Journal
APPLIED CATALYSIS B-ENVIRONMENTAL
Volume 154, Issue -, Pages 316-328Publisher
ELSEVIER
DOI: 10.1016/j.apcatb.2014.02.032
Keywords
PdZn catalyst; Hydrogen production; Methanol steam reforming; ZnO; Oxygen vacancies
Funding
- European Union' Seventh Framework Programme
- Fuel Cells and Hydrogen Joint Technology Initiative [{303476} 10]
- FCT postdoctoral [PTDC/CTM/108454/2008]
- FEDER and POFC [PTDC/EQU-EQU/104217/2008]
- FCT [SFRH/BD/45890/2008]
- Fundação para a Ciência e a Tecnologia [SFRH/BD/45890/2008] Funding Source: FCT
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The influence of the calcination atmosphere of ZnO precursor (Zn-4(CO)(3)(OH)(6)center dot H2O) on the catalytic performance of a series of PdZn/ZnO catalysts was studied for production of H-2 via low temperature (180 C) direct methanol steam reforming (low temperature-MSR). The catalytic activity and selectivity of PdZn/ZnO were found to be strongly influenced by the calcination atmosphere of ZnO precursor and increased from oxidizing to reducing atmosphere, following the order (O-2 < air < N-2
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