Article
Chemistry, Multidisciplinary
Alejandro Lopez-Moreno, Susana Ibanez, Sara Moreno-Da Silva, Luisa Ruiz-Gonzalez, Natalia Martin Sabanes, Eduardo Peris, Emilio M. Perez
Summary: Mechanically interlocked derivatives of carbon nanotubes (MINTs) are interesting and stable nanotube products. This study explores the encapsulation of single-walled carbon nanotubes within a palladium-based metallosquare, revealing the sensitivity of MINT formation to structural variations of the metallo-assemblies. The study also demonstrates the potential application expansion of MINTs through supramolecular coordination complexes.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Chemistry, Multidisciplinary
Rong Zhang, Xiujun Wang, Zhen Zhang, Wendi Zhang, Junqi Lai, Siqi Zhu, Yunfei Li, Yong Zhang, Kecheng Cao, Song Qiu, Qi Chen, Lixing Kang, Qingwen Li
Summary: In this study, CuI@SWCNT networks were successfully prepared by filling CuI into SWCNTs. CuI@SWCNT networks exhibited good stability and significantly improved current carrying capacity and conductivity compared to SWCNTs. By regulating the Fermi level position of SWCNTs, CuI guest molecules increased carrier concentration, achieving high conductivity and high current carrying capacity. This study offers ideas and solutions for the regulation of high-performance carbon tube networks, which hold great promise for future applications in carbon-based electronic devices.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Materials Science, Ceramics
R. Fernandez-Loyola, M. Muthuvel, A. B. Hernandez-Maldonado, J. A. Menchaca-Rivera, J. F. Perez-Robles, O. Solorza-Feria, G. G. Botte
Summary: A new nanocomposite material involving multi-walled carbon nanotubes (MWCNTs) was synthesized using the traditional chemical vapor deposition (CVD) method. The morphological and structural characterization, as well as the electrochemical evaluation, indicate the potential application of these nanocomposites as efficient electrocatalysts.
CERAMICS INTERNATIONAL
(2021)
Article
Chemistry, Physical
Thiago A. Moura, Wellington Q. Neves, Rafael S. Alencar, Y. A. Kim, M. Endo, Thiago L. Vasconcelos, Deyse G. Costa, Graziani Candiotto, Rodrigo B. Capaz, Paulo T. Araujo, Antonio G. Souza Filho, Alexandre R. Paschoal
Summary: The unique electronic and vibrational properties of linear carbon chains (LCCs) have attracted attention recently. Raman spectroscopy has been widely used to identify LCC and study its properties. This study investigates the optical resonance window of LCCs encapsulated by multi-walled carbon nanotubes (MWCNTs) and a Raman signature assigned to the LCC's longitudinal acoustic phonon mode. First-principles calculations support the conclusions.
Article
Chemistry, Multidisciplinary
Quan Sha, Dongwei Cao, Jiaxin Wang, Hanbin Hu, Jiaxin Li, Wei Chen, Lei He, Graham N. Newton, Yu-Fei Song
Summary: Host-guest interaction can alter the properties of composite materials. This study reveals the effect of the host on the electronic structure of guest molecules. Encapsulating polyoxometalates (POMs) in single-walled carbon nanotubes (SWNT) leads to structural changes and electron reconfiguration in POMs, which enhances charge density and accelerates electron and ion transport. This improves the electrochemical performance for sodium ion storage.
CHEMISTRY-A EUROPEAN JOURNAL
(2022)
Article
Chemistry, Multidisciplinary
D. Rybkovskiy, V. O. Koroteev, A. Impellizzeri, A. A. Vorfolomeeva, E. Yu Gerasimov, A. Okotrub, A. Chuvilin, L. G. Bulusheva, C. P. Ewels
Summary: The missing 1D-phosphorus allotrope, red phosphorus chains, is identified to form inside tip-opened single-walled carbon nanotubes. Comprehensive experimental and theoretical studies reveal the presence of linear P8]P2 chains and fibrous cross-linked double-chains of red phosphorus in intermediate diameter cavities. These findings provide a comprehensive understanding of the diameter dependence of confined 1D-phosphorus allotropes.
