4.6 Article

The Wintertime Covariation of CO2 and Criteria Pollutants in an Urban Valley of the Western United States

Journal

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
Volume 123, Issue 5, Pages 2684-2703

Publisher

AMER GEOPHYSICAL UNION
DOI: 10.1002/2017JD027917

Keywords

-

Funding

  1. Department of Energy (DOE) [DESC0010624]
  2. National Oceanic and Atmospheric Administration (NOAA) [NA140AR4310178]
  3. Utah Division of Air Quality
  4. Utah Department of Environmental Quality
  5. NSF [AGS 1723337]
  6. Center for High Performance Computing at the University of Utah
  7. National Science Foundation

Ask authors/readers for more resources

Numerous mountain valleys experience wintertime particulate pollution events, when persistent cold air pools (PCAPs) develop and inhibit atmospheric mixing, leading to the accumulation of pollutants. Here we examine the relationships between trace gases and criteria pollutants during winter in Utah's Salt Lake Valley, in an effort to better understand the roles of transport versus chemical processes during differing meteorological conditions as well as insights into how targeted reductions in greenhouse gases will impact local air quality in varying meteorological conditions. CO2 is a chemically inert gas that is coemitted during fossil fuel combustion with pollutants. Many of these coemitted pollutants are precursors that react chemically to form secondary particulate matter. Thus, CO2 can serve as a stable tracer and potentially help distinguish transport versus chemical influences on pollutants. During the winter of 2015-2016, we isolated enhancements in CO2 over baseline levels due to urban emissions (CO2ex). CO2ex was paired with similar excesses in other pollutant concentrations. These relationships were examined during different wintertime conditions and stages of pollution episodes: (a) Non-PCAP, (b) beginning, and (c) latter stages of an episode. We found that CO2ex is a good indicator of the presence of gaseous criteria pollutants and a reasonable indicator of PM2.5. Additionally, the relationships between CO2ex and criteria pollutants differ during different phases of PCAP events which provide insight into meteorological and transport processes. Lastly, we found a slight overestimation of CO:CO2 emission ratios and a considerable overestimation of NOx:CO2 by existing inventories for the Salt Lake Valley.

Authors

I am an author on this paper
Click your name to claim this paper and add it to your profile.

Reviews

Primary Rating

4.6
Not enough ratings

Secondary Ratings

Novelty
-
Significance
-
Scientific rigor
-
Rate this paper

Recommended

Article Engineering, Environmental

Community-Based Measurements Reveal Unseen Differences during Air Pollution Episodes

Kerry E. Kelly, Wei W. Xing, Tofigh Sayahi, Logan Mitchell, Tom Becnel, Pierre-Emmanuel Gaillardon, Miriah Meyer, Ross T. Whitaker

Summary: Short-term exposure to PM2.5 pollution is harmful to health, and low-cost sensor networks with Gaussian process models can accurately assess pollution gradients, revealing geographic differences.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

Article Astronomy & Astrophysics

An Interpolation Method to Reduce the Computational Time in the Stochastic Lagrangian Particle Dispersion Modeling of Spatially Dense XCO2 Retrievals

Dustin Roten, Dien Wu, Benjamin Fasoli, Tomohiro Oda, John C. Lin

Summary: The paper presents a novel algorithm that reduces the computational effort for atmospheric models by tracing the sources of a subset of OCO-3 measurements and inferring the rest, improving the efficiency of CO2 source analysis.

EARTH AND SPACE SCIENCE (2021)

Article Environmental Sciences

Expanding number of Western US urban centers face declining summertime air quality due to enhanced wildland fire activity

T. Y. Wilmot, A. G. Hallar, J. C. Lin, D. Mallia

Summary: The study reveals a connection between air quality trends in Western US urban centers during August and September from 2000 to 2019, with wildland fire activity. Spatially consistent trends in extreme levels of pollutants like PM2.5 and organic carbon were observed in the US Pacific Northwest in August. Furthermore, emerging trends were also identified in regions like the Pacific Northwest, western Montana, and Wyoming in September.

