4.7 Article

Abatement of mercury emissions in the coal combustion process equipped with a Fabric Filter Baghouse

Journal

FUEL
Volume 87, Issue 15-16, Pages 3322-3330

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.fuel.2008.05.010

Keywords

CFBC; PC; mercury emission; Fabric filter baghouse; fly ash

Funding

  1. United State Department of Energy [DE-FC26-03NT41840]
  2. Kentucky Office of Energy Policy [PO2 855 0600002929 1]
  3. USDA-ARS [6406-12630-002-02S]

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The purpose of this study was to investigate the dependence of mercury emissions on coal ranks and electric utility boilers equipped with Fabric Filter Baghouses (FF). A comparison of mercury emission rates and fly ash properties was made between a circulating Fluidized Bed Combustor (CFBC) with FF and a Pulverized Coal (PC) combustor with FF during the burning of all three ranks of American coals. The data were collected from the Environmental Protection Agency Information Collection Request (EPA ICR) and WKU ICSET's mercury testing program. A statistical stepwise regression procedure was used to determine significant factors such as coal rank and types of boilers equipped with FF on mercury emissions during coal combustion. The higher mercury emission rates were generally found in both CFB and PC units when lignite was burned. The lower mercury emission rates were generally found in both CFB equipped with FF and PC units equipped with FF when bituminous coal was burned. There was a statistically significant lower mercury emission in the CFBC equipped with FF than that in the PC units when sub-bituminous coal was burned. Lower mercury emission rates in electric utility boilers equipped with FF are due to the active fly ash generated with a larger specific surface area and pore volume. Higher mercury emission rates observed during lignite-fired boilers may be due to their lower specific area of fly ash, which results from lower LOI, as well as the pore blockage by selenium (Se) for Texas lignite; and sodium (Na) and potassium (K) for North Dakota lignite. There is no significant mutual benefit for the mercury captured by the addition of Spray Dry Absorber (SDA) or selective non-catalytic reduction (SNCR) in the CFBC system. (c) 2008 Elsevier Ltd. All rights reserved.

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