Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2012, Issue 1, Pages 183-187Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201101365
Keywords
Organocatalysis; Asymmetric catalysis; Allylic compounds; Amines
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Funding
- Shanghai Municipal Committee of Science and Technology [08dj1400100-2]
- National Basic Research Program of China [(973)-2010CB833302]
- National Natural Science Foundation of China [21072206, 20472096, 20872162, 20672127, 20821002, 20732008]
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We developed a synthetic method to prepare chiral multifunctional thiourea-phosphane catalysts for the asymmetric allylic substitution reaction of Morita-Baylis-Hillman carbonates with diphenyl phosphite or diphenylphosphane oxide to give allylic phosphites and allylic phosphane oxides in high yields with excellent enantioselectivity.
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