4.5 Article

Critical properties of the quasi-two-dimensional metallic ferromagnet Fe2.85GeTe2

Journal

JOURNAL OF PHYSICS-CONDENSED MATTER
Volume 30, Issue 34, Pages -

Publisher

IOP PUBLISHING LTD
DOI: 10.1088/1361-648X/aad43b

Keywords

critical behavior; layered structure; competing magnetic interaction

Funding

  1. Zhejiang Provincial Natural Science Foundation of China [LY14A040007, LY16A040012]
  2. National Basic Research Program of China [2016YFA0300402, 2015CB921004]
  3. National Natural Science Foundation of China [11374261]
  4. Henan Engineering Laboratory of Functional Ceramics

Ask authors/readers for more resources

We have investigated the critical behavior of Fe2.85GeTe2 single crystals near the paramagnetic-ferromagnetic transition by bulk dc magnetization measurements. The critical exponents beta gamma and delta, obtained from modified Arrott plot, Kouvel-Fisher method, and critical isothermal magnetization analysis, could fulfill the Widom scaling law. The self-consistency and reliability of these exponents are further verified by the magnetic state equations below and above the Curie temperature at high magnetic field. In addition, the exchange distance deduced from the susceptibility exponent is shown to decay as J(r) similar to r(-4.8). Based on the observations, we suggest that the competition between direct magnetic exchange and Coulombic and/or RKKY interactions should be responsible for the intrinsic magnetism in this system.

Authors

I am an author on this paper
Click your name to claim this paper and add it to your profile.

Reviews

Primary Rating

4.5
Not enough ratings

Secondary Ratings

Novelty
-
Significance
-
Scientific rigor
-
Rate this paper

Recommended

Article Physics, Condensed Matter

Metallicity and Paramagnetism of Single-Crystalline NiTe and NiTe2

Qianhui Mao, Yannan Zhang, Qin Chen, Ruixue Li, Xiaodong Geng, Jinfeng Yang, Haoshan Hao, Minghu Fang

PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS (2020)

Article Physics, Condensed Matter

Synthesis and semiconducting behavior of Zr (Cu, Fe) Se2-δ single crystals

Qianhui Mao, Xiaodong Geng, Jinfeng Yang, Ruixue Li, Haoshan Hao, Jinhu Yang, Hangdong Wang, Binjie Xu, Minghu Fang

PHYSICA B-CONDENSED MATTER (2019)

Article Physics, Applied

Superconductivity in an arc melted MoCx

Qianhui Mao, Jinfeng Yang, Ruixue Li, Haoshan Hao, Zhefeng Lou, Yuxing Zhou, Minghu Fang

PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS (2019)

Article Physics, Applied

Superconductivity in noncentrosymmetric Mo3P single crystal

Wuzhang Yang, Zhefeng Lou, Qinqing Zhu, Bin Chen, Hangdong Wang, Qianhui Mao, Jianhua Du, Jinhu Yang, Minghu Fang

SUPERCONDUCTOR SCIENCE & TECHNOLOGY (2019)

Article Physics, Condensed Matter

Magnetism and magnetocaloric effect in TlCo2-xNixS2 (0 ≤ x ≤ 0.05)

Qianhui Mao, Hangdong Wang, Jinhu Yang, HanLei Liu, Mengyang Pan, Ruixue Li, Haoshan Hao, Minghu Fang

JOURNAL OF PHYSICS-CONDENSED MATTER (2020)

Article Physics, Condensed Matter

Thermal quantum correlations in zigzag graphene nanoribbons

Xiao-Dong Tan, Qian-Hui Mao

JOURNAL OF PHYSICS-CONDENSED MATTER (2020)

Article Green & Sustainable Science & Technology

Enhancing efficiencies of solar thermophotovoltaic cells by downconversion of high-energy photons

Yuan Wang, Shao Wang, Yiwei Zhang, Qianhui Mao, Shanhe Su, Zhilin Chen

Summary: The study proposed a novel theoretical model of solar thermophotovoltaic system, with two configurations to enhance performance and considering various factors. The results show that the presence of a down converter can efficiently improve the system's performance and provide theoretical guidance for efficient solar energy harvesting.

JOURNAL OF RENEWABLE AND SUSTAINABLE ENERGY (2021)

Article Physics, Condensed Matter

Two-dimensional spin dynamics in the itinerant antiferromagnet CsCo2Se2 revealed by Cs-133-NMR measurements

Bin Chen, Jinhu Yang, Hangdong Wang, Yuhong Zhu, Qianhui Mao, Jianhua Du, Minghu Fang

Summary: In this paper, Cs-133 nuclear magnetic resonance (NMR) measurements were used to study the magnetic properties of an A-type antiferromagnet CsCo2Se2. The results showed evidence of antiferromagnetic transition at 70 K, with increasing antiferromagnetic spin fluctuations at lower temperatures. The linear relationship between T1T-T indicated that antiferromagnetic spin fluctuations are two-dimensional in the paramagnetic state.

SOLID STATE COMMUNICATIONS (2021)

Article Materials Science, Multidisciplinary

Magnetic and Critical Properties of Cr1/3NbS1.86 with T C=56 K

Qianhui Mao, Yuan Wang, Ruixue Li, Jiayun Qian, Hangdong Wang, Bin Chen, Jun Ding, Rajwali Khan, Haoshan Hao, Jinhu Yang

Summary: The magnetic and critical properties of a TeBr-transported CrNbS single crystal were studied, revealing a paramagnetic-to-ferromagnetic phase transition temperature, effective magnetic moment, and small spontaneous magnetic moment compared to effective moment. The analysis suggests dominant short-range ferromagnetic interactions and discusses the deviation of critical exponents from the theoretical model.