Article
Chemistry, Multidisciplinary
Anna A. Vorfolomeeva, Svetlana G. Stolyarova, Igor P. Asanov, Elena V. Shlyakhova, Pavel E. Plyusnin, Evgeny A. Maksimovskiy, Evgeny Yu. Gerasimov, Andrey L. Chuvilin, Alexander V. Okotrub, Lyubov G. Bulusheva
Summary: This study compares the electrochemical performance of commercial single-walled carbon nanotubes (SWCNTs) with red phosphorus deposited on the outer surface and/or encapsulated in internal channels for lithium-ion batteries. Encapsulated phosphorus demonstrates higher reaction rates and slight loss of initial capacity compared to external phosphorus. The support of SWCNTs and tubular space contribute to the stable operation and formation of chain phosphorus structures.
Article
Pharmacology & Pharmacy
Cecilia Espindola, Alejandro Javier Correa, Manuel Lopez-Lopez, Pilar Lopez-Cornejo, Eva Bernal, Jose Antonio Lebron, Francisco Jose Ostos, Mohammed Rafii-El-Idrissi Benhnia, Maria Luisa Moya
Summary: Research on flavonoids has grown significantly since their first therapeutic evidence in 1937. They have shown effective antioxidant activity in a wide range of human diseases. However, their applications have been limited due to their low solubility, poor absorption, and rapid metabolism. Encapsulating flavonoids in nanocarriers, such as carbon nanotubes, can improve their oral absorption and stability. This study investigated the encapsulation of 7-hydroxyflavone (7-HF) in different types of carbon nanotubes and studied its release at different pHs, simulating biological barriers.
Article
Chemistry, Physical
Gabrielle B. Novais, Mariana A. Dias, Adilson A. M. Santana, Thigna C. Batista, Maria N. Marques, Carlisson R. Melo, Ricardo L. C. Albuquerque Junior, Margarete Z. Gomes, Patricia Severino, Eliana B. Souto, Juliana C. Cardoso
Summary: This work focuses on the functionalization of SWCNTs and MWCNTs with two selected isoflavones and compares their physicochemical properties. Acidic treatment improved the dispersibility of both types of nanotubes, but SWCNTs still remained aggregated. However, MWCNTs showed increased dispersibility after acidic treatment. The functionalization with isoflavones was confirmed by improved dispersibility of the nanotubes.
JOURNAL OF MOLECULAR STRUCTURE
(2023)
Article
Materials Science, Multidisciplinary
Valery Ya. Rudyak, Gennady R. Dashapilov, Andrey V. Minakov, Maxim I. Pryazhnikov
Summary: The purpose of this study is to analyze the viscosity and rheology of nanofluids containing single-walled and multi-walled carbon nanotubes and compare their findings. The experiments involved a variety of nanofluids with the same base fluids and weight concentrations of CNTs and surfactants. The results showed that nanofluids with single-walled carbon nanotubes exhibited significantly higher viscosity than those with multi-walled carbon nanotubes. Most of the studied nanofluids exhibited pseudo-plastic or viscoplastic behavior, despite the Newtonian nature of the base fluids. Correlations describing the rheology of all investigated nanofluids were provided, along with the observation that the viscosity of nanofluids increased with a decrease in the average hydrodynamic size of nanotubes. The microrheology of these nanofluids was also studied, revealing the dependence of their elastic modulus on the concentration of CNTs.
DIAMOND AND RELATED MATERIALS
(2023)
Review
Energy & Fuels
Jin-Myung Choi, Jiye Han, Tushar Rane, Soyeon Kim, Ick Soo Kim, Il Jeon
Summary: This review discusses the fundamentals of utilizing SWCNTs in PSCs, including their characteristics as electron-transporting layer, hole-transporting layer, photoactive layer, and interfacial materials. It also presents strategies to improve PSCs performance through defect control and enhancement of electrical and morphological properties.
JOURNAL OF PHYSICS-ENERGY
(2022)
Article
Chemistry, Multidisciplinary
Silvia Aidee Solorio-Rodriguez, Andrew Williams, Sarah Sos Poulsen, Kristina Bram Knudsen, Keld Alstrup Jensen, Per Axel Clausen, Pernille Hogh Danielsen, Hakan Wallin, Ulla Vogel, Sabina Halappanavar
Summary: This study aimed to determine the influence of single or multi-walled structures and surface functionalization on pulmonary toxicity of carbon nanotubes (CNTs) and to identify the underlying mechanisms. Mice were exposed to different doses of SWCNTs or MWCNTs, and inflammation and DNA damage were assessed. Transcriptomics analysis showed similar responses across all CNTs, with inflammation, cellular stress, metabolism, and DNA damage responses being affected. One pristine SWCNT was found to be the most potent and potentially fibrogenic, warranting further toxicity testing.
