Journal
APPLIED CATALYSIS A-GENERAL
Volume 445, Issue -, Pages 306-311Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.apcata.2012.08.040
Keywords
Heteropolyacid; Cross-linked copolymer; Ionic liquid; Epoxidation of alkenes; Heterogeneous catalysis
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Funding
- National Natural Science Foundation of China [21206052, 21136005]
- National Twelfth Five-Year Plan for Science Technology [2012BAD32B03]
- Fundamental Research Funds for the Central Universities [JUSRP111A04]
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A heteropolyanion-based cross-linked ionic copolymer was prepared by the anion-exchange of a newly task-specific designed amino-containing ionic copolymer with a Keggin heteropolyacid, and characterized by FT-IR, SEM, TG, XRD, UV-vis, ESR, H-1 NMR, and elemental analysis. Its catalytic activity was evaluated in the epoxidation of alkenes with aqueous H2O2. The resultant heteropolyanion-based ionic copolymer is revealed to be a highly efficient heterogeneous catalyst for epoxidation of alkenes with H2O2, adding the advantages of convenient recovery and steady reuse. (C) 2012 Elsevier B.V. All rights reserved.
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