Article
Materials Science, Multidisciplinary
Nagaraj Murugan, Rajendran Jerome, Murugan Preethika, Anandhakumar Sundaramurthy, Ashok K. Sundramoorthy
Summary: This study reports the synthesis of mixed phase 2D MXene as a catalytic material for simultaneous detection of important biomolecules such as AA, DA and UA. The Ti-C-T-x modified GCE showed excellent electrocatalytic activity and separated oxidation peaks, enabling the simultaneous detection of these biomolecules with high sensitivity and stability.
JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
(2021)
Article
Chemistry, Analytical
Peng Wu, Yufu Huang, Xueling Zhao, Donghai Lin, Lili Xie, Zhanhong Li, Zhigang Zhu, Hongli Zhao, Minbo Lan
Summary: In this study, MnFe2O4/MoS2 nanocomposite (MMF) was synthesized using a one-pot solvothermal method as an artificial enzyme for simultaneous electrochemical detection of AA, DA, and UA. The MMF showed high sensitivity and anti-interference ability towards the analytes.
MICROCHEMICAL JOURNAL
(2022)
Article
Nanoscience & Nanotechnology
Hussen Maseed, Veera Manohara Reddy Yenugu, Sesha SuryaBindu Devarakonda, Shaikshavali Petnikota, Madhavi Gajulapalli, Vadali V. S. S. Srikanth
Summary: A nano-Fe3O4/few-layered graphene (FLG) composite was prepared and used as a sensor for ultrasensitive detection of dopamine (DA). The sensor demonstrated excellent sensitivity and selectivity, and could reliably detect DA even in the presence of interfering substances uric acid (UA) and ascorbic acid (AA).
ACS APPLIED NANO MATERIALS
(2023)
Article
Engineering, Electrical & Electronic
Sadik Cogal, Venkat R. Bhethanabotla
Summary: In this study, a nanocomposite of two-dimensional WSe2 nanosheets with carbon black was prepared and used for electrode modification for the simultaneous electrochemical detection of AA, DA, and UA. The modified electrode exhibited enhanced electrocatalytic properties, wide linear ranges, and low detection limits for the target analytes. Additionally, it demonstrated high reproducibility and stability.
IEEE SENSORS JOURNAL
(2022)
Article
Materials Science, Multidisciplinary
Cheng-Hui Shen, Yu-Na Chang, You-Liang Chen, Chung-Wei Kung
Summary: A highly porous and chemically stable metal-organic framework (MOF) with enriched sulfonate groups, SO3-MOF-808, is synthesized and proposed as a porous alternative to Nafion for modulating the selectivity of electrochemical reactions. The use of SO3-MOF-808 thin film as an electrode coating significantly improves the current signal for dopamine oxidation and the selectivity against interfering compounds.
ACS MATERIALS LETTERS
(2023)
Article
Chemistry, Physical
Mingyue Wang, Hao Guo, Ning Wu, Junye Zhang, Tinging Zhang, Bingqing Liu, Zhilan Pan, Liping Peng, Wu Yang
Summary: A novel triazine-based covalent organic framework and its composite were successfully constructed by in situ growth of gold nanoparticles on its surface, followed by introduction of reduced graphene oxide. The constructed nanocomposite modified electrode exhibited excellent conductivity and catalytic activity, allowing for simultaneous detection of uric acid, dopamine, and ascorbic acid in urine samples accurately and rapidly.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2022)
Article
Chemistry, Multidisciplinary
Shiqi Cheng, Jin Yang, Shangying Qin, Li Huang, Yuanjin Xu, Yilin Wang
Summary: Three-dimensional reduced graphene oxide (3DrGO) and a flower-like zinc oxide (ZnO) crystal were prepared using a hydrothermal method. A stable dispersion of the 3DrGO-ZnO composite was formed and applied to modify a glassy carbon electrode for the detection of ascorbic acid (AA), dopamine (DA) and uric acid (UA). The 3DrGO-ZnO electrode exhibited enhanced electrocatalytic properties and could distinguish and enhance the differential pulse voltammetry signals of AA, DA and UA. The modified electrode showed potential for practical application in the analysis of real samples.
