Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 357, Issue 1, Pages 41-45Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201400657
Keywords
aldehydes; asymmetric catalysis; hydroformylation; ligand design; P ligands; rhodium
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Funding
- DFG
- International Research Training Group [IRTG 1038]
- Krupp Foundation
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The synthesis of chiral bidentate bisphosphonite ligands based on the TADDOL motif from readily available starting materials has been developed. Taking advantage of the modular nature of the building blocks, a diverse ligand library has been prepared. Their catalytic potential has been evaluated in the asymmetric hydroformylation of styrene and derivatives. These catalysts showed high activity and provided the aldehydes in high enantiomeric purity.
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