycling scheme selection procedure presented in this paper can be applied to higher order nonlinear optical experiments involving more optical pulses that measure higher dimensional optical spectra. (C) 2008 American Institute of Physics.
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