NEW JOURNAL OF CHEMISTRY
(2023)
Article
Chemistry, Analytical
Iris Baffour Ansah, Won-Chul Lee, ChaeWon Mun, Jong-Joo Rha, Ho Sang Jung, Mijeong Kang, Sung-Gyu Park, Dong-Ho Kim
Summary: A simple solution-based surface-enhanced Raman spectroscopy (SERS) method was developed for rapid and direct ternary detections of ascorbic acid (AA), dopamine (DA), and uric acid (UA) in urine with high sensitivity and selectivity, achieving detection limits of 1, 0.1, and 1 nM respectively. This is the first demonstration of simultaneous detection and quantification of biomolecules using SERS.
SENSORS AND ACTUATORS B-CHEMICAL
(2022)
Article
Chemistry, Analytical
Ying Wang, Peng Zhao, Bo Gao, Min Yuan, Jiabing Yu, Zeping Wang, Xianping Chen
Summary: Two-dimensional MXene nanosheets were used to functionalize three-dimensional laser-scribed graphene (LSG) and obtain an LSG-MXene hybrid scaffold. Shape-controlled Au-Pd bimetallic nanoparticles were synthesized on the LSG-MXene surface to enhance its catalytic performance. The fabricated sensor showed low detection limits for ascorbic acid, dopamine, and uric acid and can be used for their determination in urine samples.
MICROCHEMICAL JOURNAL
(2023)
Article
Chemistry, Analytical
Yaqi Huang, Yujiao Zang, Shaojie Ruan, Yaoyao Zhang, Panpan Gao, Wei Yin, Changjun Hou, Danqun Huo, Mei Yang, Huan-bao Fa
Summary: The phosphorus-doped nitrogenous porous carbon material was used to fabricate an electrochemical sensor for simultaneous determination of ascorbic acid, dopamine, and uric acid. The sensor showed excellent linear response ranges and detection limits for the three substances, and performed well in real serum sample analysis.
MICROCHEMICAL JOURNAL
(2021)
Article
Electrochemistry
Francesca Mazzara, Bernardo Patella, Giuseppe Aiello, Alan O'Riordan, Claudia Torino, Antonio Vilasi, Rosalinda Inguanta
Summary: An electrochemical sensor based on reduced graphene oxide and gold nanoparticles was developed for sensitive and selective detection of uric acid and ascorbic acid. The sensor showed excellent performance in detecting uric acid with good selectivity to interfering species, and simultaneous detection of uric acid and ascorbic acid reached low detection limits. Validation in real samples demonstrated the sensor's accuracy compared to conventional techniques.
ELECTROCHIMICA ACTA
(2021)
Article
Chemistry, Analytical
Xia Peng, Yi Xie, Yan Du, Yonghai Song, Shouhui Chen
Summary: A vertical N-doped carbon nanosheets/three-dimensional porous carbon (3D-KSC/C-CSBP) nanocomposite was successfully prepared and characterized in this study. The electrochemical sensor based on this nanocomposite showed excellent performance in simultaneously detecting AA, DA, and UA, with good stability, repeatability, and anti-interference ability.
JOURNAL OF ELECTROANALYTICAL CHEMISTRY
(2022)
Article
Materials Science, Multidisciplinary
Jiazheng Zhang, Yuhan Zhang, Tongtong Cao, Yicheng Zhou, Li Dong, Lin Liu, Zhiwei Tong
Summary: This study synthesized ERGO-MnTMPyP and investigated its electrochemical detection performance for dopamine (DA) and uric acid (UA). The nanocomposite was prepared by combining graphene oxide (GO) nanosheets with manganese porphyrins (MnTMPyP) through electrostatic interaction. Various characterization techniques confirmed the successful synthesis of the material. The modified glass carbon electrode (GCE) exhibited enhanced electrochemical characteristics, allowing for simultaneous and effective detection of DA and UA in the presence of ascorbic acid (AA) interference.
MATERIALS CHEMISTRY AND PHYSICS
(2023)
Article
Nanoscience & Nanotechnology
Fang-Hui Wu, Mei-Juan Ren, Miao Wang, Wen-Bin Sun, Kong-Lin Wu, Yuan-Sheng Cheng, Zhengquan Yan
Summary: In this study, one-dimensional nitrogen doped porous carbon nano-arrays arranged by carbon nanotube (1D CNTs@NPC) were constructed and used to modify glassy carbon electrodes for the detection of ascorbic acid, dopamine, and uric acid. The resulting electrodes showed excellent analytical performance with low detection limits and high stability and selectivity when applied to real samples. This work provides potential for efficient diagnosis of ascorbic acid, dopamine, or uric acid-related diseases in clinical testing in the future.
