Article
Environmental Sciences
Stephanie M. Berg, Benjamin D. Peterson, Katherine D. McMahon, Christina K. Remucal
Summary: This study evaluates the composition of dissolved organic matter (DOM) in Lake Mendota as a function of time and depth. The researchers analyze dissolved organic carbon concentrations and optical properties of samples collected from June to November, and use Fourier transform-ion cyclotron resonance mass spectrometry (FT-ICR MS) to investigate DOM composition at the molecular level. The results show that DOM composition varies both temporally and with depth, with photochemical reactions and redox conditions playing important roles. The findings have implications for understanding the flux of CO2 in lakes and the impact of lake eutrophication.
JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES
(2022)
Article
Engineering, Environmental
Zhixiang She, Jin Wang, Chen He, Xin Pan, Yunyun Li, Siyu Zhang, Quan Shi, Zhengbo Yue
Summary: The study revealed a highly stratified quality of dissolved organic matter (DOM) in acid mine drainage (AMD), linked with severe biogeochemical gradients. DOM molecules exhibited significant differences across different layers, influenced by material exchange with sediments at the bottom.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2021)
Article
Engineering, Civil
Qi Huang, Lizhen Liu, Jiacong Huang, Dianwei Chi, Adam Thomas Devlin, Huawu Wu
Summary: The seasonal dynamics of CDOM and DOC in Poyang Lake are important for understanding biogeochemical processes and water quality. Rivers and wetlands greatly influence the quantity and quality of CDOM. The alternations of flood and dry periods have different effects on CDOM and DOC. Wetlands contribute a higher abundance of CDOM and DOC to the lake with lower aromaticity.
JOURNAL OF HYDROLOGY
(2022)
Article
Environmental Sciences
Donglin Li, Fengqin Chang, Yang Zhang, Lizeng Duan, Qi Liu, Haoyu Li, Guangzhi Hu, Xiaonan Zhang, Youhong Gao, Hucai Zhang
Summary: The lability and controlling factors of arsenic (As) at the sediment-water interface (SWI) were investigated using various sampling techniques and chemical analyses. The results showed that the migration of As in the lake was influenced by seasonal changes and the presence of organic matter (OM) and iron oxides. These findings provide valuable insights into the behavior and fate of arsenic in similar environments.
SCIENCE OF THE TOTAL ENVIRONMENT
(2023)
Article
Environmental Sciences
Yanan Liu, Jingya Xue, Zhifan Gui, Lu Zhang, Xiaolong Yao
Summary: This study investigates the photoreactivity of dissolved organic matter (DOM) from different sources in the Lake Taihu basin. The results show that the original composition and sources of DOM are closely related to its photoreactivity. DOM from macrophytes releases soluble components under light exposure, while DOM with higher aromacity shows photobleaching effects and increased humification degree. Allochthonous anthropogenic DOM exhibits stronger photo-ammonification. The form of inorganic nutrient releases during DOM photolysis also varies with the original DOM sources.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2023)
Article
Limnology
Michael L. Pace, Cal D. Buelo, Stephen R. Carpenter
Summary: Lake respiration is supported by a combination of autochthonous and allochthonous resources, with temperature and organic matter inputs influencing the process. However, the variability in daily inputs can lead to fluctuations in respiration rates, with nutrients not directly tracking phytoplankton blooms in the lakes. Changes in hydrologic, climatic, and land use factors may result in linear responses in ecosystem processes like respiration.
LIMNOLOGY AND OCEANOGRAPHY
(2021)
Article
Environmental Sciences
Dharshika Welikala, Brett H. Robinson, Elena Moltchanova, Adam Hartland, Niklas J. Lehto
Summary: The release of dissolved organic matter (DOM) from Cd contaminated soils is linked to the mobilisation of Cd-DOM complexes, with organic matter-rich soil amendments exacerbating this process. The quantity and quality of DOM determine the proportion of dissolved Cd that forms mobile complexes, affecting Cd transport from contaminated soils. Structural properties of DOM play a key role in the mobilisation of Cd from contaminated soils, as observed in this study.
Article
Environmental Sciences
Zhengyu Wu, Zhike Li, Bo Shao, Yiyan Zhang, Wei He, Yiren Lu, Kair Gusvitskii, Yingxin Zhao, Yurong Liu, Xuejun Wang, Yindong Tong
Summary: The input of mercury (Hg) into ecosystems has increased significantly since the industrial revolution, and methylmercury (MeHg) is the most concerning species in aquatic ecosystems due to its neurotoxicity and ability to bioaccumulate in the food chain. Dissolved organic matter (DOM) plays a crucial role in the transformation of aquatic Hg. This study collected water samples from 373 sites globally and found that Hg availability was the dominant factor influencing MeHg concentration in water, followed by DOM.
