Journal
INORGANIC CHEMISTRY
Volume 57, Issue 8, Pages 4379-4386Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.7b03271
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Funding
- NSFC [21671122, 21475078]
- Taishan Scholar's Construction Project
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A novel palladium N-heterocyclic bis-carbene dicarboxylate ligand (Pd-NHDC-H2L) was successfully synthesized. In addition, an Pd-NHDC-containing UiO-67 type MOF (UiO-67-Pd-NHDC) was prepared on the basis of a size-matched ligand mixture of biphenyl-4,4'-dicarboxylic acid/Pd-NHDC-H2L (9/1) and ZrCl4 under solvothermal conditions. The obtained UiO-67-Pd-NHC MOF can be a highly heterogeneous catalyst to promote Heck cross-coupling and intermolecular benzyne-benzyne-alkene insertion reactions.
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