Article
Chemistry, Physical
Yeji Wang, Gege Yang, Fei Jiang, Tianpei Qiu, Qian Liu, Le Zhou, Chaofan Yang, Junjie Huang, Guoliang Dai
Summary: Porous imidazole polymerized ionic liquids (PILs-Im) have been used as anodes in lithium-ion batteries for the first time. They exhibit fast Li+ diffusion kinetics and numerous molecular pores, leading to high capacity and excellent lithium storage performance. In addition, PILs-Im show excellent cycling stability and rate capability, which can be attributed to the fast Li+ diffusion in the ionic skeleton, the filtration of liquid electrolyte through abundant micropores, and the strong endurance to the volume variation of Li+ insertion provided by the large cross-linking system.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Review
Chemistry, Multidisciplinary
Yaksh Popat, David Trudgeon, Caiping Zhang, Frank C. Walsh, Peter Connor, Xiaohong Li
Summary: This article reviews the application of carbon-based materials in bromine electrodes and discusses the research progress in performance and design of zinc-bromine, hydrogen-bromine, and polysulphide-bromine RFB systems.
Article
Chemistry, Physical
M. Candan Karaeyvaz, Busarnur Duman, Berker Ficicilar
Summary: Significantly active HCMS carbon catalysts were synthesized for hydrogen-bromine flow battery cathode electrode, showing promising peak power density compared to Pt-based catalysts and commercial carbons. The synthesis was achieved by template replication, producing carbons with different core/shell structures. The findings suggest the potential of HCMS1 carbon for grid-scale energy storage.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2021)
Article
Chemistry, Physical
R. Ronen, R. Gloukhovski, M. E. Suss
Summary: With the rapid growth of renewable sources in electricity generation, the use of grid-scale battery storage is increasing. Aqueous redox flow batteries have the potential to provide safe and scalable energy storage, but high costs have hindered commercialization. The development of a single-flow battery using a multiphase electrolyte offers a low-cost system, but suffers from low Coulombic efficiency. This study compares a theoretical battery model to experimental results, revealing key findings and the need to incorporate gravitational effects in future models.
JOURNAL OF POWER SOURCES
(2022)
Article
Electrochemistry
R. Ronen, A. D. Gat, M. Z. Bazant, M. E. Suss
Summary: Redox flow batteries, specifically membraneless batteries, are being explored for grid-scale energy storage. A mathematical model for membraneless electrochemical cells using single laminar flow between electrodes and different phases of reactants is presented. The study investigates slow and fast reactant transport between phases and shows that increasing nonaqueous phase volume fraction improves battery performance. The analytical approximations agree well with numerical solutions, establishing a useful theoretical framework for single-flow batteries with multiphase flow.
ELECTROCHIMICA ACTA
(2021)
Article
Chemistry, Physical
Michael Kuettinger, Raphaeel Riasse, Jakub Wlodarczyk, Peter Fischer, Jens Tuebke
Summary: This study proposes a solution to the problem of reduced membrane conductivity and high overvoltage in hydrogen bromine redox flow batteries by excess addition of bromine to the electrolytes, leading to the formation of a permanent bromine fused salt phase. This results in improved posolyte capacity and better cell performance compared to previous investigations.
JOURNAL OF POWER SOURCES
(2022)
Article
Chemistry, Physical
Benjamin B. Peterson, Evan M. Andrews, Francisco Hung, John C. Flake
Summary: Secondary lithium-bromine (Li-Br-2) batteries with carbonized metal-organic frameworks (MOFs) show improved capacities and retention rates, with ZIF-8 derived electrodes exhibiting higher specific capacities and retention over cycles. The enhanced performance is attributed to higher LiBr loadings, improved bromine trapping and adsorption, and the microporous structure with heteroatom bonding in ZIF-8 derived carbon electrodes.
JOURNAL OF POWER SOURCES
(2021)
Review
Chemistry, Physical
Uxua Jimenez-Blasco, Jose Carlos Arrebola, Alvaro Caballero, Federico Bella
Summary: The development of energy storage systems is crucial for replacing fossil fuels with clean energy. Zinc-bromine flow batteries offer attractive features and low cost, but require the use of bromine complexing agents to prevent corrosion and toxicity issues.
