Journal
CATALYSIS COMMUNICATIONS
Volume 52, Issue -, Pages 22-25Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.catcom.2014.04.006
Keywords
Hydrodechlorination; 4-Chlorophenol; Magnetite; Rhodium
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Funding
- National Natural Science Foundation of China [21207109]
- Applied Basic Research Programs of Science and Technology Department of Sichuan Province [2014JY0107]
- Key Laboratory of Green Catalysis of Sichuan Institutes of High Education [LZJ1205]
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Amine-functionalized magnetite nanoparticles synthesized from a facile one-pot template-free method were applied as carriers for depositing Rh nanoparticles using RhCl3 as the precursor. The as-prepared nanocomposites were applied for the hydrodechlorination of 4-chlorophenol at room temperature and atmospheric pressure. A complete conversion of 4-CP was obtained with the generation of phenol, cyclohexanone as the main products. The excellent catalytic activity, stability and recyclability of the catalyst were probably contributed to the functionalities of amine groups for stabilizing the Rh nanoparticles and the magnetic effect of Fe3O4 support during consecutive recycling of the catalyst. (C) 2014 Elsevier B.V. All rights reserved.
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