Article
Chemistry, Analytical
Jinjing Han, Justin M. Stine, Ashley A. Chapin, Reza Ghodssi
Summary: In this study, a novel, simple, and low-cost electrochemical sensing platform was developed for the detection of serotonin (5-HT) in artificial biological fluids. The platform utilized Nafion/carbon nanotubes and electrochemically modified carbon fiber microelectrodes to enhance the sensitivity and selectivity of 5-HT. With a customized Ag/AgCl reference electrode and Pt counter electrode, the portable 5-HT sensing platform demonstrated a sensitivity of 0.074 mu A mu M-1 and a limit of detection (LOD) of 140 nM. The system was also capable of accurately measuring 5-HT spiked in artificial urine samples, showing nearly full recovery rates.
ANALYTICAL METHODS
(2023)
Article
Materials Science, Ceramics
Nur Hawa Nabilah Azman, Yusran Sulaiman
Summary: This research presents a new supercapattery technology with a positive electrode composed of porous functionalized carbon nanofibers (pfCNFs), poly(3,4-ethylenedioxythiophene) (PEDOT), and cobalt oxide (Co3O4). The composite exhibits a flower-like structure and demonstrates high specific capacity and cycling stability, showing great potential as an electrode for supercapattery.
CERAMICS INTERNATIONAL
(2022)
Article
Energy & Fuels
Muhammad Amirul Aizat Mohd Abdah, Marliyana Mokhtar, Lee Tian Khoon, Kamaruzzaman Sopian, Nurul Akmaliah Dzulkurnain, Azizan Ahmad, Yusran Sulaiman, Federico Bella, Mohd Sukor Su'ait
Summary: P-CNFs/PEDOT/MnO2, developed as an advanced anode material through innovative combination of electrospinning, carbonization, and electrodeposition, exhibits promising electrochemical performance with high discharge capacity and low charge-transfer resistance. The experimental results suggest that this electrode has the potential to replace commercial graphite in lithium-ion batteries.
Review
Chemistry, Physical
Dharshini Mohanadas, Yusran Sulaiman
Summary: Supercapacitors are energy storage devices with remarkable properties such as high specific capacitance, fast charge/discharge rate, high power density, and long cycle life. Researchers are exploring new applications of supercapacitors, including bifunctional devices with electrochromic properties. This review focuses on the electrochromic and supercapacitive performance of carbon-based materials, conductive polymers, and metal-organic frameworks, and discusses the criteria and challenges for bifunctional electrochromic supercapacitors.
JOURNAL OF POWER SOURCES
(2022)
Article
Polymer Science
Pei Teng Lim, Nur Hawa Nabilah Azman, Shalini Kulandaivalu, Yusran Sulaiman
Summary: A ternary composite film comprising PEDOT, NCC, and Co3O4 was successfully fabricated through facile electrodeposition. The film exhibited high specific capacitance and excellent capacitance retention, as well as low equivalent series resistance, indicating its potential as an electrode material for supercapacitors.
Article
Materials Science, Multidisciplinary
Norzila Kusnin, Nor Azah Yusof, Nurul Asyikeen Ab Mutalib, Faruq Mohammad, Jaafar Abdullah, Suriana Sabri, Shuhaimi Mustafa, Ahmad Farabi Mohamad Saman, Fatin Nabilah Mohd Faudzi, Ahmed A. Soleiman
Summary: Electrochemical application has been widely used in biosensor research. In this study, a sensor electrode was improved to enhance the electrochemical conductivity for detecting small DNA molecule interactions. The electrode was modified with copper nanowires/gold nanoparticles, which were randomly distributed and compacted on the electrode surface, enhancing its electrochemical conductivity. The modified electrode exhibited efficient electrochemical conductivity of 20.3 mu A, with an increased effective surface area of 2.3-fold compared to the unmodified electrode, making it promising for biosensor applications.
Article
Optics
Nurul Illya Muhamad Fauzi, Yap Wing Fen, Jaafar Abdullah, Mazliana Ahmad Kamarudin, Nur Alia Sheh Omar, Faten Bashar Kamal Eddin, Nur Syahira Md Ramdzan, Wan Mohd Ebtisyam Mustaqim Mohd Daniyal
Summary: In this study, a GO-PVA composite thin film was successfully synthesized using spin coating techniques, and its properties and morphology were characterized. The GO-PVA thin film exhibited high absorbance and increased thickness, and showed potential for the detection of carbaryl pesticide at low concentrations of 0.02 ppb using an optical method based on surface plasmon resonance.
