4.7 Article

Tracking oil and gas wastewater-derived organic matter in a hybrid biofilter membrane treatment system: A multi-analytical approach

Journal

SCIENCE OF THE TOTAL ENVIRONMENT
Volume 613, Issue -, Pages 208-217

Publisher

ELSEVIER SCIENCE BV
DOI: 10.1016/j.scitotenv.2017.09.031

Keywords

Dissolved organic matter; 3D fluorescence spectroscopy; Produced water; Biofiltration; Ultrafiltration; Nanofiltration

Funding

  1. National Science Foundation Sustainability Research Network program [CBET-1240584]
  2. ConocoPhillips
  3. Directorate For Engineering
  4. Div Of Chem, Bioeng, Env, & Transp Sys [1240584] Funding Source: National Science Foundation

Ask authors/readers for more resources

Dissolved organic matter (DOM) present in oil and gas (O&G) produced water and fracturing flowback was characterized and quantified by multiple analytical techniques throughout a hybrid biological-physical treatment process. Quantitative and qualitative analysis of DOM by liquid chromatography-organic carbon detection (LC-OCD), liquid chromatography-high-resolution mass spectrometry (LC-HRMS), gas chromatography-mass spectrometry (GC-MS), and 3D fluorescence spectroscopy, demonstrated increasing removal of all groups of DOM throughout the treatment train, with most removal occurring during biological pretreatment and some subsequent removal achieved during membrane treatment. Parallel factor analysis (PARAFAC) further validated these results and identified five fluorescent components, including DOM described as humic acids, fulvic acids, proteins, and aromatics. Tryptophan-like compounds bound by complexation to humics/fulvics were most difficult to remove biologically, while aromatics (particularly low molecular weight neutrals) were more challenging to remove with membranes. Strong correlation among PARAFAC, LC-OCD, LC-HRMS, and GC-MS suggests that PARAFAC can be a quick, affordable, and accurate tool for evaluating the presence or removal of specific DOM groups in O& G wastewater. (C) 2017 Elsevier B.V. All rights reserved.

Authors

I am an author on this paper
Click your name to claim this paper and add it to your profile.

Reviews

Primary Rating

4.7
Not enough ratings

Secondary Ratings

Novelty
-
Significance
-
Scientific rigor
-
Rate this paper

Recommended

Review Chemistry, Multidisciplinary

Rating the risks of anticoagulant rodenticides in the aquatic environment: a review

Julia Regnery, Anton Friesen, Anke Geduhn, Bernd Goeckener, Matthias Kotthoff, Pia Parrhysius, Eleonora Petersohn, Georg Reifferscheid, Erik Schmolz, Robert S. Schulz, Jan Schwarzbauer, Marvin Brinke

ENVIRONMENTAL CHEMISTRY LETTERS (2019)

Article Engineering, Environmental

Removal of per- and polyfluoroalkyl substances using super-fine powder activated carbon and ceramic membrane filtration

Conner C. Murray, Hooman Vatankhah, Carrie A. McDonough, Anastasia Nickerson, Tayler T. Hedtke, Tzahi Y. Cath, Christopher P. Higgins, Christopher L. Bellona

JOURNAL OF HAZARDOUS MATERIALS (2019)

Review Engineering, Environmental

Data-driven performance analyses of wastewater treatment plants: A review

Kathryn B. Newhart, Ryan W. Holloway, Amanda S. Hering, Tzahi Y. Cath

WATER RESEARCH (2019)

Article Environmental Sciences

Variable non-linear removal of viruses during transport through a saturated soil column

Walter Q. Betancourt, Jack Schijven, Julia Regnery, Alexandre Wing, Christina M. Morrison, Joerg E. Drewes, Charles P. Gerba

JOURNAL OF CONTAMINANT HYDROLOGY (2019)

Article Environmental Sciences

Emergence and fate of volatile iodinated organic compounds during biological treatment of oil and gas produced water

Nohemi Almaraz, Julia Regnery, Gary F. Vanzin, Stephanie M. Riley, Danika C. Ahoor, Tzahi Y. Cath

SCIENCE OF THE TOTAL ENVIRONMENT (2020)

Article Environmental Sciences

Hydrogeochemical and microbiological effects of simulated recharge and drying within a 2D meso-scale aquifer

Julia Regnery, Dong Li, Jonghyun Lee, Kathleen M. Smits, Jonathan O. Sharp

CHEMOSPHERE (2020)

Article Environmental Sciences

Developing a novel biofiltration treatment system by coupling high-rate infiltration trench technology with a plug-flow porous-media bioreactor

Sema Karakurt-Fischer, Alicia Sanz-Prat, Janek Greskowiak, Martin Ergh, Heiko Gerdes, Gudrun Massmann, Juergen Ederer, Julia Regnery, Uwe Huebner, Joerg E. Drewes

SCIENCE OF THE TOTAL ENVIRONMENT (2020)

Article Environmental Sciences

Heavy rainfall provokes anticoagulant rodenticides' release from baited sewer systems and outdoor surfaces into receiving streams

Julia Regnery, Robert S. Schulz, Pia Parrhysius, Julia Bachtin, Marvin Brinke, Sabine Schaefer, Georg Reifferscheid, Anton Friesen

SCIENCE OF THE TOTAL ENVIRONMENT (2020)

Article Environmental Sciences

Does galvanic cathodic protection by aluminum anodes impact marine organisms?