ENVIRONMENTAL RESEARCH LETTERS (2021)

Article Meteorology & Atmospheric Sciences

Improving CLM5.0 Biomass and Carbon Exchange Across the Western United States Using a Data Assimilation System

Brett Raczka, Timothy J. Hoar, Henrique F. Duarte, Andrew M. Fox, Jeffrey L. Anderson, David R. Bowling, John C. Lin

Summary: The Western United States is heavily influenced by natural lands that are crucial for carbon balance, water quality, and timber reserves, while also being susceptible to forest mortality from various factors. By adjusting simulations and incorporating water limitations, it is possible to improve carbon monitoring and understand the impact of water availability on carbon uptake through photosynthesis.

JOURNAL OF ADVANCES IN MODELING EARTH SYSTEMS (2021)

Article Environmental Sciences

Intra-city variability of fine particulate matter during COVID-19 lockdown: A case study from Park City, Utah

Daniel L. Mendoza, Tabitha M. Benney, Ryan Bares, Erik T. Crosman

Summary: Research tracked emissions patterns in a mid-sized, high-altitude city during the COVID-19 pandemic lockdown as a natural experiment to understand the effects of human behavior on air pollution. The results showed differences in emissions between commercial and residential areas during lockdown, with both experiencing a rebound post-lockdown.

ENVIRONMENTAL RESEARCH (2021)

Article Astronomy & Astrophysics

Mars Methane Sources in Northwestern Gale Crater Inferred From Back Trajectory Modeling

Y. Luo, M. A. Mischna, J. C. Lin, B. Fasoli, X. Cai, Y. L. Yung

Summary: Inverse Lagrangian modeling techniques were used to identify methane emission regions, revealing that the northwestern crater floor inside Gale crater has the strongest influence on methane detections, while the common upstream regions for all methane spikes outside Gale crater extend northwards.

EARTH AND SPACE SCIENCE (2021)

Article Environmental Sciences

The impact of the COVID-19 lockdown on greenhouse gases: a multi-city analysis of in situ atmospheric observations

V Monteiro, N. L. Miles, S. J. Richardson, J. Turnbull, A. Karion, J. Kim, L. Mitchell, J. C. Lin, J. C. M. Sargent, S. Wofsy, F. Vogel, K. J. Davis

Summary: We tested the capabilities of urban greenhouse gas measurement networks to detect abrupt changes in emissions, specifically during the COVID-19 lockdown in March 2020. The results showed a significant decrease in CO2 and CO emissions during the lockdown period, while changes in CH4 emissions were variable and not statistically significant. The study demonstrated the sensitivity of these tower networks to rapid changes in urban emissions, which were mainly influenced by reductions in traffic. Additionally, using measurements at different altitudes in urban observatories could improve the sensitivity of the observational network to both city-scale and local fluxes.

ENVIRONMENTAL RESEARCH COMMUNICATIONS (2022)

Article Multidisciplinary Sciences

A multi-city urban atmospheric greenhouse gas measurement data synthesis

Logan E. Mitchell, John C. Lin, Lucy R. Hutyra, David R. Bowling, Ronald C. Cohen, Kenneth J. Davis, Elizabeth DiGangi, Riley M. Duren, James R. Ehleringer, Clayton Fain, Matthias Falk, Abhinav Guha, Anna Karion, Ralph F. Keeling, Jooil Kim, Natasha L. Miles, Charles E. Miller, Sally Newman, Diane E. Pataki, Steve Prinzivalli, Xinrong Ren, Andrew Rice, Scott J. Richardson, Maryann Sargent, Britton B. Stephens, Jocelyn C. Turnbull, Kristal R. Verhulst, Felix Vogel, Ray F. Weiss, James Whetstone, Steven C. Wofsy

Summary: Urban regions are major contributors to greenhouse gas emissions. Increasing numbers of urban policymakers and stakeholders are taking action to reduce emissions and establish monitoring networks. However, the coordination among these efforts is limited, necessitating the integration of urban observations to enable comprehensive analyses and address scientific questions.

