Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 9, Issue 10, Pages 2736-2739Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201402510
Keywords
acyloxylation; CH activation; copper; site-selective; unactivated sp(3) carbons
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Funding
- Indiana University-Purdue University Indianapolis
- NSF-MRI award [CHE-0619254]
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The site-selective acyloxylation of aliphatic amides was achieved via a copper-promoted C(sp(3))H bond functionalization process directed by a bidentate ligand. The reaction showed a great preference for activating CH bonds of -methyl groups over those of -methyl and unactivated methylene groups.
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