Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 80, Issue 12, Pages 6350-6359Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.5b00784
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Funding
- National Natural Science Foundation of China [21372030]
- Program for Changjiang Scholars and Innovative Research Team in University
- Beijing Municipal Commission of Education
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A novel and efficient method for the highly enantioselective synthesis of chiral 4,5-dihydropyridazin-3-one derivatives has been developed based on the chiral N-heterocyclic carbene-catalyzed oxidative annulation between alpha,beta-unsaturated aldehydes and hydrazones. Meanwhile, the selective synthesis of either 4,5-dihydropyridazin-3-ones or pyridazin-3-one derivatives from the same reactants has been achieved by simply varying catalytic and reaction conditions.
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