SCIENTIFIC DATA (2022)

Article Environmental Sciences

Wildfire activity is driving summertime air quality degradation across the western US: a model-based attribution to smoke source regions

Taylor Y. Wilmot, Derek Mallia, A. Gannet Hallar, John C. Lin

Summary: In recent decades, wildfire activity in western North America has increased, leading to degradation of air quality in urban centers. A study using atmospheric modeling and observational data links the worsening air quality to regional wildfire sources. The study finds that many urban centers in western US have experienced significant increases in extreme air quality episodes caused by wildfires, particularly in August and September. The results highlight the importance of regional forest management and understanding the connection between climate change, wildfire activity, and air quality.

ENVIRONMENTAL RESEARCH LETTERS (2022)

Article Meteorology & Atmospheric Sciences

Using Space-Based CO2 and NO2 Observations to Estimate Urban CO2 Emissions

Emily G. Yang, Eric A. Kort, Lesley E. Ott, Tomohiro Oda, John C. Lin

Summary: Since a majority of CO2 emissions from fossil fuels come from cities, it is important to use novel techniques to utilize satellite observations of CO2 and proxy species to control urban CO2. This study aims to establish the relationship between satellite observations of CO2 and the proxy species of NO2 and estimate CO2 emissions based on NO2 data. The method was tested in Buenos Aires, Melbourne, and Mexico City and proved to be viable throughout the year. This method provides a valuable observational constraint on urban CO2 emissions, with comparable monthly urban CO2 emissions estimates to inventory estimates.

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (2023)

Review Green & Sustainable Science & Technology

The History of Air Quality in Utah: A Narrative Review

Logan E. Mitchell, Chris A. B. Zajchowski

Summary: Utah has a rich history of air pollution, which has become a major concern for urban residents. The shift in fuel sources and scientific advances have changed the relationship between air pollution and the state's residents. Efforts have been made to raise public awareness and improve air quality through legislation and court rulings. The future of air quality in Utah presents both challenges and opportunities, and can serve as a case study for other urban areas grappling with similar issues.

SUSTAINABILITY (2022)

Article Geosciences, Multidisciplinary

A model for urban biogenic CO2 fluxes: Solar-Induced Fluorescence for Modeling Urban biogenic Fluxes (SMUrF v1)

Dien Wu, John C. Lin, Henrique F. Duarte, Vineet Yadav, Nicholas C. Parazoo, Tomohiro Oda, Eric A. Kort

Summary: The study highlights the challenges in estimating fossil fuel carbon dioxide emissions in urban areas due to biogenic carbon exchanges. By developing a simple model representation, it was possible to estimate ecosystem respiration and gross primary production across cities globally. Through advanced data analysis and modeling, the study provides valuable insights into the dynamics of biogenic carbon fluxes in urban environments.

GEOSCIENTIFIC MODEL DEVELOPMENT (2021)

Article Environmental Sciences

A mass-weighted isentropic coordinate for mapping chemical tracers and computing atmospheric inventories

Yuming Jin, Ralph F. Keeling, Eric J. Morgan, Eric Ray, Nicholas C. Parazoo, Britton B. Stephens

Summary: In this study, a new transformed isentropic coordinate M-theta e is introduced and effectively used to study the seasonal cycle of CO2, serving as an alternative to latitude in related research. The findings suggest that when calculating the CO2 seasonal cycle using M-theta e, the relationship with pressure is more stable and short-term variability is smaller compared to organizing by latitude and pressure.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

Article Environmental Sciences

The role of coarse aerosol particles as a sink of HNO3 in wintertime pollution events in the Salt Lake Valley

Amy Hrdina, Jennifer G. Murphy, Anna Gannet Hallar, John C. Lin, Alexander Moravek, Ryan Bares, Ross C. Petersen, Alessandro Franchin, Ann M. Middlebrook, Lexie Goldberger, Ben H. Lee, Munkh Baasandorj, Steven S. Brown

Summary: Wintertime ammonium nitrate pollution events in urban mountain basins are exacerbated by persistent cold-air pools, leading to the build-up of secondary pollutants like PM2.5 NH4NO3 causing severe haze. The study in Utah found that fine particulate matter was dominated by secondary NH4NO3 during pollution events, with excess NHx and a potential significant role of uptake by coarse-mode dust.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2021)

No Data Available