Anna Maria Bell, Marcus von der Au, Julia Regnery, Matthias Schmid, Bjoern Meermann, Georg Reifferscheid, Thomas Ternes, Sebastian Buchinger

ENVIRONMENTAL SCIENCES EUROPE (2020)

Article Environmental Sciences

New insights on in vitro biotransformation of anticoagulant rodenticides in fish

Julia Regnery, Carolin Riegraf, Stefanie Jacob, Anton Friesen

Summary: The study investigates the in vitro biotransformation rates of eight biocidal and one pharmaceutical anticoagulants in rainbow trout liver subcellular S9 fraction. The results show that four of the tested substances exhibit significant intrinsic clearance in the assay, and the metabolism is slow and temperature-dependent. However, further research is needed to determine the influence of in vitro biotransformation rates on the prediction of bioconcentration factors.

CHEMOSPHERE (2022)

Article Engineering, Environmental

Multistage Surface-Heated Vacuum Membrane Distillation Process Enables High Water Recovery and Excellent Heat Utilization: A Modeling Study

Yiming Liu, Jingbo Wang, Eric M. V. Hoek, Federico Municchi, Nils Tilton, Tzahi Y. Cath, Craig S. Turchi, Michael B. Heeley, David Jassby

Summary: This study investigates the design and performance of a multistage surface-heated vacuum membrane distillation (SHVMD) system with heat recovery. The results show that surface heating enhances the performance of SHVMD compared to conventional vacuum membrane distillation (VMD), achieving higher water recovery and gained output ratio (GOR). The internal and external heat exchangers capture and reuse additional heat, further improving the GOR values. Additionally, surface heating reduces the energy consumption of membrane distillation for brine concentration.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2023)

Article Environmental Sciences

Functional Data Analysis Approach for Detecting Faults in Cyclic Water and Wastewater Treatment Processes

Aurora Kuras, Tzahi Y. Cath, Amanda S. Hering

Summary: Early and effective fault detection is important for maintaining water quality and preventing disruptions in water and wastewater treatment plants. This paper applies functional data analysis (FDA) to detect drift faults in a sequencing batch membrane bioreactor and a closed-circuit reverse osmosis system. FDA enables the analysis of cyclic data and identifies unusual functions by comparing them to a reference set.

ACS ES&T WATER (2023)

Article Environmental Sciences

A Holistic Evaluation of Multivariate Statistical Process Monitoring in a Biological and Membrane Treatment System

Kathryn B. Newhart, Molly C. Klanderman, Amanda S. Hering, Tzahi Y. Cath

Summary: Unsupervised process monitoring for fault detection and data cleaning in wastewater treatment plants is underdeveloped due to the complexity and volume of data. This study evaluates the performance of the adaptive dynamic principal component analysis (AD-PCA) method in detecting faults in a decentralized WWTP. The results show that implementing AD-PCA with appropriate parameters can detect faults prior to existing operational thresholds, although further work is needed to improve its consistency in real-time fault detection.

ACS ES&T WATER (2023)

Article Environmental Sciences

Membrane Bioreactor Pretreatment of High-Salinity O&G Produced Water

Brett D. Van Houghton, Shwetha M. Acharya, James S. Rosenblum, Romy Chakraborty, Susannah Green Tringe, Tzahi Y. Cath

Summary: The study showed that membrane bioreactors (MBRs) exhibit excellent long-term performance in removing organic constituents from produced water (PW), even in high salinity conditions. MBRs were effective in removing dissolved organic carbon from PW from different shale basins, but showed less consistent removal of surfactants. The study also found that microbial diversity decreased during reactor establishment but increased at higher total dissolved solid (TDS) concentrations.

