Journal
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
Volume 6, Issue 3, Pages 3546-3555Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.7b03870
Keywords
Organic; Inorganic; Self-assembly; PPC; Corrosion resistance
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Funding
- First Research Grant of the National Research Foundation - Ministry of Science and ICT, Republic of Korea [NRF-2017R1C1B5077139]
- Nano-Material Technology Development Program [2009-0082580]
- [NRF-2017H1D2A2063357]
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Organic-inorganic coating has been desirable for practical applications in electrochemistry and analytical science. Up to this investigation, a report of a flowerlike structure made from organic components has been rarely reported. Here, we proposed a novel strategy to fabricate the flowerlike hybrid coating through the combination of plasma electrolysis and dip chemical coating in which 4-[4-(phyenylazo)phenylazo]-o-cresol (PPC) was used as the organic component. The formation of organic molecules was initiated effectively on the rough inorganic coating by the charge transfer complexes which facilitate the nucleation of organic molecules. The quantum chemical analysis was implemented to discuss the binding sites activated by PPC. The electrochemical resistance was improved significantly due to the synergistic influences of the inorganic coating via plasma electrolysis and organic coating via self-assembly of PPC.
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