Journal
CHEMICAL COMMUNICATIONS
Volume 46, Issue 29, Pages 5280-5282Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cc00481b
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Funding
- NSFC [20702032, 20872098]
- MOE [IRT0846]
- MOST [2010CB833200]
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A concise 8-step synthetic route toward ent-heliespirones A & C is described. This synthetic strategy features a highly diastereoselective palladium-catalyzed Michael addition to form 3,5-trans lactone and a final biomimetic intramolecular oxa-spirocyclization.
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