Article
Chemistry, Physical
Xiaoqiong Wang, Hao Guo, Ning Wu, Mengni Xu, Longwen Zhang, Wu Yang
Summary: A novel dual-emission ratio fluorescent sensor has been developed by introducing nitrogen-doped blue fluorescence carbon dots and red fluorescence carbon dots into the synthetic environment of ZIF-8. The sensor shows high selectivity and sensitivity for detecting Pb2+, making it a potential fluorescent sensor for Pb2+ detection.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2021)
Article
Chemistry, Physical
Mengde Li, Junjie Liu, Shuping Deng, Qian Liu, Ning Qi, Zhiquan Chen
Summary: In this study, three types of zeolite imidazole frameworks were synthesized and analyzed for their pore structures and CO2 adsorption capacities. The results indicate that at atmospheric pressure, CO2 is effectively captured by micropores, while at extremely low pressures, CO2 is mainly enriched around ultramicropores.
ACS APPLIED ENERGY MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Xinhua Zheng, Yongchao Wang, Yan Xu, Touqeer Ahmad, Yuan Yuan, Jifei Sun, Ruihao Luo, Mingming Wang, Mingyan Chuai, Na Chen, Taoli Jiang, Shuang Liu, Wei Chen
Summary: By utilizing a bromine redox mediator, a high-performance aqueous electrolytic MnO2-Zn battery has been developed with enhanced electrochemical performance, showing high discharge voltage and excellent cycling stability, thus opening up new possibilities for large-scale energy storage.
Article
Nanoscience & Nanotechnology
Yuxin Li, Kunpeng Wang, Lei Liu, Yuhong Liu
Summary: This paper investigates the potential of zeolite imidazole frameworks (ZIFs) in achieving solid superlubricity and reveals the influence mechanism of adhesion and surface stiffness on lubrication properties. By adjusting molecular structure, superlubricity modulation can be achieved, providing promising results for the precise design of two-dimensional superlubricity materials.
MATERIALS TODAY NANO
(2023)
Article
Engineering, Environmental
Jianbin Liu, Cunjian Lin, Qingshui Xie, Dong-Liang Peng, Rong-Jun Xie
Summary: This study introduces a catalytic interlayer (ZnSe@CoSe2/C@CC) for Li-S batteries, which regulates dissolved polysulfides and accelerates lithium-ion diffusion to enhance the initial capacity and cycling stability. The heterostructure shows potential applications in other rechargeable metal-sulfur batteries.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Applied
Xiutao Li, Haichang Zhang, Chao Liu, Junyu Qiao, Xiaomeng Zhou
Summary: In this study, a new type of fluorinated carbon was developed using Cr-MOF as a precursor via direct F-2 fluorination method, exhibiting a high energy density of 2110.7 W.h kg(-1) and maximum power density of 6540 W kg(-1) at different temperatures. The fluorinated carbon cathodes derived from MOF show an anti-swelling function with volume expansion not exceeding 12%, providing a new approach for designing advanced multifunctional fluorinated carbons.
MICROPOROUS AND MESOPOROUS MATERIALS
(2021)
Article
Materials Science, Multidisciplinary
Yan Jiang, Pei Hu
Summary: Nano-metal phosphides/carbon microspheres, Ni0.5Co0.5P2/carbon (NCP@C), with unique hollow structure were synthesized and used as anode material for Li-ion batteries. The composites exhibit high reversible specific capacity, good rate performance and excellent cycling stability.
