Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2014, Issue 6, Pages 1177-1181Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201301849
Keywords
Radicals; Cyclization; Dienes; C-H activation; Nitrogen heterocycles
Categories
Funding
- National Natural Science Foundation of China [21172060]
- Specialized Research Fund for Doctoral Program of Higher Education [20120161110041]
- Hunan Provincial Natural Science Foundation of China [13JJ2018]
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A general and conceptually novel method for preparing polychloro-substituted pyrrolidin-2-ones and indeno[2,1-c]pyrrol-3(3aH)-ones is established by visible-light-facilitated 5-exo-trig cyclization of 1,6-dienes with alkyl chlorides through selectively splitting the C(sp(3))-H bond adjacent to the chloride atom to form an alkyl radical.
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