Journal
DYES AND PIGMENTS
Volume 149, Issue -, Pages 246-252Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.dyepig.2017.10.003
Keywords
Perovskite quantum dots; Perhydropolysilazane; Silica composites; White light-emitting diodes; Wide color gamut
Funding
- National Research Foundation of Korea (NRF) grant - Korea government (MSIP) [NRF-2016R1A2B2013629]
- Future Key Technology Program by Korea Institute of Science and Technology [2E26960]
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In this study, highly efficient green-to-red-emitting CsPbBr3-zIz perovskite quantum dots (PQDs) with high color purity are synthesized and a facile route for the formation of PQD-inorganic SiO2 composites is proposed. To improve thermal and water stability of the PQDs, perhydropolysilazane (PHPS)-derived SiO2 composites are prepared. The CsPbBr3-SiO2 composites exhibit highly enhanced thermal stability and water stability. The green emitting CsPbBr3-SiO2 composites and red-emitting CsPbBr1.2I1.8 PQDs are coated on blue light-emitting diodes (LEDs) and the fabricated green and red LEDs show high color purities of 95.1 and 99.5%, respectively. Finally, the white LED is fabricated by combining a blue LED with CsPbBr3-SiO2 composites and CsPbBr1.2I1.8 PQDs. The fabricated white LED shows bright natural white light (luminous efficacy = 35.4 linW(-1), correlated color temperature = 5623 K) with excellent color reproducibility due to wide color gamut (127% National Television System Committee color space).
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