Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 24, Issue 21, Pages 5434-5438Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201800986
Keywords
asymmetric catalysis; carbohelicenes; circularly polarized luminescence; gold; hydroarylation
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Funding
- ACT-C from JST, Japan [JPMJCR1122YR]
- JSPS, Japan [JP26102004]
- Grants-in-Aid for Scientific Research [26102004] Funding Source: KAKEN
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The enantioselective synthesis of fully benzenoid single and double carbo[6]helicenes has been achieved via the gold-catalyzed intramolecular hydroarylation. The single crystal of the racemic double carbo[6]helicene consists of unique layer structures like timbers with halving joints in the woodworking. Furthermore, the double carbo[6]helicenes exhibited relatively large CPL activities among chiral small organic molecules.
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