Article
Chemistry, Physical
Fuxiang Wang, Qike Jiang, Zihan Song, Shanshan Liu, Kai Fen, Xin Yang, Zhenbo Cao, Jinsheng Jia, Hongzhang Zhang
JOURNAL OF POWER SOURCES
(2020)
Article
Chemistry, Multidisciplinary
Shanshan Liu, Guochun Zhang, Kai Feng, Yanyang Han, Tao He, Jinglin You, Yicheng Wu
CRYSTAL GROWTH & DESIGN
(2020)
Article
Nanoscience & Nanotechnology
Fuxiang Wang, Yanping Li, Wenjing Zhu, Xiuli Ge, Hongtao Cui, Kai Feng, Shanshan Liu, Xin Yang
Summary: KVHCF@DCCF cathode material, with multielectron reactions and high electronic conductivity, delivers high specific capacity and excellent rate performance among reported PBAs. It also shows high specific capacity even at low temperatures and maintains good capacity retention after cycles.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Shanshan Liu, Xiuli Ge, Tao Zhang, Yanyang Han, Wei Cui, Rengui Guan, Xin Yang, Tao He, Qingzhong Li, Kai Feng, Steve Scheiner
Summary: The experiment designed a feasible way to prepare flexible packaging batteries using inexpensive, safe, and easy-to-use materials. It offers students a new route to familiarize themselves with the construction and mechanism of lithium ion batteries.
JOURNAL OF CHEMICAL EDUCATION
(2021)
Article
Chemistry, Inorganic & Nuclear
Huibin Ding, Zihan Song, Kai Feng, Hongzhang Zhang, Huamin Zhang, Xianfeng Li
Summary: In this study, pure-phase metastable tetragonal niobium pentoxide (M-Nb2O5) was successfully synthesized using amorphous SiO2 shells as a confinement agent. The pure-phase M-Nb2O5 showed promising physical and electrochemical performance as an anode material for lithium-ion batteries.
JOURNAL OF SOLID STATE CHEMISTRY
(2021)
Article
Chemistry, Multidisciplinary
Yuanqing He, Lulu Jia, Xueyi Lu, Chenhui Wang, Xiaohe Liu, Gen Chen, Dan Wu, Zuxin Wen, Ning Zhang, Yusuke Yamauchi, Takayoshi Sasaki, Renzhi Ma
Summary: Heterostructure nanocomposites composed of different types of oxide nanosheets and layered double hydroxide nanosheets were assembled using electrostatic layer-by-layer assembly. The resulting bilayer films exhibited enhanced electrochemical activity for oxygen evolution reaction. The study provides insight into the rational control and manipulation of redox-active surface layers and conductive underlying layers for efficient electrocatalysis.
Article
Chemistry, Physical
Xiuli Ge, Ning Li, Xuefang Yu, Jianbo Cheng, Siliang Chang, Qian Zhao, Hongtao Cui, Kai Feng, Shanshan Liu, Xin Yang
Summary: The new tungstate anode material Li2Ni(WO4)(2)/C shows promising performance in lithium-ion batteries, with high specific capacity and multi-electronic reactions. The carbon coating improves conductivity and particle size, resulting in good cycle stability and rate performance for the material.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Electrochemistry
Xiuli Ge, Yongkai Chen, Shanshan Liu, Xin Yang, Kai Feng
Summary: In this study, Li-free polyanion vanadium sulfates containing Na/K alkali metals were successfully synthesized and mixed with carbon black to improve conductivity. These composites were investigated as cathode materials for lithium-ion batteries and showed reversible insertion-extraction of lithium ions. However, their rate performance and cyclic stability were poor.
JOURNAL OF SOLID STATE ELECTROCHEMISTRY
(2022)
Article
Nanoscience & Nanotechnology
Qian Zhao, Yaru Zhu, Shanshan Liu, Ye Liu, Tao He, Xuemei Jiang, Xin Yang, Kai Feng, Jianjiang Hu
Summary: A new rocking-chair-type cathode material Zn3V4(PO4)(6)@C (ZVP@C) with a stable crystal structure is synthesized, and a composite carbon coating is used to improve its electronic conductivity. The material exhibits a good capacity retention of 80% after 400 cycles at 1 A.g(-1).