Article
Chemistry, Physical
Saeed Ahmad, Qiang Zhang, Er-Xiong Ding, Hua Jiang, Esko I. Kauppinen
Summary: Floating-catalyst CVD (FCCVD) is a highly promising technique for scalable synthesis of single-walled carbon nanotubes (SWCNTs), and the number concentration (NC) of catalyst particles is a crucial parameter in determining the yield of SWCNTs. In this study, a novel FCCVD technique was employed to investigate the effects of catalyst NC on SWCNTs synthesis. Experimental results showed that under carefully chosen reaction conditions, a single catalyst particle can grow multiple SWCNTs.
CHEMICAL PHYSICS LETTERS
(2023)
Article
Polymer Science
Maria-Malvina Stathouraki, Christos Pantazidis, Emmanouil Mygiakis, Apostolos Avgeropoulos, Georgios Sakellariou
Summary: A facile method for surface functionalization of single-walled carbon nanotubes with end-capped polystyrene chains was developed, involving a thermal cycloaddition reaction and anionic polymerization. Successful synthesis and quantitative end-capping reaction were confirmed by various analytical methods. The presence of thin polystyrene film on the CNT surface was directly evidenced by TEM and AFM.
Article
Chemistry, Analytical
Mohammad Rostampour, Brian Bailey, Cody Autrey, Karla Ferrer, Brooke Vantoorenburg, Parth K. Patel, Percy Calvo-Marzal, Karin Y. Chumbimuni-Torres
Summary: The study investigated the effect of different solvents on the reproducibility of ISEs and proposed a method to integrate semiconducting/transducer polymer with single-walled carbon nanotubes into paper-based ISE substrates in a single step. PBISEs for potassium and sodium ions were developed with excellent sensor performance and reproducibility.
ANALYTICAL CHEMISTRY
(2021)
Article
Materials Science, Multidisciplinary
F. Regan Maria Sundar Raj, N. Victor Jaya, G. Boopathi, D. Kalpana, A. Pandurangan
MATERIALS CHEMISTRY AND PHYSICS
(2020)
Article
Materials Science, Multidisciplinary
D. Johnsirani, A. Pandurangan
DIAMOND AND RELATED MATERIALS
(2020)
Article
Chemistry, Multidisciplinary
Adithya Lenin, Pandurangan Arumugam, Revathi Shanmugham, Arumugam Sonachalam, Sivaprakash Paramasivam, Aruna Prakasa Rao, Ganesan Singaravelu, Ramani Venkatesan
Article
Chemistry, Organic
Koppada Masthan Raju, Ravi Kumar Cheedarala, Arumugam Pandurangan
CURRENT ORGANIC CHEMISTRY
(2020)
Article
Chemistry, Analytical
P. Sivaprakash, K. Ashok Kumar, S. Muthukumaran, A. Pandurangan, Ambesh Dixit, S. Arumugam
JOURNAL OF ELECTROANALYTICAL CHEMISTRY
(2020)
Article
Engineering, Electrical & Electronic
Karthikeyan Gunasekaran Govindarasu, Boopathi Ganesan, Ramani Venkatesan, Pandurangan Arumugam
Summary: Doping phosphorous into graphitic hollow carbon spheres grown over Fe-KIT-6 can greatly enhance the capacitive performance, with the optimized sample showing high specific capacitance of 321 F g(-1) and excellent cycling stability. The P-GHCS-800 supercapacitor device exhibits remarkable cyclic stability, with a relatively high energy density of 10.83 Wh kg(-1) and a power density of 222.78 W kg(-1), showcasing potential realistic applications.
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
(2021)
Article
Chemistry, Applied
Shanmugam Manimaran, Kathavarayan Subramanian, Roman Tschentscher, Arumugam Pandurangan
Summary: The 3D cubic cage-like Im3m mesoporous SBA-16 was successfully synthesized and used for the epoxidation of styrene. The addition of different ratios of manganese nitrate and ammonium tungsten oxide significantly affected the selectivity of the reaction, with MnWO4 (3 wt%)/SBA-16 showing the highest selectivity.