ACS ES&T WATER (2022)

Article Environmental Sciences

Comparing nearshore and embayment scale assessments of submarine groundwater discharge: Significance of offshore groundwater discharge as a nutrient pathway

Toshimi Nakajima, Mao Kuragano, Makoto Yamada, Ryo Sugimoto

Summary: This study compared the contribution of submarine groundwater discharge (SGD) to river nutrient budgets at nearshore and embayment scales, and found that SGD-derived nutrients become more important at larger spatial scales.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Impact of NO2 emissions from household heating systems with wall-mounted gas stoves on indoor and ambient air quality in Chinese urban areas

Fan Liu, Lei Zhang, Chongyang Zhang, Ziguang Chen, Jingguang Li

Summary: NO2 emissions from wall-mounted gas stoves used for household heating have become a significant source of indoor pollution in Chinese urban areas. The high indoor concentration of NO2 poses potential health risks to residents. It is urgently necessary to establish relevant regulations and implement emission reduction technologies to reduce NO2 emissions from wall-mounted gas stoves.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Letter Environmental Sciences

Letter to the editor regarding Collard et al. (2023): Persistence and mobility (defined as organic-carbon partitioning) do not correlate to the detection of substances found in surface and groundwater: Criticism of the regulatory concept of persistent and mobile substances

Hans Peter H. Arp, Raoul Wolf, Sarah E. Hale, Sivani Baskaran, Juliane Gluege, Martin Scheringer, Xenia Trier, Ian T. Cousins, Harrie Timmer, Roberta Hofman-Caris, Anna Lennquist, Andre D. Bannink, Gerard J. Stroomberg, Rosa M. A. Sjerps, Rosa Montes, Rosario Rodil, Jose Benito Quintana, Daniel Zahn, Herve Gallard, Tobias Mohr, Ivo Schliebner, Michael Neumann

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Harnessing the composition of dissolved organic matter in lagoon sediment in association with rare earth elements using fluorescence and UV-visible absorption spectroscopy

Philomina Onyedikachi Peter, Binessi Edouard Ifon, Francois Nkinahamira, Kayode Hassan Lasisi, Jiangwei Li, Anyi Hu, Chang-Ping Yu

Summary: This study investigates the relationship between dissolved organic matter (DOM) and Rare Earth Elements (REEs) in sediments from Yundang Lagoon, China. The results show four distinct fluorescent components, with protein-like substances being the most prevalent. Additionally, the total fluorescence intensity and LREE concentrations exhibit a synchronized increase from Outer to Inner to Songbai Lake core sediments. The findings demonstrate a strong correlation between DOM content and pollution levels.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

An advanced global soil erodibility (K) assessment including the effects of saturated hydraulic conductivity

Surya Gupta, Pasquale Borrelli, Panos Panagos, Christine Alewell

Summary: The objective of this study is to incorporate soil hydraulic properties into the erodibility factor (K) of USLE-type models. By modifying and improving the existing equations for soil texture and permeability, the study successfully included information on saturated hydraulic conductivity (Ksat) into the calculation of K factor. Using the Random Forest machine learning algorithm, two independent K factor maps with different spatial resolutions were generated. The results show that the decrease in K factor values has a positive impact on the modeling of soil erosion rates.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Comparison of adsorption-extraction (AE) workflows for improved measurements of viral and bacterial nucleic acid in untreated wastewater

Jesmin Akter, Wendy J. M. Smith, Yawen Liu, Ilho Kim, Stuart L. Simpson, Phong Thai, Asja Korajkic, Warish Ahmed

Summary: The choice of workflow in wastewater surveillance has a significant impact on SARS-CoV-2 concentrations, while having minimal effects on HF183 and no effect on HAdV 40/41 concentrations. Certain components in the workflow can be interchangeable, but factors such as buffer type, chloroform, and homogenization speed can affect the recovery of viruses and bacteria.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Insights the dominant contribution of biomass burning to methanol-soluble PM2.5 bounded oxidation potential based on multilayer perceptron neural network analysis in Xi'an, China

Yu Luo, Xueting Yang, Diwei Wang, Hongmei Xu, Hongai Zhang, Shasha Huang, Qiyuan Wang, Ningning Zhang, Junji Cao, Zhenxing Shen

Summary: Atmospheric PM2.5, which can generate reactive oxygen species (ROS), is associated with cardiorespiratory morbidity and mortality. The study found that both the mass concentration of PM2.5 and the DTT activity were higher during the heating season than during the nonheating season. Combustion sources were the primary contributors to DTT activity during the heating season, while secondary formation dominated during the nonheating season. The study also revealed that biomass burning had the highest inherent oxidation potential among all sources investigated.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

A macroplastic vulnerability index for marine mammals, seabirds, and sea turtles in Hawai'i

Erin L. Murphy, Leah R. Gerber, Chelsea M. Rochman, Beth Polidoro

Summary: Plastic pollution has devastating consequences for marine organisms. This study uses a trait-based framework to develop a vulnerability index for marine mammals, seabirds, and sea turtles in Hawai'i. The index ranks 63 study species based on their vulnerability to macroplastic pollution, providing valuable information for species monitoring and management priorities.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Anthropic disturbances impact the soil microbial network structure and stability to a greater extent than natural disturbances in an arid ecosystem