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Chemistry, Physical
Siliang Chang, Shuai Han, Sen Ji, Shanshan Liu, Ye Liu, Xin Yang, Kai Feng, Jianjiang Hu
Summary: Niobium-based anode materials show promise for use in lithium-ion batteries due to their high specific capacity and safety. However, their low electronic conductivity limits their performance. In this study, a mixed-valent niobium-based phosphate, K3Nb6P4O26@C, was developed as an anode material. The mixed-valent Nb in KNPO enables multi-electron reactions and higher electronic conductivity. The 3D channels in the crystal structure of KNPO facilitate rapid lithium-ion transport. KNPO@C anode demonstrates a high specific capacity and excellent cycling stability, making it a potential practical material for high-performance LIBs.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
Article
Materials Science, Multidisciplinary
Chenhui Wang, Nobuyuki Sakai, Yasuo Ebina, Daiming Tang, Renzhi Ma, Takayoshi Sasaki
Summary: Zinc-based aqueous energy storage technology has attracted widespread interest due to its low cost, high energy density, high safety, and environmentally friendly manufacturing process. However, the generation of hydrogen gas and zinc dendrite formation have impeded its progress. This study introduces a promising interfacial engineering strategy by depositing molecularly thin Ti0.87O2 nanosheets on a zinc electrode surface, which effectively suppresses hydrogen gas evolution and reduces the nucleation potential of zinc. The improved electrode performance leads to a drastically increased cycle life of over 1400 hours at 1 mA cm(-2)/1 mAh cm(-2), enabling practical applications of zinc metal electrodes and showing potential for other metal batteries.
ACS MATERIALS LETTERS
(2023)
Article
Chemistry, Physical
Chuan Tang, Siliang Chang, Qian Wu, Lei Kang, Kai Feng, Xianghe Meng, Shengqi Chu, Hongwei Huang, Mingjun Xia
Summary: The study investigated a new high-performance titanyl germanate anode, Rb4Li2TiOGe4O12 (RLTG), for lithium-ion storage properties. Due to the multi-electron reactions of Ti and Ge and the polyanion framework, RLTG exhibits a high discharge specific capacity and decent capacity retention performance. In addition, RLTG shows a good rate capability in a wide range of current densities. Furthermore, detailed analysis of discharge/charge behaviors was conducted using various techniques and calculations.
JOURNAL OF MATERIALS CHEMISTRY A
(2023)
Article
Chemistry, Physical
Chenhui Wang, Nobuyuki Sakai, Yasuo Ebina, Shigeru Suehara, Takayuki Kikuchi, Daiming Tang, Renzhi Ma, Takayoshi Sasaki
Summary: In this study, a molecular pairwise/sandwich-like assembly of TaO3/rGO was fabricated to improve the loading and utilization of sulfur in Li-S batteries. The heterostructure exhibited fast Li+ transfer, effective confinement of polysulfides, and high catalytic activity, leading to high sulfur utilization and achieving a high areal capacity of 10.5 mA h cm(-2) at 2 mA cm(-2). This versatile strategy can be applied to various energy storage systems.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Article
Chemistry, Physical
Chenhui Wang, Nobuyuki Sakai, Yasuo Ebina, Takayuki Kikuchi, Monika R. Snowdon, Daiming Tang, Renzhi Ma, Takayoshi Sasaki
Summary: A three-in-one cathode host based on a superlattice of two-dimensional materials was designed to tackle the shuttle effect, sluggish kinetics of lithium polysulfide conversion, and nonuniform nucleation of Li2S in lithium-sulfur batteries. The Nb3O8/rGO superlattice cathode host showed high affinity, excellent catalytic activity, abundance of exposed active sites, and high electrical conductivity, resulting in high-performance lithium-sulfur batteries with an initial capacity of 1529 mA h g(-1) at 0.1C and a slow capacity decay of 0.064% per cycle at 1C over 1000 cycles.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Article
Chemistry, Physical
Di Ma, Zihan Song, Hongzhang Zhang, Arshad Hussain, Kai Feng, Huamin Zhang, Xianfeng Li
JOURNAL OF MATERIALS CHEMISTRY A
(2020)
Article
Chemistry, Physical
Sirinya Ukasi, Paritta Jutapukti, Chiranicha Ninthub, Nattapong Pinpru, Phakkhananan Pakawanit, Wanwilai Vittayakorn, Satana Pongampai, Naratip Vittayakorn, Thitirat Charoonsuk
Summary: This study explores the enhancement of electrical output of flexible hybrid piezoelectric-triboelectric nanogenerators by incorporating gamma-glycine into fully organic composites. The research demonstrates the importance of optimized concentrations of gamma-glycine and chitosan in achieving superior performance. The study identifies the critical content of gamma-glycine that leads to the highest output signal, and provides theoretical explanations for this observation.
