Journal
CHEMICAL COMMUNICATIONS
Volume 48, Issue 22, Pages 2764-2766Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc17709a
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Funding
- Shanghai Municipal Committee of Science and Technology [11JC1402600]
- National Basic Research Program of China (973) [2010CB833302]
- Fundamental Research Funds for the Central Universities
- National Natural Science Foundation of China [20902019, 20872162, 20672127, 20821002, 20732008, 20772030, 20702059]
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A novel axially chiral spiro-phosphine-catalyzed highly regio-, diastereo- and enantioselective [3 + 2] cycloaddition of alkylidene azlactones with various allenic esters has been developed, affording the corresponding functionalized spirocyclic products in moderate to excellent yields under mild conditions. These spirocyclic products as masked amino acids can be easily transformed into aspartic amino acid analogues.
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