PHYSICA STATUS SOLIDI-RAPID RESEARCH LETTERS (2022)

Article Materials Science, Multidisciplinary

Critical behavior of ferromagnetic transition in La0.85Co1.68As2 crystal

Binjie Xu, Qianhui Mao, Yuxing Zhou, Qin Chen, Huancheng Chen, Shuijin Chen, Zhefeng Lou, Chunxiang Wu, Jianhua Du, Jinhu Yang, Hangdong Wang, Minghu Fang

Summary: The critical behavior of ferromagnetic transition in La0.85Co1.68As2 crystal with a ThCr2Si2-type structure was investigated, revealing critical exponents and characteristics of magnetic interaction. The results belong to the three-dimensional Heisenberg model and suggest short range coupling, providing important insights into the mechanism of ferromagnetism in La0.85Co1.68As2 compound.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2022)

Article Materials Science, Multidisciplinary

Observation of quantum criticality in antiferromagnetic based (Ce1_xYx)2Ir3Ge5 Kondo-Lattice system

Rajwali Khan, Khaled Althubeiti, Merfat Algethami, Nasir Rahman, Mohammad Sohail, Qianhui Mao, Quaid Zaman, Asad Ullah, Nasir Ilyas, Amir Mohammad Afzal, Alamzeb Khan, Mian Akif Safeen, Aurangzeb Khan

Summary: In this study, a detailed investigation was conducted on the (Ce1_xYx)(2)Ir3Ge5 antiferromagnetic compounds, demonstrating that the substitution of Y can decrease the antiferromagnetic phase temperature. When x=0.3, the antiferromagnetic transition temperature is suppressed to zero kelvin at an apparent antiferromagnetic quantum critical point without showing any signs of superconductivity, and the temperature dependence of heat capacity and electrical resistivity in this region display non-Fermi Liquid behavior.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2022)

Article Nanoscience & Nanotechnology

MoSi2N4/CrS2 van der Waals heterostructure with high solar-to-hydrogen efficiency

Rui-Xue Li, Xing-Ling Tian, Si-Cong Zhu, Qian-Hui Mao, Jun Ding, Hai-Dong Li

Summary: This study systematically investigates the electronic properties and photocatalytic performance of MoSi2N4/CrS2 heterostructure based on first-principle calculations. The results show that the heterostructure exhibits promising photocatalytic properties and a high solar-to-hydrogen efficiency, providing useful guidance for the design and application of MoSi2N4-based heterostructures.

PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES (2022)

Article Physics, Condensed Matter

Localized magnetism, magnetic entropy change and critical properties of Mn1/4+δNbS2 single crystals

Qianhui Mao, Yingying Xu, Ruixue Li, Yuan Wang, Haidong Li, Lisha Xue, Haoshan Hao, Rajwali Khan, Bin Chen, Jinhu Yang

Summary: The magnetic properties, magnetic entropy change, and critical behavior of Mn1/4+delta NbS2 single crystals were investigated. Two magnetic phase transitions were observed, and the effective magnetic moment and saturation moment were deduced. The magnetic entropy change exhibited two series of peaks, and the critical exponents were analyzed, indicating competing magnetic couplings in the crystal.

PHYSICA B-CONDENSED MATTER (2023)

Article Engineering, Electrical & Electronic

Fast synthesis and thermoelectric properties of BixCu2-3xSe0.95Te0.05 (x=0, 0.001, 0.002, 0.003, 0.004)

Lisha Xue, Yuan Wang, Shuangmei Zhu, Qianhui Mao, Xiaopeng Jia, Yuewen Zhang

Summary: We synthesized the quaternary copper selenide BixCu2-3xSe0.95Te0.05 compounds by high-pressure followed with ball milling method and investigated their thermoelectric properties. The crystal structure and element doping were characterized and verified by X-ray diffraction, high-resolution transmission electron microscope and X-ray photoelectron spectroscopy. Samples with x = 0.001 and 0.002 exhibited larger layered grain size and smaller grain boundary compared to other samples, which resulted in reduced resistivity and optimized electronic characteristics in a wide temperature range. Surprisingly, dislocation-induced lattice strain fluctuations caused abrupt thermal conductivity, contrary to previous results. Ultimately, a peak value of zT = 1.03 at 873 K was achieved for Bi0.001Cu1.997Se0.95Te0.05 and Bi0.002Cu1.994Se0.95Te0.05.

JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS (2023)

Article Physics, Applied

Performance analysis of photon-enhanced thermionic emission systems mediated by quantum tunneling

Yuan Wang, Aoao Ding, Haidong Li, Shaohui Liu, Qianhui Mao, Zhimin Yang, Shanhe Su

Summary: In this work, a model of a photon-enhanced thermionic emission system with a nanoscale vacuum gap is established, incorporating electron transport due to electron tunneling and near-field radiation resulting from photon tunneling. Analytical expressions for thermionic emission current, electron tunneling current, and heat flux due to near-field radiation are provided. The impacts of voltage, electron affinity, and gap distance on performance are further analyzed. Results demonstrate that the proposed system can achieve high efficiency at low-temperature cathodes, with up to 34.7% solar-to-electricity efficiency possible at a cathode temperature of 472.5 K. The proposed model offers a strategy for designing highly efficient thermionic emission devices operating at low temperatures.

JOURNAL OF APPLIED PHYSICS (2023)

No Data Available