Article
Chemistry, Physical
Yoonsang Ra, Yu-seop Kim, Seonmo Yang, Namgyu Kang, Gyuwon Oh, Chungyeon Cho, Sangmin Lee, Dongwhi Choi
Summary: In this study, a portable energy harvester (STEP) was proposed to drive various functional LEDs using biomechanical energy. The roles and functionalities of a triboelectric nanogenerator (TENG) and electromagnetic generator (EMG) in the hybrid energy harvester were experimentally demonstrated, and the necessity of hybridization for LED-involved devices was described. The STEP showed promising potential as an effective energy supply strategy for various functional LEDs in related industries.
Article
Chemistry, Physical
Dae Sol Kong, Kyung Hoon Kim, Ying Chieh Hu, Jong Hun Kim, Inseo Kim, Jeongwan Lee, Joonhyuk Lee, Won Hyuk Shon, Hanjin Yoo, Chul-Un Ro, Seungsu Lee, Hyoungjeen Jeen, Minbaek Lee, Minseok Choi, Jong Hoon Jung
Summary: With the rapid development of the Internet of Things and artificial intelligence, smart home has emerged to fulfill the security, convenience, and energy-saving issues of modern life. A flexoelectric mica crystal is used to augment the finger touch-driven triboelectric output for operating a wireless and multichannel smart home controller. This work provides important ingredients for enhancing triboelectric output and realizing a convenient, multifunctional, cost-effective, and adaptable smart home control system without batteries.
Article
Chemistry, Physical
Yi Han, Fang Wu, Xiaozhen Du, Zihao Li, Haixiang Chen, Dongxing Guo, Junlei Wang, Hong Yu
Summary: This paper presents a novel type of triboelectric nanogenerator that utilizes wind energy, with a Y-type bluff body to enhance vibration and output power. The application of this generator successfully provides power for a wireless temperature and humidity sensor.
Article
Chemistry, Physical
Wen Zhang, Fangyuan Cheng, Miao Chang, Yue Xu, Yuyu Li, Shixiong Sun, Liang Wang, Leimin Xu, Qing Li, Chun Fang, Meng Wang, Yuhao Lu, Jiantao Han, Yunhui Huang
Summary: This study successfully induced the formation of a uniform and robust CEI by constructing ZrO2 nano-rivets on the surface of LCO, stabilizing the surface of high-voltage LCO and facilitating lithium-ion diffusion.
Article
Chemistry, Physical
Karl P. Olson, Laurence D. Marks
Summary: This paper investigates the role of contacting shapes in triboelectricity and provides scaling rules for designing energy harvesting devices.
Article
Chemistry, Physical
Jong-An Choi, Jingu Jeong, Mingyu Kang, Hee-Jin Ko, Taehoon Kim, Keun Park, Jongbaeg Kim, Soonjae Pyo
Summary: Wind-driven triboelectric nanogenerators (WTENGs) are a promising emerging technology for sustainable wind energy harvesting, offering high output performance, lightweight design, and compact dimensions. This study introduces an innovative WTENG design that leverages a rolling-based mechanism to achieve efficient omnidirectional wind energy harvesting.
Article
Chemistry, Physical
Liwei Dong, Qian Tang, Chaoyang Zhao, Guobiao Hu, Shuai Qu, Zicheng Liu, Yaowen Yang
Summary: This paper proposes a novel hybrid scheme for flag-type nanogenerators (FNGs) that enhances their performance and broadens their operational wind speed ranges by harnessing the synergistic potential of two aerodynamic behaviors. The proposed flag-type triboelectric-piezoelectric hybrid nanogenerator (FTPNG) integrates flapping piezoelectric flags (PEFs) and a fluttering triboelectric flag (TEF). The FTPNG achieves significant power generation and a broad wind speed range, surpassing other FNGs, making it suitable for various self-powered systems and Internet of Things applications.