Kenji Maurice, Amelia Bourceret, Sami Youssef, Stephane Boivin, Liam Laurent-Webb, Coraline Damasio, Hassan Boukcim, Marc-Andre Selosse, Marc Ducousso

Summary: Growing pressure from climate change and agricultural land use is destabilizing soil microbial community interactions. Little is known about microbial community resistance and adaptation to disturbances, hindering our understanding of recovery latency and implications for ecosystem functioning. This study found that anthropic disturbance and natural disturbance have different effects on the topology and stability of soil microbial networks.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Adsorption of metal ions by oceanic manganese nodule and deep-sea sediment: Behaviour, mechanism and evaluation

Yunhao Li, Yali Feng, Haoran Li, Yisong Yao, Chenglong Xu, Jinrong Ju, Ruiyu Ma, Haoyu Wang, Shiwei Jiang

Summary: Deep-sea mining poses a serious threat to marine ecosystems and human health by disturbing sediment and transmitting metal ions through the food chain. This study developed a new regenerative adsorption material, OMN@SA, which effectively removes metal ions. The adsorption mechanism and performance of the material for metal ion fixation were investigated.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Advanced oxidation process of valsartan by activated peroxymonosulfate: Chemical characterization and ecotoxicological effects of its byproducts

Antonio Medici, Margherita Lavorgna, Marina Isidori, Chiara Russo, Elena Orlo, Giovanni Luongo, Giovanni Di Fabio, Armando Zarrelli

Summary: Valsartan, a widely used antihypertensive drug, has been detected in high concentrations in surface waters due to its unchanged excretion and incomplete degradation in wastewater treatment plants. This study investigated the degradation of valsartan and identified 14 degradation byproducts. The acute and chronic toxicity of these byproducts were evaluated in key organisms in the freshwater trophic chain.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Photodegradation of typical pharmaceuticals changes toxicity to algae in estuarine water: A metabolomic insight

Jiang Lin, Lianbao Chi, Qing Yuan, Busu Li, Mingbao Feng

Summary: This study investigated the photodegradation behavior and product formation of two representative pharmaceuticals in simulated estuary water. The study found that the formed transformation products of these pharmaceuticals have potential toxicity on marine organisms, including oxidative stress and damage to cellular components.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Association of ambient air pollution and pregnancy rate among women undergoing assisted reproduction technology in Fujian, China: A retrospective cohort study

Hua Fang, Dongdong Jiang, Ye He, Siyi Wu, Yuehong Li, Ziqi Zhang, Haoting Chen, Zixin Zheng, Yan Sun, Wenxiang Wang

Summary: This study revealed that exposure to lower levels of air pollutants led to decreased pregnancy rates, with PM10, NO2, SO2, and CO emerging as the four most prominent pollutants. Individuals aged 35 and above exhibited heightened susceptibility to pollutants.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

The predictive machine learning model of a hydrated inverse vulcanized copolymer for effective mercury sequestration from wastewater

Ali Shaan Manzoor Ghumman, Rashid Shamsuddin, Amin Abbasi, Mohaira Ahmad, Yoshiaki Yoshida, Abdul Sami, Hamad Almohamadi

Summary: In this study, inverse vulcanized polysulfides (IVP) were synthesized by reacting molten sulfur with 4-vinyl benzyl chloride, and then functionalized using N-methyl D-glucamine (NMDG). The functionalized IVP showed a high mercury adsorption capacity and a machine learning model was developed to predict the amount of mercury removed. Furthermore, the functionalized IVP can be regenerated and reused, providing a sustainable and cost-effective adsorbent.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)

Article Environmental Sciences

Aluminium bioaccumulation in colon cancer, impinging on epithelial-mesenchymal-transition and cell death

Rita Bonfiglio, Renata Sisto, Stefano Casciardi, Valeria Palumbo, Maria Paola Scioli, Erica Giacobbi, Francesca Servadei, Gerry Melino, Alessandro Mauriello, Manuel Scimeca

Summary: This study investigated the presence of aluminum in human colon cancer samples and its potential association with biological processes involved in cancer progression. Aluminum was found in tumor areas of 24% of patients and was associated with epithelial to mesenchymal transition (EMT) and cell death. Additional analyses revealed higher tumor mutational burden and mutations in genes related to EMT and apoptosis in aluminum-positive colon cancers. Understanding the molecular mechanisms of aluminum toxicity may improve strategies for the management of colon cancer patients.

SCIENCE OF THE TOTAL ENVIRONMENT (2024)