Journal
AUSTRALIAN JOURNAL OF CHEMISTRY
Volume 66, Issue 8, Pages 882-890Publisher
CSIRO PUBLISHING
DOI: 10.1071/CH13287
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Funding
- Australian Research Council
- Monash University
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Two strategies for the assembly of homochiral carbazolones have been investigated. The first exploited desymmetrisation of 1,3-cyclohexadione derivatives however this failed to deliver satisfactory outcomes. An orthogonal route exploiting palladium catalysed decarboxylative allylation of racemic carbazolone beta-ketoesters has been developed. Herein we report full details on the development of this reaction and clarify apparent discrepancies between our preliminary reports and those of Shao.
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