Article
Environmental Sciences
Pei Lei, Jinjie Zhu, Jin Zhang, Huan He, Mingying Chen, Huan Zhong
Summary: Algal organic matter (AOM) hinders the photodegradation of neurotoxic methylmercury (MeHg) in eutrophic lakes due to dynamic changes in AOM during algal decomposition. The inhibitory effect of AOM on MeHg photodegradation varies among lakes and their eutrophication states. Reactive oxygen species (ROS), including hydroxyl radical, singlet oxygen, and DOM-D-3*, play different roles in driving MeHg photodegradation throughout the algal decomposition process. This study highlights the importance of considering AOM-MeHg interactions in predicting MeHg risks and suggests integrating them into Hg biogeochemical cycling models.
SCIENCE OF THE TOTAL ENVIRONMENT
(2023)
Article
Environmental Sciences
Haoyu Ren, Xin Yao, Feiyang Ma, Tuantuan Fan, Huanguang Deng, Yinghao Zhang
Summary: Nansi Lake is the largest lake along the eastern route of China's SNWDP, with spatial and temporal differences in DOM properties between its upper and lower areas. Protein-like substances play a significant role in influencing DOM properties in April and July.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2021)
Article
Environmental Sciences
Sarah E. Janssen, Michael T. Tate, Brett A. Poulin, David P. Krabbenhoft, John F. DeWild, Jacob M. Ogorek, Matthew S. Varonka, William H. Orem, Jeffrey L. Kline
Summary: Mercury contamination in the Florida Everglades has been a persistent concern. This study examined mercury and methylmercury dynamics in different media and found strong linkages between air, water, and biota in the system. Changes in hydrology and climate were the main drivers of temporal patterns across different matrices. Unlike other regions, there was no evidence of a decline in atmospheric mercury deposition in this region. The study also identified geographic regions susceptible to higher methylmercury bioaccumulation, particularly in the Shark River Slough and Coastal areas. Improved water quality and flow rates, two key targets of the restoration program, are expected to reduce methylmercury production and exposure.
SCIENCE OF THE TOTAL ENVIRONMENT
(2022)
Article
Environmental Sciences
Biao Li, Muhua Feng, Xiangchao Chen, Yarui Wang, Yue Shen, Qinglong L. Wu
Summary: Abundant organic matters potentially exacerbate chemical iron reduction, leading to the occurrence of black bloom in deep lakes like Lake Fuxian.
ENVIRONMENTAL POLLUTION
(2021)
Article
Engineering, Environmental
Xilin Xiao, Leanne C. Powers, Jihua Liu, Michael Gonsior, Rui Zhang, Lianbao Zhang, Hugh L. MacIntyre, Xiaowei Chen, Chen Hu, John Batt, Qiang Shi, Dapeng Xu, Yao Zhang, Nianzhi Jiao
Summary: A study found that microbial processes play important roles in the transformation of terrigenous organic matter (TOM) during freshwater-seawater mixing, including the biodegradation of dissolved organic matter, changes in bacterial community structure and diversity. In addition, the sinking of surface-derived TOM may lead to increased transformation of dissolved organic matter and carbon storage in the bottom water.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2022)
Article
Engineering, Environmental
Katarina Kajan, Helena Osterholz, James Stegen, Marija Gligora Udovic, Sandi Orlic
Summary: Lakes play a crucial role in the global carbon cycle, and understanding the interactions between microbial and dissolved organic matter (DOM) diversity is essential for predicting the function of lake ecosystems. This study used high-throughput sequencing and mass spectrometry to investigate the structure and patterns of DOM and microbial communities in six lakes. The results showed a strong correlation between molecular-level DOM diversity and the diversity of microbial communities, indicating a dynamic feedback mechanism. The study also found that deterministic assembly processes governed DOM composition, while microbial community composition was highly variable across lakes with different environmental conditions. Overall, understanding the coupling between DOM and microbial communities is important for predicting future lake ecology and function.
Article
Environmental Sciences
Changsheng Jin, Zhongwu Li, Andrew S. Hursthouse, Xiang Ding, Mi Zhou, Jia Chen, Bolin Li
Summary: In sediment environments, Mn minerals have strong affinities for DOM and can regulate its constituents and reactivity through fractionation. However, the effects of DOM fractionation by Mn minerals on contaminant behaviors are still unclear.
ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY
(2023)
Article
Limnology
Beatriz Ferreira Araujo, Holger Hintelmann, Brian Dimock, Rodrigo de Lima Sobrinho, Marcelo Correa Bernardes, Marcelo Gomes de Almeida, Alex Krusche, Thiago Pessanha Rangel, Fabiano Thompson, Carlos Eduardo de Rezende
LIMNOLOGY AND OCEANOGRAPHY
(2018)
Article
Geochemistry & Geophysics
Liugen Zheng, Ruoyu Sun, Holger Hintelmann, Jianming Zhu, Ruwei Wang, Jeroen E. Sonke
Article
Multidisciplinary Sciences
Daniel C. Rearick, Lena Telgmann, Holger Hintelmann, Paul C. Frost, Marguerite A. Xenopoulos
Article
Engineering, Environmental
Fei Dang, Yuan-Zhen Chen, Ying-Nan Huang, Holger Hintelmann, You-Bin Si, Dong-Mei Zhou
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2019)
Article
Environmental Sciences
Maria Teresa Cabrita, Bernardo Duarte, Rute Cesario, Ricardo Mendes, Holger Hintelmann, Kevin Eckey, Brian Dimock, Isabel Cacador, Joao Canario
SCIENCE OF THE TOTAL ENVIRONMENT
(2019)
Article
Environmental Sciences
Marko Strok, Pascale Anabelle Baya, Doerthe Dietrich, Brian Dimock, Holger Hintelmann
SCIENCE OF THE TOTAL ENVIRONMENT
(2019)
Article
Engineering, Environmental
Wenli Tang, Holger Hintelmann, Baohua Gu, Xinbin Feng, Yurong Liu, Yuxi Gao, Jiating Zhao, Huike Zhu, Pei Lei, Huan Zhong
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2019)
Article
Multidisciplinary Sciences
Nives Ogrinc, Holger Hintelmann, Joze Kotnik, Milena Horvatl, Nicola Pirrone
SCIENTIFIC REPORTS
(2019)
Article
Environmental Sciences
Pablo A. Perez, Holger Hintelmann, Gabriela Lobos, Manuel A. Bravo
Article
Chemistry, Multidisciplinary
Min Li, Hai-Long Liu, Fei Dang, Holger Hintelmann, Bin Yin, Dongmei Zhou
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2020)
Article
Environmental Sciences
Anna K. Karjalainen, Johanna Salmelin, Brian Dimock, Holger Hintelmann
WATER AIR AND SOIL POLLUTION
(2020)
Article
Environmental Sciences
Beatriz Bento, Holger Hintelmann, Margarida Correia dos Santos, Rute Cesario, Joao Canario
Summary: Research found that Deception Island in Antarctica is an active volcano, with volcanic eruptions being one of the reasons for high mercury concentrations. Higher levels of total mercury and monomethylmercury were found in this ecosystem, with biotic methylation rates in water being significantly higher and abiotic methylation playing an important role.
MARINE POLLUTION BULLETIN
(2021)
Article
Multidisciplinary Sciences
Paul J. Blanchfield, John W. M. Rudd, Lee E. Hrenchuk, Marc Amyot, Christopher L. Babiarz, Ken G. Beaty, R. A. Drew Bodaly, Brian A. Branfireun, Cynthia C. Gilmour, Jennifer A. Graydon, Britt D. Hall, Reed C. Harris, Andrew Heyes, Holger Hintelmann, James P. Hurley, Carol A. Kelly, David P. Krabbenhoft, Steve E. Lindberg, Robert P. Mason, Michael J. Paterson, Cheryl L. Podemski, Ken A. Sandilands, George R. Southworth, Vincent L. St Louis, Lori S. Tate, Michael T. Tate
Summary: The 15-year experiment conducted to reduce fish MeHg concentrations by decreasing Hg additions to a boreal lake and its watershed demonstrated that any reduction in Hg loadings to lakes, whether from direct deposition or runoff, will have immediate benefits to fish consumers.
Article
Environmental Sciences
Audrey Campeau, Karin Eklof, Anne L. Soerensen, Staffan Akerblom, Shengliu Yuan, Holger Hintelmann, Magdalena Bieroza, Stephan Kohler, Christian Zdanowicz
Summary: The Arctic environment contains a complex mosaic of mercury and carbon reservoirs, some of which are destabilizing rapidly due to climate warming. Measurements and analyses of mercury and carbon concentrations in river water revealed major differences in the sources of particulate and dissolved riverine mercury, despite a common positive association with older material.