JOURNAL OF POROUS MATERIALS
(2022)
Article
Engineering, Mechanical
Adithya Lenin, Pandurangan Arumugam, Aruna Prakasa Rao, Angayarkanny Subramanian
Summary: This research reports the fabrication of a functional composite material that simultaneously exhibits hydrophobicity and water droplet adhesion. By drop casting, Boron Nitride Nanotubes (BNNTs) were combined with Polydimethylsiloxane (PDMS) to create a petal wetting biomimetic nanocomposite. The nanotubes were synthesized through chemical vapor deposition and characterized by various techniques. The resulting nanocomposites displayed a characteristic trait of high contact angle hysteresis.
SURFACE TOPOGRAPHY-METROLOGY AND PROPERTIES
(2022)
Article
Chemistry, Applied
R. Ragavan, A. Pandurangan
Summary: A series of heteroatom doped ordered mesoporous carbons (HOMCs) were synthesized using chemical vapor deposition nanocasting (CVD nanocasting) with SBA-15 as the template. The properties of the HOMCs were characterized, and the NPOMC sample showed high specific capacitance and good cyclic stability and columbic efficiency in the fabricated device.
MICROPOROUS AND MESOPOROUS MATERIALS
(2022)
Article
Engineering, Electrical & Electronic
Johnsirani Devarajan, Pandurangan Arumugam
Summary: This paper reports a sustainable and cost-effective method to synthesize boron-doped activated biomass-derived carbon from the stems of Prosopis juliflora for supercapacitor applications. The material showed high specific capacitance and energy efficiency, and exhibited stable performance in a supercapacitor device.
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
(2022)
Article
Chemistry, Applied
Siva Kannan, Pandurangan Arumugam, Gopalakrishnan Govindasamy
Summary: This study focuses on the production of sustainable aviation fuels through the hydrodeoxygenation of lignin derivatives. The use of mono and bi-functional catalysts supported on SBA-15 and carbons was evaluated, with the bi-functional catalysts showing higher conversion and selectivity for propyl benzene and propyl cyclohexane. The optimum temperature for the HDO reaction was found to be 400 degrees C for the bi-functional catalysts.
JOURNAL OF POROUS MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Johnsirani Devarajan, Pandurangan Arumugam
Summary: Nitrogen and phosphorous dual-doped carbon nanotubes (N,P/CNT) were synthesized using iron-loaded mesoporous SBA-15 support in a single-step CVD process. The N,P/CNT demonstrated a maximum specific capacitance of 358.2 F/g at 0.5 A/g current density in three-electrode investigations. As a symmetric supercapacitor device, it delivered a specific capacitance of 108.6 F/g at 0.5 A/g with energy density of 15 Wh/kg and power density of 250 W/kg, exhibiting an energy efficiency of 92.3%. Over 5000 charge-discharge cycles, the capacitance retention and coulombic efficiency were calculated to be 96.2% and 90.6%, respectively.
Article
Chemistry, Multidisciplinary
N. S. Palani, N. S. Kavitha, K. S. Venkatesh, K. Ashok Kumar, M. Senthilkumar, A. Pandurangan, R. Ilangovan
Summary: Two-dimensional RuO2 nanoparticle-decorated V2O5 nanoflakes were successfully synthesized by a solvothermal method, showing high charge-discharge capacity and cyclic retention. The RuO2-decorated V2O5 nanocomposite exhibited a significantly higher specific capacitance in a three-electrode system compared to pure V2O5 nanosheets, with an energy density and power density surpassing previously reported V2O5 nanostructured asymmetric supercapacitors.
NEW JOURNAL OF CHEMISTRY
(2021)
Article
Chemistry, Multidisciplinary
P. Muthu Pandian, A. Pandurangan
Summary: The article introduces the synthesis of boron and nitrogen co-doped reduced graphene material (BNUG) and its application in solid-state supercapacitors. BNUG exhibits high specific capacitance and cycling stability, and the fabricated supercapacitors show high energy density and efficiency in different electrolytes.
