Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 3, Pages 1125-1129Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201405360
Keywords
gas hydrates; host-guest chemistry; inclusion compounds; metal-organic frameworks; water
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Funding
- National Research Foundation Korea [2013-059738]
- Recovery/Production of Natural Gas Hydrate using Swapping Technique project (KIGAM-Gas Hydrate R&D Organization) - Korean government (MEST)
- Center for Hybrid Interface Materials (HIM) through the National Research Foundation of Korea (NRF) - Ministry of Science, ICT and Future Planning [2013M3A6B1078884, 2013-073298]
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Unusual CO2 storage in water-saturated MOFs was investigated by combining experiment and simulation. It was found that the micropores of HKUST-1 saturated with water provide an environment that is thermodynamically and kinetically favorable for CO2 capture, but not for N-2 and H-2 capture. We expect that this phenomenon have potential to be used for successful separation of CO2 from versatile flue streams and pre-combustion gas.
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