Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 54, Issue 10, Pages 3074-3078Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201410369
Keywords
antitumor agents; cascade reactions; natural products; total synthesis; trioxacarcins
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Funding
- Cancer Prevention & Research Institute of Texas (CPRIT)
- Welch Foundation
- Chongqing University
- Danish Agency for Science, Technology and Innovation (The Frants Alling Scholarship)
- Deutsche Akademie der Naturforscher Leopoldina
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An enantioselective total synthesis of trioxacarcin DC-45-A2 (1) featuring a novel Lewis acid-induced cascade rearrangement of epoxyketone 6 to forge the polyoxygenated 2,7-dioxabicyclo[2.2.1]heptane core of the molecule is described.
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