Article
Chemistry, Multidisciplinary
Muhammad Hafiznur Yunus, Nor Azah Yusof, Suhainie Ismail, Siti Suraiya Md Noor, Faruq Mohammad, Yusran Sulaiman, Nurul Hanun Ahmad Raston, Jaafar Abdullah, Ahmed A. Soleiman
Summary: This study proposes an improved tuberculosis diagnosis method based on an amperometry approach, which can sensitively detect the MPT64 antigen in clinical samples. The developed aptasensor is found to be simple in fabrication, sensitive, and capable of efficiently detecting and diagnosing TB in sputum samples.
Article
Chemistry, Analytical
Zixuen Gan, Muhamad Aidilfitri Mohamad Roslan, Mohd Yunus Abd Shukor, Murni Halim, Nur Adeela Yasid, Jaafar Abdullah, Ina Salwany Md Yasin, Helmi Wasoh
Summary: Aptamers are synthetic single-stranded nucleic acids generated through the SELEX technology with high affinity and specificity. While progress has been made in aptamer design and applications, only a few have achieved widespread commercial and clinical acceptance. Finding more effective ways to acquire high-affinity aptamers remains a challenge.
Article
Pharmacology & Pharmacy
Fariza Aina Abd Manan, Nor Azah Yusof, Jaafar Abdullah, Armania Nurdin
Summary: Cancer is a devastating disease with high mortality rates worldwide, leading to extensive research on drug nanocarrier vectors as a potential treatment option. In this study, a drug delivery system was developed using chitosan nanocarriers to optimize the encapsulation efficiency of an anticancer drug. The optimized parameters resulted in an encapsulation efficiency of 55.31%, and the nanocarriers showed efficient drug release in different pH conditions. The study demonstrates the potential of the synthesized MMC nanocarrier for effective drug delivery and treatment of non-muscle invasive bladder cancer.
Article
Chemistry, Physical
Muhammad Amirul Aizat Mohd Abdah, Tian Khoon Lee, Azizan Ahmad, Yusran Sulaiman, Nurul Akmaliah Dzulkarnain, Marliyana Mokhtar, Mohammad Khalid, Mohd Sukor Su'ait
Summary: CNFs/V2O5/PEDOT composite electrode shows significant enhancement in electrochemical performance in lithium-ion batteries, with initial discharge capacity of 520 mAh/g, nearly doubling that of CNFs/V2O5 electrode. However, the electrode exhibits rapid degradation due to electrode pulverization and unstable SEI formation. By applying cut-off voltages of 1.0 to 2.5 V, the cycling performance improves with enhanced charge transfer resistance, indicating that PEDOT can serve as a protective layer for the electrodes.
ACS APPLIED ENERGY MATERIALS
(2023)
Article
Chemistry, Analytical
Muhammad Hafiznur Yunus, Nor Azah Yusof, Jaafar Abdullah, Yusran Sulaiman, Nurul Hanun Ahmad Raston, Siti Suraiya Md Noor
Summary: A novel dual aptasensor was developed for the simultaneous detection of Mycobacterium tuberculosis secreted antigens CFP10 and MPT64, improving the diagnosis and control of TB.
Article
Energy & Fuels
Nur Hawa Nabilah Azman, Muhammad Mustaqhim Alias, Yusran Sulaiman
Summary: The copper-based metal-organic framework (HKUST-1) with high porosity and large specific surface area is a promising electrode material for supercapattery. The synthesized HKUST-1 exhibited an octahedral structure and a high specific surface area. The HKUST-1//N-doped graphene supercapattery device showed excellent performance with good conductivity.
Article
Energy & Fuels
Chunying Ma, Chu Zhang, Shennan Chen, Yongchun Ye, Lei Sun, Liguo Gao, Yusran Sulaiman, Tingli Ma, Miaogen Chen
Summary: Perovskite solar cells have promising potential as photovoltaic devices, but the interface between the perovskite and hole transport layer can limit their efficiency and stability. This study introduces the organic molecule BTFZA to passivate surface defects and enhance carrier transport. The modified perovskite device shows a significant increase in power conversion efficiency and maintains better performance after aging in extreme conditions.
SOLAR ENERGY MATERIALS AND SOLAR CELLS
(2023)