Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 53, Issue 20, Pages 5161-5164Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201310136
Keywords
asymmetric catalysis; chemoselectivity; cyclization; furans; Lewis base
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Funding
- National University of Singapore [143-000-509-112]
- A*STAR-Public Sector Funding [143-000-536-305]
- GSK-EDB [143-000-564-592]
- A*STAR
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A facile, efficient, and highly diastereo- and enantioselective bromoetherification of diolefinic diols has been developed using an amino-thiocarbamate catalyst. Further manipulations of the bromoether products enabled entry into a new class of spirocycles which are distinctively lacking in the literature.
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