NEW JOURNAL OF CHEMISTRY
(2021)
Article
Chemistry, Multidisciplinary
Janakiraman Babu, Shanmugam Ganesan, Kaliamurthy Ashok Kumar, Masiyappan Karuppusamy, Arumugam Pandurangan, Perumal Rajakumar
NEW JOURNAL OF CHEMISTRY
(2019)
Article
Chemistry, Physical
Jie Sheng, Jingshan He, Dun Ma, Yuanbo Wang, Wu Shao, Tian Ding, Ronghao Cen, Jingwen He, Zhihao Deng, Wenjun Wu
Summary: This study presents an innovative approach to improve the photovoltaic conversion characteristics and stability of perovskite solar cells through carbon electrode interface modification. By in-situ polymerization and carbonization on the surface of nano-graphite, a dendritic structure carbon electrode is formed, reducing the work function and aligning the energy levels with perovskite. This leads to improved charge and hole collection efficiency, resulting in increased photovoltaic conversion efficiency. Furthermore, the modified carbon electrode-based perovskite solar cells exhibit exceptional stability, maintaining high efficiency even without encapsulation.
Article
Chemistry, Physical
Guodong Shi, Jian Song, Xiaoxiao Tian, Tongtong Liu, Zhanjun Wu
Summary: This study demonstrates the improvement of mechanical properties and reduction of coefficient of thermal expansion (CTE) in graphene oxide (GO)/epoxy (EP) nanocomposites by enhancing the interface between GO and EP through functionalization and incorporating rigid-flexible interphases. The results reveal that the SiO2-PEA-GO hybrid exhibits better strengthening and toughening effects, as well as lower CTE, compared to the PEA-GO hybrid due to the presence of rigid-flexible interfaces with higher bonding strength and better energy dissipation mechanisms. Additionally, the nanocomposites with longer polyetheramine (PEA) molecules in the rigid-flexible interphases demonstrate higher strength and toughness, while maintaining a lower CTE. This work provides a promising strategy for constructing adjustable flexible-rigid interfacial structures and offers potential in developing GO/EP nanocomposites with high mechanical properties and low CTE.
Article
Chemistry, Physical
Rafal Janus, Sebastian Jarczewski, Jacek Jagiello, Piotr Natkanski, Mariusz Wadrzyk, Marek Lewandowski, Marek Michalik, Piotr Kustrowski
Summary: In this study, a facile procedure for the synthesis of CMK-1 and CMK-2 carbon replicas was developed. The method utilizes basic laboratory equipment and a renewable carbon source, and operates under mild conditions. The resulting carbon mesostructures exhibit exquisite replication fidelity and structural homogeneity, making them suitable for applications in various fields.
Article
Chemistry, Physical
Anqi Wang, Connor J. MacRobbie, Alex Baranovsky, Jean-Pierre Hickey, John Z. Wen
Summary: In this study, a novel polymer-free nanothermite aerogel with a wide range of nanoparticle loading was fabricated via a new additive manufacturing process. The SEM images showed a unique porous structure formed by extra thin rGO sheets, wrapping individual nanothermite clusters. The DSC-TGA results and high-speed combustion videos confirmed the enhanced energetic performance of the printed specimen.
Article
Chemistry, Physical
Wanze Wu, Misheng Zhao, Shiwei Miao, Xiaoyan Li, Yongzhong Wu, Xiao Gong, Hangxiang Wang
Summary: Superhydrophobic solar-driven interfacial evaporator is an energy-efficient technology for seawater desalination, which is easily fabricated using robust photothermal superhydrophobic coating and substrate. The created bifunctional coating on the melamine sponge substrate shows stable and highly efficient photothermal and superhydrophobic performance for seawater desalination. This superhydrophobic solar-driven interfacial evaporator is expected to have wide applications in seawater desalination.
Article
Chemistry, Physical
Zichen Xiang, Zhi Song, Tiansheng Wang, Menghang Feng, Yijing Zhao, Qitu Zhang, Yi Hou, Lixi Wang
Summary: This study presents a co-electrospinning synthesis strategy to fabricate lightweight and porous Co@C composite nanofibres with wideband microwave attenuation capacity. The addition of MOF-derived Co additives enhances the low-frequency absorption performance.
