4.8 Article

Anomalous density fluctuations in a strange metal

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.1721495115

Keywords

non-Fermi liquid; strange metal; cuprates; quantum criticality; electron energy-loss spectroscopy

Funding

  1. Center for Emergent Superconductivity, an Energy Frontier Research Center - US Department of Energy (DOE), Office of Basic Energy Sciences [DE-AC02-98CH10886]
  2. DOE [DE-SC0012704]
  3. EPiQS program of the Gordon and Betty Moore Foundation [GBMF4542]
  4. NSF CAREER Grant [DMR-1352604]
  5. Alexander von Humboldt Foundation through the Feodor Lynen Fellowship program

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A central mystery in high-temperature superconductivity is the origin of the so-called strange metal (i.e., the anomalous conductor from which superconductivity emerges at low temperature). Measuring the dynamic charge response of the copper oxides, chi(q, omega), would directly reveal the collective properties of the strange metal, but it has never been possible to measure this quantity with millielectronvolt resolution. Here, we present a measurement of chi(q, omega) for a cuprate, optimally doped Bi2.1Sr1.9CaCu2O8+x (T-c = 91 K), using momentum-resolved inelastic electron scattering. In the medium energy range 0.1-2 eV relevant to the strange metal, the spectra are dominated by a featureless, temperature- and momentum-independent continuum persisting to the electronvolt energy scale. This continuum displays a simple power-law form, exhibiting q(2) behavior at low energy and q(2)/omega(2) behavior at high energy. Measurements of an overdoped crystal (T-c = 50 K) showed the emergence of a gap-like feature at low temperature, indicating deviation from power law form outside the strange-metal regime. Our study suggests the strange metal exhibits a new type of charge dynamics in which excitations are local to such a degree that space and time axes are decoupled.

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