SCIENCE OF THE TOTAL ENVIRONMENT
(2022)
Article
Environmental Sciences
Neusa Figueiredo, Maria Luisa Serralheiro, Joao Canario, Aida Duarte, Holger Hintelmann, Cristina Carvalho
INTERNATIONAL JOURNAL OF ENVIRONMENTAL RESEARCH AND PUBLIC HEALTH
(2018)
Review
Environmental Sciences
Attila Csaba Kondor, Anna Viktoria Vancsik, Laszlo Bauer, Lili Szabo, Zoltan Szalai, Gergely Jakab, Gabor Maasz, Marta Pedrosa, Maria Jose Sampaio, Ana Rita Lado Ribeiro
Summary: This review provides a critical overview of research on the removal efficiency of priority substances and compounds of emerging concern through bank filtration, discussing influencing factors and future challenges. The findings show that the efficiency of bank filtration is influenced by multiple factors and varies for different substances.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Xinyan Wang, Shuai Zhang, Huihui Yan, Zhao Ma, Yunshan Zhang, Haining Luo, Xueli Yang
Summary: This study investigated the association between ambient PM2.5, O3 pollution, and ovarian reserve in reproductive-aged Chinese women. The results showed that increased exposure to PM2.5 and O3 was associated with decreased AMH levels, indicating reduced ovarian reserve. Notably, the effects of O3 exposure on ovarian reserve were different from those of PM2.5 exposure.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Tingting Ma, Yanjuan Ding, Fengjiao Xu, Chen Zhang, Min Zhou, Ya Tang, Yanrong Chen, Yating Wen, Rufei Chen, Bin Tang, Shigui Wang
Summary: The dragonfly species Orthetrum albistylum can accumulate heavy metals, and its heat shock protein genes have the potential to serve as biomarkers for monitoring environmental pollutants.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Naoto Ishiwaka, Koya Hashimoto, Masayoshi K. Hiraiwa, Francisco Sanchez-Bayo, Taku Kadoya, Daisuke Hayasaka
Summary: Systemic insecticides and rising temperatures have combined effects on the abundance of Odonata nymphs in paddy fields. The standalone effect of insecticide exposure decreased the Odonata community, while nymphs decreased synergistically with temperature rise in paddy water. However, the impacts of each stressor alone varied among species.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Marco Vecchiato, Carlo Barbante, Elena Barbaro, Francois Burgay, Warren R. L. Cairns, Alice Callegaro, David Cappelletti, Federico Dallo, Marianna D'Amico, Matteo Feltracco, Jean-Charles Gallet, Andrea Gambaro, Catherine Larose, Niccolo Maffezzoli, Mauro Mazzola, Ivan Sartorato, Federico Scoto, Clara Turetta, Massimiliano Varde, Zhiyong Xie, Andrea Spolaor
Summary: The Arctic region is facing contamination from long-range pollution and local human activities. Polycyclic Aromatic Hydrocarbons (PAHs) are used as environmental indicators for emission, transport, and deposition processes. Research conducted in the Arctic surface snow in Ny-Ålesund, Svalbard from October 2018 to May 2019 shows that long-range inputs of PAHs mainly occur in winter, while the most abundant analyte retene exhibits opposite seasonal trends.
