Journal
CHEMICAL COMMUNICATIONS
Volume 50, Issue 94, Pages 14797-14800Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc05895j
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Funding
- National Natural Sciences Foundation of China [21072027, 21172030, 21272034, 21202015]
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The first formal [3+2] cycloaddition using alpha-trifluoromethyl-(indol-3-yl)methanols as the trifluoromethylated C-3 1,3-dipoles for the construction of the five-membered carbocycle of 1-trifluoromethylated cyclopenta[b]indole alkaloids is described. An unprecedented step-wise dehydrative alkenylation of alpha-trifluoromethyl alcohols was revealed as the crucial transformation.
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