Review
Chemistry, Physical
Yunmeng Li, Xin Liu, Zewei Ren, Jianjun Luo, Chi Zhang, Changyong (Chase) Cao, Hua Yuan, Yaokun Pang
Summary: The demand for green and eco-friendly materials is growing due to increasing environmental concerns related to traditional petroleum-based products. Marine biomaterials have emerged as a promising alternative, thanks to their abundant availability, biocompatibility, biodegradability, and low toxicity. In this review, we discuss the development and applications of triboelectric nanogenerators (TENGs) based on marine biomaterials. The operational modes, foundational principles, intrinsic qualities, and advantages of marine biomaterials commonly used in TENG designs are highlighted. Approaches to enhance the efficacy of TENGs derived from marine biomaterials are also discussed, along with documented applications from existing literature. Furthermore, the existing challenges and future directions in marine biomaterial-inspired TENGs are explored.
Article
Chemistry, Physical
Matthew P. Wells, Adam J. Lovett, Yizhi Zhang, Zhongxia Shang, Kosova Kreka, Babak Bakhit, Haiyan Wang, Albert Tarancon, Judith L. MacManus-Driscoll
Summary: Reversible solid oxide cells (rSOCs) offer a promising solution to efficient energy conversion, but have been limited in portable power and electrolysis applications due to excessive polarisation resistance of the oxygen electrode at low temperatures. This study demonstrates the growth of symmetric and complete rSOC structures with reduced polarisation resistance by tuning oxygen vacancy through annealing, providing a promising route towards high-performance rSOC devices for portable power applications.
Article
Chemistry, Physical
Kangkang Bao, Minghui Wang, Yue Zheng, Panpan Wang, Liwen Yang, Yang Jin, Hui Wu, Bin Sun
Summary: This study utilizes ethanol as an electrolyte additive to modulate the migration of zinc ions and the surface structure of zinc anodes, resulting in improved capacity retention and cycle life of zinc-based aqueous batteries.
Article
Chemistry, Physical
Haichao Yang, Wensi Cai, Ming Wang, Saif M. H. Qaid, Zhiyuan Xu, Huaxin Wang
Summary: The introduction of sodium alginate (SA) into perovskite solar cells improves the carrier dynamics, stability, and performance by inhibiting nonradiative recombination and retarded charge dynamics.
Article
Chemistry, Physical
Cuirong Zhang, Mingyuan Wei, Zihan Chen, Wansheng Lin, Shifan Yu, Yijing Xu, Chao Wei, Jinwei Zhang, Ziquan Guo, Yuanjin Zheng, Qingliang Liao, Xinqin Liao, Zhong Chen
Summary: Artificial Intelligence of Things (AIoT) aims to establish smart and informative interactions between humans and devices. However, common pixelated sensing arrays in AIoT applications present problems such as hard and brittle devices, complex structures, and low precision. This article introduces an innovative solution called the all-in-one intelligent semitransparent interactive nerve patch (AISI nerve patch), which integrates sensing, recognition, and transmission functionalities into a thin and flexible patch. The AISI nerve patch is semitransparent, allowing for accurate identification without affecting aesthetics, and it can be attached to any curved surface for intelligent and interactive applications. With rapid response time and high precision recognition, it enables the integration of artificial intelligence and achieves high recognition accuracy for further development of AIoT.
Article
Chemistry, Physical
Youcun Bai, Heng Zhang, Huijun Song, Chong Zhu, Lijin Yan, Qin Hu, Chang Ming Li
Summary: A novel stainless-steel supported lattice-mismatched V-S-Se layered compound with high selenium vacancy was synthesized by adjusting the molar ratio of sulfur to selenium. The introduction of selenium vacancies created additional redox peaks of sulfur, providing more mass transport channels and active sites for zinc ions. The specific capacity and cycle stability of the electrode were significantly improved, demonstrating great potential for practical applications and providing insights into the effects of defects on battery performance.
Article
Chemistry, Physical
Yao Xiao, Puxian Xiong, Yakun Le, Zhenjie Lun, Kang Chen, Zhiduo Wang, Peishan Shao, Zhicong Chen, Dongdan Chen, Zhongmin Yang
Summary: This study successfully synthesized a material with multi-stimulus-responsive luminescence and confirmed the internal relationship between luminescence and defects by regulating the distribution and depth of defects. The dynamic process of multi-stimulus-responsive luminescence was validated by experimental and calculation results.