ENVIRONMENTAL POLLUTION
(2024)
Review
Environmental Sciences
Maoshui Zhuo, Zhijie Chen, Xiaoqing Liu, Wei Wei, Yansong Shen, Bing-Jie Ni
Summary: This paper discusses the application of three catalytic processes (photocatalysis, electrocatalysis, and biocatalysis) in the management of microplastic pollution, and introduces the efficiency and catalytic mechanisms of different catalysts. It also proposes the development prospects for sustainable management of microplastic pollution.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Shiyu Chen, Zhenzhen Shi, Qiang Zhang
Summary: In this study, a human physiologically based pharmacokinetic (PBPK) model of diethyl phthalate (DEP) was developed to assess its toxicity. The model considers the distribution and metabolism of DEP and its active metabolite monoethyl phthalate (MEP) in different tissue compartments. Sensitivity analysis and Bayesian Markov chain Monte Carlo (MCMC) simulations were performed to evaluate the uncertainty and variability of the model parameters. The results suggest that dermal absorption is an important route of exposure to DEP in the environment.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Bangguo Wang, Lijing Wang, Wenxi Cen, Tao Lyu, Peter Jarvis, Yang Zhang, Yuanxun Zhang, Yinghui Han, Lei Wang, Gang Pan, Kaili Zhang, Wei Fan
Summary: This study investigates the feasibility and mechanisms of a chemical-free nanobubble-based AOP for treating organic micropollutants in water. The results show that the oxygen nanobubble AOP has a significantly higher removal efficiency compared to air and nitrogen nanobubbles. The treatment performance is not affected by pH and the presence of ions. Higher initial concentrations of the micropollutant lead to slower treatment processes, but similar removal performance is achieved in the end. The presence of organic matter reduces the removal rate of the micropollutant. The results have practical feasibility for water and wastewater treatment.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Yingmei Huang, Jicai Yi, Yao Huang, Songxiong Zhong, Bin Zhao, Jing Zhou, Yuxuan Wang, Yiwen Zhu, Yanhong Du, Fangbai Li
Summary: This study investigates the impact of biochar on methylmercury (MeHg) accumulation in rice. The results show that biochar reduces MeHg levels in paddy soils by decreasing bioavailable Hg and microbial Hg methylation. Additionally, biochar decreases the uptake and translocation of MeHg in rice plants, resulting in a reduction of MeHg accumulation in rice grains.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Nengde Zeng, Fei Huang, Jiani Du, Chenghao Huang, Qian Yang, Xinhua Zhan, Baoshan Xing
Summary: This study investigates the protein targets and protein-ligand interactions related to PAH contamination in crop xylem sap using computational tools. The results show that phenanthrene has a more pronounced effect on the xylem sap proteins of maize and wheat, with maize DEPs associated with lipid biosynthesis and wheat DEPs exhibiting an increase in ABC transporters. This study provides insights into the regulation and movement of PAHs within plant xylem.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Xinwei Chen, Hao Ma, Run Wang, Man Wang, Binbin Zhu, Yanqing Cong, Xiayue Zhu, Guoqin Wang, Yi Zhang
Summary: Co3O4/TiO2-NRs electrodes with excellent photoresponse were prepared via plasma-assisted modification of Co3O4 on TiO2. The combination of Co3O4 and TiO2 improved the light utilization efficiency and showed potential for degradation of pollutants.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Wenjing Ji, Liying Song, Jing Wang, Hongqing Song
Summary: This study conducted a life-cycle assessment to examine the correlation between natural gas consumption and carbon emissions in different end uses in China. The results showed that both natural gas consumption and life-cycle carbon emissions have been increasing since 2017. Significant variations in NG life-cycle carbon emissions were found across different provinces and sectors, highlighting the need for targeted efforts to reduce carbon emissions.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Youyi Chen, Boxuan Zhang, Pojun Zhang, Guogui Shi, Hao Liang, Wu Cai, Jingyu Gao, Sumin Zhuang, Kaiyin Luo, Jiaqi Zhu, Chaoxiang Chen, Kunyu Ma, Jinrong Chen, Chun Hu, Xueci Xing
Summary: The synergistic effects of trace sulfadiazine and cast-iron corrosion scales on the formation of disinfection by-products in drinking water distribution systems were investigated. The presence of magnetite resulted in increased concentrations of DBPs due to the higher microbial activity and enhanced microbial extracellular electron transport pathway. The study highlights the importance of considering trace antibiotics pollution and corrosion scales in water sources for DBP control.
ENVIRONMENTAL POLLUTION
(2024)
Review
Environmental Sciences
Bishwa Raj Pokharel, Vijay Sheri, Manoj Kumar, Zhiyong Zhang, Baohong Zhang
Summary: This review summarizes the interactions, uptake, and transport of aluminum nanoparticles (Al-NPs) in plants, highlighting their negative effects on plant growth and development, as well as their potential to alter plant defense systems and gene expression.
ENVIRONMENTAL POLLUTION
(2024)
Article
Environmental Sciences
Yonglu Wang, Fengsong Zhang, Xiaoyong Liao, Xiao Yang, Guixiang Zhang, Liyun Zhang, Chaojun Wei, Pengge Shi, Jiongxin Wen, Xiaorong Ju, Can Xu, Yang Liu, Ying Lan
Summary: This study aims to explore the effects of thiencarbazone-methyl center dot isoxaflutole on soil microflora and the potential mitigation mechanisms to bacterial communities. It was found that increasing the application of thiencarbazone-methyl center dot isoxaflutole resulted in increased stress on soil bacterial community structure and diversity. Increasing soil pH was recognized as a key factor in improving the diversity and structure of soil microflora. Supplemental use of nitrapyrin or modified attapulgite can increase soil pH and improve bacterial diversity.
ENVIRONMENTAL POLLUTION
(2024)