Article
Chemistry, Physical
J. Snow, C. Olson, E. Torres, K. Shirley, E. Cazalas
Summary: This study investigates the use of a perovskite-based graphene field effect transistor (P-GFET) device for X-ray detection. The sensitivity and responsivity of the device were found to be influenced by factors such as X-ray tube voltage, current, and source-drain voltage. Simulation experiments were conducted to determine the dose rate and energy incident on the device during irradiation.
Article
Chemistry, Physical
Zuzana Jankovska, Lenka Matejova, Jonas Tokarsky, Pavlina Peikertova, Milan Dopita, Karolina Gorzolkova, Dominika Habermannova, Michal Vastyl, Jakub Belik
Summary: This study provides new insights into microwave-assisted pyrolysis of scrap tyres, demonstrating that it can produce microporous carbon black with potential application in xylene adsorption. Compared to conventional pyrolysis, microwave pyrolysis requires less time and energy while maintaining similar adsorption capacity.
Article
Chemistry, Physical
Max Bommert, Bruno Schuler, Carlo A. Pignedoli, Roland Widmer, Oliver Groning
Summary: A detailed understanding of the interaction between molecules and two-dimensional materials is crucial for incorporating functional molecular films into next-generation 2D material-organic hybrid devices. This study compares the energy level alignment of different-sized fullerenes on a Moire superstructure and finds that C-84 fullerenes can be either neutral or negatively charged depending on slight variations of the electrostatic potential. This discovery suggests a new path to achieve ambipolar charge transfer without overcoming the electronic gap of fullerenes.
Article
Chemistry, Physical
Yuanjing Cheng, Xianxian Sun, Ye Yuan, Shuang Yang, Yuanhao Ning, Dan Wang, Weilong Yin, Yibin Li
Summary: The dual-structure aerogel (GS) consisting of flexible silica fibers and graphene honeycomb structures exhibits excellent resilience, flexibility, and reliability. It also shows remarkable wave absorbing performance, making it an ideal candidate for microwave absorption applications such as flexible electronics and aerospace.
Article
Chemistry, Physical
Shuyu Fan, Yinong Chen, Shu Xiao, Kejun Shi, Xinyu Meng, Songsheng Lin, Fenghua Su, Yifan Su, Paul K. Chu
Summary: Graphene coatings are promising solid lubrication materials due to their mechanical properties. This study presents a new method for in situ deposition of high-quality graphene coatings on hard substrates using NiCo solid solution and competitive reaction strategies. The graphene coating deposited on substrates with deep NiCo solid solution demonstrates superior low-friction and durability.
Article
Chemistry, Physical
Mengdi Wang, Sanyin Qu, Yanling Chen, Qin Yao, Lidong Chen
Summary: The improved thermoelectric properties of conducting polymers are achieved by selectively capturing single-walled carbon nanotubes (SWNTs) in a conducting polymer film, leading to increased carrier mobility and reduced thermal conductivity. The resulting composite film exhibits significantly higher electrical conductivity and lower thermal conductivity compared to films with a mixture of SWNTs. This work provides a convenient and efficient method to enhance the thermoelectric properties of conducting polymers.
Review
Chemistry, Physical
Heng Wei, Weihua Li, Kareem Bachagha
Summary: This article reviews the research progress of carbon nanotube-based microwave absorbing materials (MAMs) in recent years, covering the fundamental theory, design strategies, synthesis methods, and future development directions.
Article
Chemistry, Physical
Chenguang Shi, Junlong Huang, Zongheng Cen, Tan Yi, Shaohong Liu, Ruowen Fu
Summary: This study developed a high-performance Li metal host material, which achieved dendrite-free Li deposition with a low nucleation overpotential and high Coulombic efficiencies through the combination of Ti3C2-g-PV4P sheets and Ag nanoparticles. The full cells assembled with the Li@host anode and LiFePO4 cathode exhibited high discharge capacity and excellent cycling stability, demonstrating a perspective design for future energy storage devices.
Article
Chemistry, Physical
Tomotaro Mae, Kentaro Kaneko, Hiroki Sakurai, Suguru Noda
Summary: A new partial prelithiation method for SiO/C-CNT electrodes was developed, which showed reduced irreversible capacity and achieved high energy densities with good reversibility. The method allows for precise control of the degree of prelithiation and is applicable to various chemistries.